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We examine the effect of decoherence and intermolecular interactions (chiral discrimination energies) on the chiral stability and the distinguishability of initially pure versus mixed states in an open chiral system. Under a two-level approximation for a system, intermolecular interactions are introduced by a mean-field theory, and interaction between a system and an environment is modeled by a continuous measurement of a population difference between the two chiral states. The resultant equations are explored for various parameters, with emphasis on the combined effects of the initial condition of the system, the chiral discrimination energy and the decoherence. We focus on factors affecting the distinguishability as measured by population difference between the initially pure and mixed states and on the chiral stability as measured by the purity decay.
We examine how initial coherences in open chiral systems affect distinguishability of pure versus mixed states and purity decay. Interaction between a system and an environment is modeled by a continuous position measurement and a two-level approxima
The physical origin of the so-called chirality-induced spin selectivity (CISS) effect has puzzled experimental and theoretical researchers over the past few years. Early experiments were interpreted in terms of unconventional spin-orbit interactions
We study theoretically and experimentally the infrared (IR) spectrum of an adamantane monolayer on a Au(111) surface. Using a new STM-based IR spectroscopy technique (IRSTM) we are able to measure both the nanoscale structure of an adamantane monolay
Distinguishability and predictability are part of complementarity relations which apply to two different kinds of interference experiments, with and without a path-detector, respectively. In [Opt. Comm. 179, 337 (2000)], Englert and Bergou pointed ou
We address the time evolution of the quantum correlations ($QCs$) such as entanglement, purity, and coherence for a model of two non-interacting qubits initially prepared as a maximally entangled bipartite state. We contrast the comparative potential