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Angle-resolved photoemission spectroscopy (ARPES) is typically used to study only the occupied electronic band structure of a material. Here we use laser-based ARPES to observe a feature in bismuth-based superconductors that, in contrast, is related to the unoccupied states. Specifically, we observe a dispersive suppression of intensity cutting across the valence band, which, when compared with relativistic one-step calculations, can be traced to two final-state gaps in the bands 6 eV above the Fermi level. This finding opens up possibilities to bring the ultra-high momentum resolution of existing laser-ARPES instruments to the unoccupied electron states. For cases where the final-state gap is not the object of study, we find that its effects can be made to vanish under certain experimental conditions.
We use time- and angle-resolved photoemission spectroscopy to characterize the dynamics of the energy gap in superconducting Bi2Sr2CaCu2O8+delta (Bi2212). Photoexcitation drives the system into a nonequilibrium pseudogap state: Near the Brillouin zon e diagonal (inside the normal-state Fermi arc), the gap completely closes for a pump fluence beyond F = 15 {mu}J/cm^2; toward the Brillouin zone face (outside the Fermi arc), it remains open to at least 24 {mu}J/cm^2. This strongly anisotropic gap response may indicate multiple competing ordering tendencies in Bi2212. Despite these contrasts, the gap recovers with relatively momentum-independent dynamics at all probed momenta, which shows the persistent influence of superconductivity both inside and outside the Fermi arc.
Single crystal metal films on insulating substrates are attractive for microelectronics and other applications, but they are difficult to achieve on macroscopic length scales. The conventional approach to obtaining such films is epitaxial growth at h igh temperature using slow deposition in ultrahigh vacuum conditions. Here we describe a different approach: sputter deposition at modest temperatures followed by annealing to induce secondary grain growth. We show that polycrystalline as-deposited Cu on alpha-Al2O3(0001) can be transformed into Cu(111) with centimeter-sized grains. Employing optical microscopy, x-ray diffraction, and electron backscatter diffraction to characterize the films before and after annealing, we find a particular as-deposited grain structure that promotes the growth of giant grains upon annealing. To demonstrate one potential application of such films, we grow graphene by chemical vapor deposition on wafers of annealed Cu and obtain epitaxial graphene grains of 0.2 mm diameter.
228 - L. Miller , T.J. Turner 2013
Active Galactic Nuclei (AGN) show excess X-ray emission above 10 keV compared with extrapolation of spectra from lower energies. Risaliti et al. have recently attempted to model the hard X-ray excess in the type 1.8 AGN NGC 1365, concluding that the hard excess most likely arises from Compton-scattered reflection of X-rays from an inner accretion disk close to the black hole. Their analysis disfavored a model in which the hard excess arises from a high column density of circumnuclear gas partially covering a primary X-ray source, despite such components being required in the NGC 1365 data below 10 keV. Using a Monte Carlo radiative transfer approach, we demonstrate that this conclusion is invalidated by (i) use of slab absorption models, which have unrealistic transmission spectra for partial covering gas, (ii) neglect of the effect of Compton scattering on transmitted spectra and (iii) inadequate modeling of the spectrum of scattered X-rays. The scattered spectrum is geometry dependent and, for high global covering factors, may dominate above 10 keV. We further show that, in models of circumnuclear gas, the suppression of the observed hard X-ray flux by reprocessing may be no larger than required by the `light bending model invoked for inner disk reflection, and the expected emission line strengths lie within the observed range. We conclude that the time-invariant `red wing in AGN X-ray spectra is probably caused by continuum transmitted through and scattered from circumnuclear gas, not by highly redshifted line emission, and that measurement of black hole spin is not possible.
A likelihood-based method for measuring weak gravitational lensing shear in deep galaxy surveys is described and applied to the Canada-France-Hawaii Telescope (CFHT) Lensing Survey (CFHTLenS). CFHTLenS comprises 154 sq deg of multicolour optical data from the CFHT Legacy Survey, with lensing measurements being made in the i band to a depth i(AB)<24.7, for galaxies with signal-to-noise ratio greater than about 10. The method is based on the lensfit algorithm described in earlier papers, but here we describe a full analysis pipeline that takes into account the properties of real surveys. The method creates pixel-based models of the varying point spread function (PSF) in individual image exposures. It fits PSF-convolved two-component (disk plus bulge) models, to measure the ellipticity of each galaxy, with bayesian marginalisation over model nuisance parameters of galaxy position, size, brightness and bulge fraction. The method allows optimal joint measurement of multiple, dithered image exposures, taking into account imaging distortion and the alignment of the multiple measurements. We discuss the effects of noise bias on the likelihood distribution of galaxy ellipticity. Two sets of image simulations that mirror the observed properties of CFHTLenS have been created, to establish the methods accuracy and to derive an empirical correction for the effects of noise bias.
