The London penetration depth $lambda$ is the basic length scale for electromagnetic behavior in a superconductor. Precise measurements of $lambda$ as a function of temperature, field, and impurity scattering have been instrumental in revealing the na
ture of the order parameter and pairing interactions in a variety of superconductors discovered over the past decades. Here we recount our development of the tunnel-diode resonator technique to measure $lambda$ as a function of temperature and field in small single crystal samples. We discuss the principles and applications of this technique to study unconventional superconductivity in the copper oxides and other materials such as iron-based superconductors. The technique has now been employed by several groups worldwide as a precision measurement tool for the exploration of new superconductors.
Closed-topology magnetic domains are usually observed in thin films and in an applied magnetic field. Here we report the observation of rectangular cross-section tubular ferromagnetic domains in thick single crystals of CeAgSb2 in zero applied field.
Relatively low exchange energy, small net magnetic moment, and anisotropic in-plane crystal electric fields lower the domain wall energy and allow for the formation of the closed-topology patterns. Upon cycling the magnetic field, the domain structure irreversibly transforms into a dendritic open-topology pattern. This transition between closed and open topologies results in a topological magnetic hysteresis - the actual hysteresis in magnetization, not due to the imperfections and pinning, but due to the difference in the pattern morphology. Similar physics was suggested before in pure type-I superconductors and is believed to be a generic feature of other nonlinear multi-phase systems in the clean limit.
Magnetic susceptibility of non-ellipsoidal samples is a long-standing problem in experimental studies of magnetism and superconductivity. Here the quantitative description of the Meissner-London response (no Abrikosov vortices) of right circular cyli
nders in an axial magnetic field is given. The three-dimensional adaptive finite-element modeling was used to calculate the total magnetic moment, m, in a wide range of London penetration depth, lambda, to sample size ratios. By fitting the numerical data, the closed-form universal magnetic susceptibility is formulated involving only sample dimensions and lambda, thus providing a recipe for determining the London penetration depth from the accurate magnetic susceptibility measurements. Detailed examples of the experimental data analysis using the developed approach are given. The results can be extended to the frequently used cuboid-shaped samples.
A simple procedure to extract anisotropic London penetration depth components from the magnetic susceptibility measurements in realistic samples of cuboidal shape is described.
Temperature dependent $^{57}$Fe Mossbauer spectroscopy and specific heat measurements for CaK(Fe$_{1-x}$Ni$_x$)$_4$As$_4$ with $x$ = 0, 0.017, 0.033, and 0.049 are presented. No magnetic hyperfine field (e.g. no static magnetic order) down to 5.5 K w
as detected for $x$ = 0 and 0.017 in agreement with the absence of any additional feature below superconducting transition temperature, $T_c$, in the specific heat data. The evolution of magnetic hyperfine field with temperature was studied for $x$ = 0.033 and 0.049. The long-range magnetic order in these two compounds coexists with superconductivity. The magnetic hyperfine field, $B_{hf}$, (ordered magnetic moment) below $T_c$ in CaK(Fe$_{0.967}$Ni$_{0.033}$)$_4$As$_4$ is continuously suppressed with the developing superconducting order parameter. The $B_{hf}(T)$ data for CaK(Fe$_{0.967}$Ni$_{0.033}$)$_4$As$_4$, and CaK(Fe$_{0.951}$Ni$_{0.049}$)$_4$As$_4$ can be described reasonably well by Machidas model for coexistence of itinerant spin density wave magnetism and superconductivity [K. Machida, J. Phys. Soc. Jpn. {bf 50}, 2195 (1981)]. We demonstrate directly that superconductivity suppresses the spin density wave order parameter if the conditions are right, in agreement with the theoretical analysis.
The equilibrium topology of superconducting and normal domains in flat type-I superconductors is investigated. Important improvements with respect to previous work are: (1) the energy of the external magnetic field, as deformed by the presence of sup
erconducting domains, is calculated in the same way for three different topologies, and (2) calculations are made for arbitrary orientation of the applied field. A phase diagram is presented for the minimum-energy topology as a function of applied field magnitude and angle. For small (large) applied fields normal (superconducting) tubes are found, while for intermediate fields parallel domains have a lower energy. The range of field magnitudes for which the superconducting-tubes structure is favored shrinks when the field is more in-plane oriented.
