It is proposed that the ground-state manifold of the neutral nitrogen-vacancy center in diamond could be used as a quantum two-level system in a solid-state-based implementation of a broadband, noise-free quantum optical memory. The proposal is based
on the same-spin $Lambda$-type three-level system created between the two E orbital ground states and the A$_1$ orbital excited state of the center, and the cross-linear polarization selection rules obtained with the application of transverse electric field or uniaxial stress. Possible decay and decoherence mechanisms of this system are discussed, and it is shown that high-efficiency, noise-free storage of photons as short as a few tens of picoseconds for at least a few nanoseconds could be possible at low temperature.
It is shown that a classical optical Fourier processor can be used for the shaping of quantum correlations between two or more photons, and the class of Fourier masks applicable in the multiphoton Fourier space is identified. This concept is experime
ntally demonstrated using two types of periodic phase masks illuminated with path-entangled photon pairs, a highly non-classical state of light. Applied first were sinusoidal phase masks, emulating two-particle quantum walk on a periodic lattice, yielding intricate correlation patterns with various spatial bunching and anti-bunching effects depending on the initial state. Then, a periodic Zernike-like filter was applied on top of the sinusoidal phase masks. Using this filter, phase information lost in the original correlation measurements was retrieved.
We consider the propagation of classical and non-classical light in multi-mode optical waveguides. We focus on the evolution of the few-photon correlation functions, which, much like the light-intensity distribution in such systems, evolve in a perio
dic manner, culminating in the revival of the initial correlation pattern at the end of each period. It is found that when the input state possesses non trivial symmetries, the correlation revival period can be longer than that of the intensity, and thus the same intensity pattern can display different correlation patterns. We experimentally demonstrate this effect for classical, pseudo-thermal light, and compare the results with the predictions for non-classical, quantum light.
We experimentally show that two-photon path-entangled states can be coherently manipulated by multi-mode interference in multi-mode waveguides. By measuring the output two-photon spatial correlation function versus the phase of the input state, we sh
ow that multi-mode waveguides perform as nearly-ideal multi-port beam splitters at the quantum level, creating a large variety of entangled and separable multi-path two-photon states.
We demonstrate control over the spin state of a semiconductor quantum dot exciton using a polarized picosecond laser pulse slightly detuned from a biexciton resonance. The control pulse follows an earlier pulse, which generates an exciton and initial
izes its spin state as a coherent superposition of its two non-degenerate eigenstates. The control pulse preferentially couples one component of the exciton state to the biexciton state, thereby rotating the excitons spin direction. We detect the rotation by measuring the polarization of the exciton spectral line as a function of the time-difference between the two pulses. We show experimentally and theoretically how the angle of rotation depends on the detuning of the second pulse from the biexciton resonance.
We detect a novel radiative cascade from a neutral semiconductor quantum dot. The cascade initiates from a metastable biexciton state in which the holes form a spin-triplet configuration, Pauli-blockaded from relaxation to the spin-singlet ground sta
te. The triplet biexciton has two photon-phonon-photon decay paths. Unlike in the singlet-ground state biexciton radiative cascade, in which the two photons are co-linearly polarized, in the triplet biexciton cascade they are crosslinearly polarized. We measured the two-photon polarization density matrix and show that the phonon emitted when the intermediate exciton relaxes from excited to ground state, preserves the excitons spin. The phonon, thus, does not carry with it any which-path information other than its energy. Nevertheless, entanglement distillation by spectral filtering was found to be rather ineffective for this cascade. This deficiency results from the opposite sign of the anisotropic electron-hole exchange interaction in the excited exciton relative to that in the ground exciton.
We measured, for the first time, two photon radiative cascades due to sequential recombination of quantum dot confined electron hole pairs in the presence of an additional spectator charge carrier. We identified direct, all optical cascades involving
spin blockaded intermediate states, and indirect cascades, in which non radiative relaxation precedes the second recombination. Our measurements provide also spin dephasing rates of confined carriers.
We measured the polarization memory of excitonic and biexcitonic optical transitions from single quantum dots at either positive, negative or neutral charge states. Positive, negative and no circular or linear polarization memory was observed for var
ious spectral lines, under the same quasi-resonant excitation below the wetting layer band-gap. We developed a model which explains both qualitatively and quantitatively the experimentally measured polarization spectrum for all these optical transitions. We consider quite generally the loss of spin orientation of the photogenerated electron-hole pair during their relaxation towards the many-carrier ground states. Our analysis unambiguously demonstrates that while electrons maintain their initial spin polarization to a large degree, holes completely dephase.
We present an experimental and theoretical study of the polarized photoluminescence spectrum of single semiconductor quantum dots in various charge states. We compare our high resolution polarization sensitive spectral measurements with a new many-ca
rrier theoretical model, which was developed for this purpose. The model considers both the isotropic and anisotropic exchange interactions between all participating electron-hole pairs. With this addition, we calculate both the energies and polarizations of all optical transitions between collective, quantum dot confined charge carrier states. We succeed in identifying most of the measured spectral lines. In particular, the lines resulting from singly-, doubly- and triply- negatively charged excitons and biexcitons. We demonstrate that lines emanating from evenly charged states are linearly polarized. Their polarization direction does not necessarily coincide with the traditional crystallographic direction. It depends on the shells of the single carriers, which participate in the recombination process.
