اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدNear-field examination of perovskite-based superlenses and superlens-enhanced probe-object coupling
68
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
A planar slab of negative index material works as a superlens with sub-diffraction-limited imaging resolution, since propagating waves are focused and, moreover, evanescent waves are reconstructed in the image plane. Here, we demonstrate a superlens for electric evanescent fields with low losses using perovskites in the mid-infrared regime. The combination of near-field microscopy with a tunable free-electron laser allows us to address precisely the polariton modes, which are critical for super-resolution imaging. We spectrally study the lateral and vertical distributions of evanescent waves around the image plane of such a lens, and achieve imaging resolution of wavelength/14 at the superlensing wavelength. Interestingly, at certain distances between the probe and sample surface, we observe a maximum of these evanescent fields. Comparisons with numerical simulations indicate that this maximum originates from an enhanced coupling between probe and object, which might be applicable for multifunctional circuits, infrared spectroscopy, and thermal sensors.
قيم البحث
اقرأ أيضاً
The coherent exchange of optical near fields between two neighboring dipoles plays an essential role for the optical properties, quantum dynamics and thus for the function of many naturally occurring and artificial nanosystems. These interactions are
inherently short-ranged, extending over a few nanometers only, and depend sensitively on relative orientation, detuning and dephasing, i.e., on the vectorial properties of the coupled dipolar near fields. This makes it challenging to analyze them experimentally. Here, we introduce plasmonic nanofocusing spectroscopy to record coherent light scattering spectra with 5-nm spatial resolution from a small dipole antenna, excited solely by evanescent fields and coupled to plasmon resonances in a single gold nanorod. We resolve mode couplings, resonance energy shifts and Purcell effects as a function of dipole distance and relative orientation, and show how they arise from different vectorial components of the interacting optical near-fields. Our results pave the way for using dipolar alignment to control the optical properties and function of nanoscale systems.
Near-field scanning optical microscopy has been an indispensable tool for designing, characterizing and understanding the functionalities of diverse nanoscale photonic devices. As the advances in fabrication technology have driven the devices smaller
and smaller, the demand has grown steadily for improving its resolving power, which is determined mainly by the size of the probe attached to the scanner. The use of a smaller probe has been a straightforward approach to increase the resolving power, but it cannot be made arbitrarily small in practice due to the steep reduction of the collection efficiency. Here, we develop a method to enhance the resolving power of near-field imaging beyond the limit set by the physical size of the probe aperture. The main working principle is to unveil high-order near-field eigenmodes invisible with conventional near-field microscopy. The destructive interference of near-field waves is induced in these high-order eigenmodes by the locally varying phases, which can reveal subaperture-scale fine structural details. To extract these eigenmodes, we construct a self-interference near-field microscopy system and measure a fully phase-referenced far- to near-field transmission matrix (FNTM) composed of near-field amplitude and phase maps recorded for various angles of far-field illumination. By the singular value decomposition of the measured FNTM, we could extract the antisymmetric mode, quadrupole mode, and other higher-order modes hidden under the lowest-order symmetric mode. This enables us to resolve double and triple nano-slots whose gap size (50 nm) is three times smaller than the diameter of the probe aperture (150 nm). The subaperture near-field mode mapping by the FTNM can be potentially combined with various existing near-field imaging modalities and promote their ability to interrogate local near-field optical waves of nanoscale devices.
Recent theoretical and experimental studies have shown that imaging with resolution well beyond the diffraction limit can be obtained with so-called superlenses. Images formed by such superlenses are, however, in the near field only, or a fraction of
wavelength away from the lens. In this paper, we propose a far-field superlens (FSL) device which is composed of a planar superlens with periodical corrugation. We show in theory that when an object is placed in close proximity of such a FSL, a unique image can be formed in far-field. As an example, we demonstrate numerically that images of 40 nm lines with a 30 nm gap can be obtained from far-field data with properly designed FSL working at 376nm wavelength.
We present experimental evidence of plasmonic-enhanced optical tweezers, of polystyrene beads in deionized water in the vicinity of metal-coated nanostructures. The optical tweezers operate with a continuous wave (CW) near-infrared laser. We employ a
Cu/Au bilayer that significantly improves dissipation of heat generated by the trapping laser beam and avoid de-trapping from heat convection currents. We investigate the improvement of the optical trapping force, the effective trapping quality factor, and observe an exponential distance dependence of the trapping force from the nanostructures, expected from the evanescent plasmon field.
We demonstrate a high-performance apertureless near-field probe made of a tapered metal tip with a set of periodic shallow grooves near the apex. The spontaneous emission from a single emitter near the tip is investigated systematically for the side-
illumination tip enhanced spectroscopy (TES). In contrast with the bare tapered metal tip in conventional side-illumination TES, the corrugated probe not only enhances strongly local excitation field but also concentrates the emission directivity, which leads to high collection efficiency and signal-to-noise ratio. In particular, we propose an asymmetric TES tip based on two coupling nanorods with different length at the apex to realize unidirectional enhanced emission rate from a single emitter. Interestingly, we find that the radiation pattern is sensitive to the emission wavelength and the emitter positions respective to the apex, which can result in an increase of signal-to-noise ratio by suppressing undesired signal. The proposed asymmetrical corrugated probe opens up a broad range of practical applications, e.g. increasing the detection efficiency of tip enhanced spectroscopy at the single-molecule level.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
