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We report on the realization of quantum degenerate gas mixtures of the alkaline-earth element strontium with the alkali element rubidium. A key ingredient of our scheme is sympathetic cooling of Rb by Sr atoms that are continuously laser cooled on a narrow linewidth transition. This versatile technique allows us to produce ultracold gas mixtures with a phase-space density of up to 0.06 for both elements. By further evaporative cooling we create double Bose-Einstein condensates of 87Rb with either 88Sr or 84Sr, reaching more than 10^5 condensed atoms per element for the 84Sr-87Rb mixture. These quantum gas mixtures constitute an important step towards the production of a quantum gas of polar, open-shell RbSr molecules.
We report on an improved scheme to generate Bose-Einstein condensates (BECs) and degenerate Fermi gases of strontium. This scheme allows us to create quantum gases with higher atom number, a shorter time of the experimental cycle, or deeper quantum d egeneracy than before. We create a BEC of 84-Sr exceeding 10^7 atoms, which is a 30-fold improvement over previously reported experiments. We increase the atom number of 86-Sr BECs to 2.5x10^4 (a fivefold improvement), and refine the generation of attractively interacting 88-Sr BECs. We present a scheme to generate 84-Sr BECs with a cycle time of 2s, which, to the best of our knowledge, is the shortest cycle time of BEC experiments ever reported. We create deeply-degenerate 87-Sr Fermi gases with T/T_F as low as 0.10(1), where the number of populated nuclear spin states can be set to any value between one and ten. Furthermore, we report on a total of five different double-degenerate Bose-Bose and Bose-Fermi mixtures. These studies prepare an excellent starting point for applications of strontium quantum gases anticipated in the near future.
We report on the creation of ultracold 84Sr2 molecules in the electronic ground state. The molecules are formed from atom pairs on sites of an optical lattice using stimulated Raman adiabatic passage (STIRAP). We achieve a transfer efficiency of 30% and obtain 4x10^4 molecules with full control over the external and internal quantum state. STIRAP is performed near the narrow 1S0-3P1 intercombination transition, using a vibrational level of the 0u potential as intermediate state. In preparation of our molecule association scheme, we have determined the binding energies of the last vibrational levels of the 0u, 1u excited-state, and the 1Sigma_g^+ ground-state potentials. Our work overcomes the previous limitation of STIRAP schemes to systems with Feshbach resonances, thereby establishing a route that is applicable to many systems beyond bi-alkalis.
Fermionic 87Sr has a nuclear spin of I=9/2, higher than any other element with similar electronic structure. This large nuclear spin has many applications in quantum simulation and computation, for which preparation and detection of the spin state ar e requirements. For an ultracold 87Sr cloud, we show two complementary methods to characterize the spin-state mixture: optical Stern-Gerlach state separation and state-selective absorption imaging. We use these methods to optimize the preparation of a variety of spin-state mixtures by optical pumping and to measure an upper bound of the 87Sr spin relaxation rate.
We report on the attainment of Bose-Einstein condensation of 86Sr. This isotope has a scattering length of about +800 a0 and thus suffers from fast three-body losses. To avoid detrimental atom loss, evaporative cooling is performed at low densities a round 3x10^12 cm^-3 in a large volume optical dipole trap. We obtain almost pure condensates of 5x10^3 atoms.
We report on the attainment of a spin-polarized Fermi sea of 87-Sr in thermal contact with a Bose-Einstein condensate (BEC) of 84-Sr. Interisotope collisions thermalize the fermions with the bosons during evaporative cooling. A degeneracy of T/T_F=0. 30(5) is reached with 2x10^4 87-Sr atoms together with an almost pure 84-Sr BEC of 10^5 atoms.
We present the essential experimental steps of our all-optical approach to prepare a double-degenerate Fermi-Fermi mixture of 6Li and 40K atoms, which then serves as a starting point for molecule formation. We first describe the optimized trap loadin g procedures, the internal-state preparation of the sample, and the combined evaporative and sympathetic cooling process. We then discuss the preparation of the sample near an interspecies Feshbach resonance, and we demonstrate the formation of heteronuclear molecules by a magnetic field ramp across the resonance.
We report on the attainment of Bose-Einstein condensation with ultracold strontium atoms. We use the 84Sr isotope, which has a low natural abundance but offers excellent scattering properties for evaporative cooling. Accumulation in a metastable stat e using a magnetic-trap, narrowline cooling, and straightforward evaporative cooling in an optical trap lead to pure condensates containing 1.5x10^5 atoms. This puts 84Sr in a prime position for future experiments on quantum-degenerate gases involving atomic two-electron systems.
We investigate the collisional stability of a sample of 40K atoms immersed in a tunable spin mixture of 6Li atoms. In this three-component Fermi-Fermi mixture, we find very low loss rates in a wide range of interactions as long as molecule formation of 6Li is avoided. The stable fermionic mixture with two resonantly interacting spin states of one species together with another species is a promising system for a broad variety of phenomena in few- and many-body quantum physics.
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