اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدWave-diffusion theory of spin transport in metals after ultrashort-pulse excitation
141
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
Spin and charge-current dynamics after ultrafast spin-polarized excitation in a normal metal are studied theoretically using a wave-diffusion theory. It is shown analytically how this macroscopic approach correctly describes the ballistic and diffusive properties of spin and charge transport, but also applies to the intermediate regime between these two limits. Using the wave-diffusion equations we numerically analyze spin and charge dynamics after ultrafast excitation of spin polarized carriers in thin gold films. Assuming slightly spin-dependent momentum relaxation times, we find that a unified treatment of diffusive and ballistic transport yields robust signatures in the spin and charge dynamics, which are in qualitative agreement with recent experimental results [Phys. Rev. Lett 107, 076601 (2011)]. The influence of boundary effects on the temporal signatures of spin transport is also studied.
قيم البحث
اقرأ أيضاً
The out-of-equilibrium dynamics of electrons and phonons upon laser excitation are often described by the two-temperature model, which assumes that both subsystems are separately in thermal equilibrium. However, recent experiments show that this desc
ription is not sufficient to describe the out-of-equilibrium dynamics on ultrashort timescales. Here, we extend and apply a parameter-free microscopic out-of-equilibrium model to describe the ultrafast laser-induced system dynamics of archetypical metallic systems such as gold, aluminum, iron, nickel, and cobalt. We report strong deviations from the two-temperature model on the picosecond timescale for all the materials studied, even for those where the assumption of separate thermal equilibriums seemed less restrictive, like in gold. Furthermore, we demonstrate the importance of the phonon-mode dependent electron-phonon coupling for the relaxation process and reveal the significance of this channel in the lattice equilibration through an indirect coupling between phonons via the electronic system.
We present measurements of pure spin current absorption on lateral spin valves. By varying the width of the absorber we demonstrate that spin current absorption measurements enable to characterize efficiently the spin transport properties of ferromag
netic elements. The analytical model used to describe the measurement takes into account the polarization of the absorber. The analysis of the measurements allows thus determining the polarization and the spin diffusion length of a studied material independently, contrarily to most experiments based on lateral spin valves where those values are entangled. We report the spin transport parameters of some of the most important materials used in spinorbitronics (Co60Fe40, Ni81Fe19, Co, Pt, and Ta), at room and low (10 K) temperatures.
Relaxation dynamics of embedded metal nanoparticles after ultrafast laser pulse excitation is driven by thermal phenomena of different origins the accurate description of which is crucial for interpreting experimental results: hot electron gas genera
tion, electron-phonon coupling, heat transfer to the particle environment and heat propagation in the latter. Regardingthis last mechanism, it is well known that heat transport in nanoscale structures and/or at ultrashort timescales may deviate from the predictions of the Fourier law. In these cases heat transport may rather be described by the Boltzmann transport equation. We present a numerical model allowing us to determine the electron and lattice temperature dynamics in a spherical gold nanoparticle core under subpicosecond pulsed excitation, as well as that of the surrounding shell dielectric medium. For this, we have used the electron-phonon coupling equation in the particle with a source term linked with the laser pulse absorption, and the ballistic-diffusive equations for heat conduction in the host medium. Either thermalizing or adiabatic boundary conditions have been considered at the shell external surface. Our results show that the heat transfer rate from the particle to the matrix can be significantly smaller than the prediction of Fouriers law. Consequently, the particle temperature rise is larger and its cooling dynamics might be slower than that obtained by using Fouriers law. This difference is attributed to the nonlocal and nonequilibrium heat conduction in the vicinity of the core nanoparticle. These results are expected to be of great importance for analyzing pump-probe experiments performed on single nanoparticles or nanocomposite media.
We use the Boltzmann transport theory in the relaxation time approximation to describe the thermal transport of spin waves in a ferromagnet. By treating spin waves as magnon excitations we are able to compute analytically and numerically the coeffici
ents of the constitutive thermo-magnetic transport equations. As a main result, we find that the absolute thermo-magnetic power coefficient $epsilon_M$, relating the gradient of the potential of the magnetization current and the gradient of the temperature, in the limit of low temperature and low field, is a constant $epsilon_M = -0.6419 , k_B/mu_B$. The theory correctly describes the low-temperature and magnetic-field dependencies of spin Seebeck experiments. Furthermore, the theory predicts that in the limit of very low temperatures the spin Peltier coefficient $Pi_M$, relating the heat and the magnetization currents, tends to a finite value which depends on the amplitude of the magnetic field. This indicates the possibility to exploit the spin Peltier effect as an efficient cooling mechanism in cryogenics.
We present a microcavity structure with a shifted photonic stop-band to enable efficient non-resonant injection of a polariton condensate with spectrally broad femtosecond pulses. The concept is demonstrated theoretically and confirmed experimentally
for a planar GaAs/AlGaAs multilayer heterostructure pumped with ultrashort near-infrared pulses while photoluminescence is collected to monitor the optically injected polariton density. As the excitation wavelength is scanned, a regime of polariton condensation can be reached in our structure at a consistently lower fluence threshold than in a state-of-the-art conventional microcavity. Our microcavity design improves the polariton injection efficiency by a factor of 4, as compared to a conventional microcavity design, when broad excitation pulses are centered at a wavelength of 740 nm. Most remarkably, this improvement factor reaches 270 when the excitation wavelength is centered at 750 nm.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
