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We propose the use of nanostructured photonic nanocavities made of second-order nonlinear materials as prospective passive devices to generate strongly sub-Poissonian light via single-photon blockade of an input coherent field. The simplest scheme is based on the requirement that the nanocavity be doubly resonant, i.e. possess cavity modes with good spatial overlap at both the fundamental and second-harmonic frequencies. We discuss feasibility of this scheme with state-of-the art nanofabrication technology, and the possibility to use it as a passive single-photon source on-demand.
It is shown that non-centrosymmetric materials with bulk second-order nonlinear susceptibility can be used to generate strongly antibunched radiation at an arbitrary wavelength, solely determined by the resonant behavior of suitably engineered couple
We performed quantum manipulations of the multi-level spin system S=5/2 of a Mn$^{2+}$ ion, by means of a two-tone pulse drive. The detuning between the excitation and readout radio frequency pulses allows one to select the number of photons involved
Resonant Raman spectra of single layer WS$_{2}$ flakes are presented. A second order Raman peak (2LA) appears under resonant excitation with a separation from the E$^{1}_{2g}$ mode of only $4$cm$^{-1}$. Depending on the intensity ratio and the respec
Optical nonlinearity plays a pivotal role in quantum information processing using photons, from heralded single-photon sources to long-sought quantum repeaters. Despite the availability of strong light-atom interaction, an all-optical nonlinearity is
Second order optical nonlinear processes involve the coherent mixing of two electromagnetic waves to generate a new optical frequency, which plays a central role in a variety of applications, such as ultrafast laser systems, rectifiers, modulators, a