Asymmetric parametric generation of images with nonlinear dielectric metasurfaces

Subwavelength dielectric resonators assembled into metasurfaces have become versatile tools to miniaturise optical components towards the nanoscale. An important class of such functionalities is associated with asymmetries in both generation and propagation of light with respect to reversals of the positions of transmitters and receivers. A promising pathway towards miniaturisation of asymmetric light control is via nonlinear light-matter interactions. Here we demonstrate asymmetric parametric generation of light at the level of individual subwavelength resonators. We assemble thousands of dissimilar nonlinear dielectric resonators into translucent metasurfaces that produce images in the visible spectral range when illuminated by infrared radiation. By design, these nonlinear metasurfaces produce different and completely independent images for the reversed directions of illumination, that is when the positions of the infrared transmitter and the visible light receiver are exchanged. Nonlinearity-enabled asymmetric control of light at the level of individual subwavelength resonators opens an untapped potential for developing novel nanophotonic components via dense integration of large quantities of nonlinear resonators into compact metasurfaces.

Nanoscale topological corner states in nonlinear optics

Topological states of light have received significant attention due to the existence of counter-intuitive nontrivial boundary effects originating from the bulk properties of optical systems. Such boundary states, having their origin in topological properties of the bulk, are protected from perturbations and defects, and they show promises for a wide range of applications in photonic circuitry. The bulk-boundary correspondence relates the N-dimensional bulk modes to (N-1)-dimensional boundary states. Recently, the bulk-boundary correspondence was generalized to higher-order effects such that an N-dimensional bulk defines its (N-M)-dimensional boundary states. Prominent examples are topological corner states of light in two-dimensional structures that have been realized at the micrometer-scale. Such corner states, due to their tight confinement in all directions, provide a novel route towards topological cavities. Here we bring the concept of topological corner states to the nanoscale for enhancing nonlinear optical processes. Specifically, we design topologically nontrivial hybrid metasurfaces with C6-symmetric honeycomb lattices supporting both edge and corner states. We report on direct observations of nanoscale topology-empowered localization of light in corner states revealed via a nonlinear imaging technique. Nanoscale topological corner states pave the way towards on-chip applications in compact classical and quantum nanophotonic devices.

Topological nanophotonics for photoluminescence control

Rare-earth doped nanocrystals are emerging light sources used for many applications in nanotechnology enabled by human ability to control their various optical properties with chemistry and material science. However, one important optical problem -- polarisation of photoluminescence -- remains largely out of control by chemistry methods. Control over photoluminescence polarisation can be gained via coupling of emitters to resonant nanostructures such as optical antennas and metasurfaces. However, the resulting polarization is typically sensitive to position disorder of emitters, which is difficult to mitigate. Recently, new classes of disorder-immune optical systems have been explored within the framework of topological photonics. Here we explore disorder-robust topological arrays of Mie-resonant nanoparticles for polarisation control of photoluminescence of nanocrystals. We demonstrate polarized emission from rare-earth-doped nanocrystals governed by photonic topological edge states supported by zigzag arrays of dielectric resonators. We verify the topological origin of polarised photoluminescence by comparing emission from nanoparticles coupled to topologically trivial and nontrivial arrays of nanoresonators.

Topological states in disordered arrays of dielectric nanoparticles

We study the interplay between disorder and topology for the localized edge states of light in topological zigzag arrays of resonant dielectric nanoparticles. We characterize topological properties by the winding number that depends on both zigzag angle and spacing between nanoparticles in the array. For equal-spacing arrays, the system may have two values of the winding number $ u=0$ or $1$, and it demonstrates localization at the edges even in the presence of disorder, being consistent with experimental observations for finite-length nanodisk structures. For staggered-spacing arrays, the system possesses richer topological phases characterized by the winding numbers $ u=0$, $1$ or $2$, which depend on the averaged zigzag angle and disorder strength. In a sharp contrast to the equal-spacing zigzag arrays, staggered-spacing arrays reveal two types of topological phase transitions induced by the angle disorder, (i) $ u = 0 leftrightarrow u = 1$ and (ii) $ u = 1 leftrightarrow u = 2$. More importantly, the spectrum of staggered-spacing arrays may remain gapped even in the case of a strong disorder.

Individual nanoantennas empowered by bound states in the continuum for nonlinear photonics

Bound states in the continuum (BICs) represent localized modes with energies embedded in the continuous spectrum of radiating waves. BICs were discovered initially as a mathematical curiosity in quantum mechanics, and more recently were employed in photonics. Pure mathematical bound states have infinitely-large quality factors (Q factors) and zero resonant linewidth. In optics, BICs are physically limited by a finite size, material absorption, structural disorder, and surface scattering, and they manifest themselves as the resonant states with large Q factors, also known as supercavity modes or quasi-BICs. Optical BIC resonances have been demonstrated only in extended 2D and 1D systems and have been employed for distinct applications including lasing and sensing. Optical quasi-BIC modes in individual nanoresonators have been discovered recently but they were never observed in experiment. Here, we demonstrate experimentally an isolated subwavelength nanoresonator hosting a quasi-BIC resonance. We fabricate the resonator from AlGaAs material on an engineered substrate, and couple to the quasi-BIC mode using structured light. We employ the resonator as a nonlinear nanoantenna and demonstrate record-high efficiency of second-harmonic generation. Our study brings a novel platform to resonant subwavelength photonics.

Third-harmonic generation in photonic topological metasurfaces

We study nonlinear effects in two-dimensional photonic metasurfaces supporting topologically-protected helical edge states at the nanoscale. We observe strong third-harmonic generation mediated by optical nonlinearities boosted by multipolar Mie resonances of silicon nanoparticles. Variation of the pump-beam wavelength enables independent high-contrast imaging of either bulk modes or spin-momentum-locked edge states. We demonstrate topology-driven tunable localization of the generated harmonic fields and map the pseudospin-dependent unidirectional waveguiding of the edge states bypassing sharp corners. Our observations establish dielectric metasurfaces as a promising platform for the robust generation and transport of photons in topological photonic nanostructures.