We present data products from the Canada-France-Hawaii Telescope Lensing Survey (CFHTLenS). CFHTLenS is based on the Wide component of the Canada-France-Hawaii Telescope Legacy Survey (CFHTLS). It encompasses 154 deg^2 of deep, optical, high-quality, sub-arcsecond imaging data in the five optical filters u^*griz. The article presents our data processing of the complete CFHTLenS data set. We were able to obtain a data set with very good image quality and high-quality astrometric and photometric calibration. Our external astrometric accuracy is between 60-70 mas with respect to SDSS data and the internal alignment in all filters is around 30 mas. Our average photometric calibration shows a dispersion on the order of 0.01 to 0.03 mag for griz and about 0.04 mag for u^* with respect to SDSS sources down to i <= 21. In the spirit of the CFHTLS all our data products are released to the astronomical community via the Canadian Astronomy Data Centre. We give a description and how-to manuals of the public products which include image pixel data, source catalogues with photometric redshift estimates and all relevant quantities to perform weak lensing studies.
In this Letter, we derive an effective theory of graphene on a hexagonal Boron Nitride (h-BN) substrate. We show that the h-BN substrate generically opens a spectral gap in graphene despite the lattice mismatch. The origin of that gap is particularly intuitive in the regime of strong coupling between graphene and its substrate, when the low-energy physics is determined by the topology of a network of zero energy modes. For twisted graphene bilayers, where inversion symmetry is present, this network percolates through the system and the spectrum is gapless. The breaking of that symmetry by h-BN causes the zero energy modes to close into rings. The eigenstates of these rings hybridize into flat bands with gaps in between. The size of this band gap can be tuned by a gate voltage and it can reach the order of magnitude needed to confine electrons at room temperature.
Films of (111)-textured Cu, Ni, and Cu$_x$Ni$_y$ were evaluated as substrates for chemical vapor deposition of graphene. A metal thickness of 400 nm to 700 nm was sputtered onto a substrate of $alpha-$Al$_2$O$_3$(0001) at temperatures of 250 C to 650 C. The films were then annealed at 1000 C in a tube furnace. X-ray and electron backscatter diffraction measurements showed all films have (111) texture but have grains with in-plane orientations differing by $60^{circ}$. The in-plane epitaxial relationship for all films was $[110]_{metal}$||$[10bar{1}0]_{{Al}_{2}{O}_{3}}$. Reactive sputtering of Al in O$_2$ before metal deposition resulted in a single in-plane orientation over 97 % of the Ni film but had no significant effect on the Cu grain structure. Transmission electron microscopy showed a clean Ni/Al$_2$O$_3$ interface, confirmed the epitaxial relationship, and showed that formation of the $60^{circ}$ twin grains was associated with features on the Al$_2$O$_3$ surface. Increasing total pressure and Cu vapor pressure during annealing decreased the roughness of Cu and and Cu$_x$Ni$_y$ films. Graphene grown on the Ni(111) films was more uniform than that grown on polycrystalline Ni/SiO$_2$ films, but still showed thickness variations on a much smaller length scale than the distance between grains.
We use computer simulations to investigate the stability of a two-component polymer brush de-mixing on a curved template into phases of different morphological properties. It has been previously shown via molecular dynamics simulations that immiscibl e chains having different length and anchored to a cylindrical template will phase separate into striped phases of different widths oriented perpendicularly to the cylindrical axis. We calculate free energy differences for a variety of stripe widths, and extract simple relationships between the sizes of the two polymers, N_1 and N_2, and the free energy dependence on the stripe width. We explain these relationships using simple physical arguments based upon previous theoretical work on the free energy of polymer brushes.
168 - L. Miller , T.J. Turner 2011
Reverberation from scattering material around the black hole in active galactic nuclei is expected to produce a characteristic signature in a Fourier analysis of the time delays between directly-viewed continuum emission and the scattered light. Narr ow-line Seyfert 1 galaxies (NLS1) are highly variable at X-ray energies, and are ideal candidates for the detection of X-ray reverberation. We show new analysis of a small sample of NLS1 that clearly shows the expected time-delay signature, providing strong evidence for the existence of a high covering fraction of scattering and absorbing material a few tens to hundreds of gravitational radii from the black hole. We also show that an alternative interpretation of time delays in the NLS1 1H0707-495, as arising about one gravitational radius from the black hole, is strongly disfavoured in an analysis of the energy-dependence of the time delays.
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