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CO2 laser-driven electron acceleration is demonstrated with particle-in-cell simulation in low-density plasma. An intense CO2 laser pulse with long wavelength excites wakefield. The bubble behind it has a broad space to sustain a large amount of elec trons before reaching its charge saturation limit. A transversely propagating inject pulse is used to induce and control the ambient electron injection. The accelerated electron bunch with total charge up to 10 nC and the average charge per energy interval of more than 0.6 nC/MeV are obtained. Plasma-based electron acceleration driven by intense CO2 laser provides a new potential way to generate high-charge electron bunch with low energy spread, which has broad applications, especially for X-ray generation by table-top FEL and bremsstrahlung.
Subwavelength semiconductor nanowires have recently attracted interest for photonic applications because they possess various unique optical properties and offer great potential for miniaturizing devices. However, realizing tight light confinement or efficient coupling with photonic circuits is not straightforward and remains a challenge. Here we show that a high Q nanocavity can be created by placing a single III/V semiconductor nanowire with a diameter of under 100 nm in a grooved waveguide in a Si photonic crystal, by means of nanoprobe manipulation. We observe very fast spontaneous emission (91 ps) from nanowires accelerated by the strong Purcell enhancement in nanocavities, which proves that very strong light confinement can be achieved. Furthermore, this system enables us to move the nanocavity anywhere along the waveguide. This configuration provides a significant degree of flexibility in integrated photonics and permits the addition and displacement of various functionalities of III/V nanocavity devices in Si photonic circuits.
An effective scheme of isostructural alloying was applied to establish a Curie-temperature window in isostructural MnNiGe-CoNiGe system. With the simultaneous accomplishment of decreasing structural-transition temperature and converting antiferromagn etic martensite to ferromagnetic state, a 200 K Curie-temperature window was established between Curie temperatures of austenite and martensite phases. In the window, a first-order magnetostructural transition between paramagnetic austenite and ferromagnetic martensite occurs with a sharp jump in magnetization, showing a magnetic entropy change as large as -40 J kg-1 K-1 in a 50 kOe field change. This giant magnetocaloric effect enables Mn1-xCoxNiGe to become a potential magnetic refrigerant.
Abundant phenomena in CoCr2-xMnxO4 (x = 0 ~ 2) samples such as magnetic compensation, magnetostriction and exchange bias effect have been observed and investigated in this work. A structure transition from cubic to tetragonal symmetry has been found in the samples with x around 1.4. It has shown that the doped Mn3+ ions initially occupy the A (Co) sites when x < 0.2, and then mainly take the B1 (Cr) sites. This behavior results in a role conversion of magnetic contributors, and thus a magnetic compensation between two competitively magnetic sublattices at the composition near x = 0.5. Furthermore, temperature compensation has also been found in the samples with x = 0.5 and 0.6, with the compensation temperature in the range of 45 ~ 75 K. The Mn-doping also changes the frustration degree and modulates the exchange interaction in this system, and thus prevents the formation of long range conical order of spins. Therefore, the magnetoelectric transition temperature at 23 K in CoCr2O4 is shifted to lower temperature with increased dopants. The magnetostriction effect in this Cobalt spinel system has been considered for the first time. The strain has a maximum value of about 240 ppm at x = 0.2 and shows the similar tendency as the compensation behaviors. Additionally, the exchange bias effect observed in the samples with x < 0.5 shows a negative value under low cooling field for x = 0.5.
A new disordered atom configuration in Fe2CrGa alloy has been created by ball-milling method. This leads to a significant enhancement of the magnetic moment up to 3.2~3.9 {mu}B and an increase of Curie temperature by about 200 K, compared with the ar c-melt samples. Combination of first-principles calculations and experimental results reveals that Fe2CrGa alloy should crystallize in Hg2CuTi based structure with different atomic disorders for the samples prepared by different methods. It is addressed that magnetic interactions play a crucial role for the system to adopt such an atomic configuration which disobeys the empirical rule.
The Heusler alloys Fe2NiZ (Z=Al, Ga, Si and Ge) have been synthesized and investigated focusing on the phase stability and the magnetic properties. The experimental and theoretical results reveal the covalent bonding originated from p-d hybridization takes an important role in these alloys, which dominates the stability of ordered structure but leads to the decline of the band splitting. The electronic structure shows the IV group main group element (Si and Ge) provides stronger covalent effect than that of the III group element (Al and Ga). It has been found that the variations of the physical parameters, lattice constants, critical ordering temperature, magnetic moments and Curie temperature, precisely follow these covalent characters.
We have investigated the impact of covalent hybridization on martensitic structure and magnetic properties of Ni50Mn5+xGa35-xCu10 shape memory alloys. We found that the lattice distortion ((c-a)/a) of L10 martensite monotonously changes with the subs titution of Mn for Ga atoms and shows a kink behavior at Ga(at.%)= 25 due to the weakened covalent effect between main-group and transition-metal atoms. Moreover, owing to the competition between covalence hybridization and magnetic ordering of introduced Mn atoms, the molecular magnetic moment and Curie temperature coincidently show maximums at Ga(at.%)=25 as well. These behaviors are closely associated with corresponding changes of the strength of covalent hybridization. The results therefore suggest that careful control of the concentration of main-group atoms in Heusler alloys can serve as an additional general tuning parameter for searching new multifunctional materials.
203 - H. G. Zhang , H. Hu , Y. Pan 2009
Laterally localized electronic states are identified on a single layer of graphene on ruthenium. The individual states are separated by 3 nm and comprise regions of about 90 carbon atoms. This constitutes a quantum dot array, evidenced by quantum wel l resonances that are modulated by the corrugation of the graphene layer. The quantum well resonances are strongest on the isolated hill regions where the graphene is decoupled from the surface. This peculiar nanostructure is expected to become important for single electron physics where it bridges zero-dimensional molecule-like and two-dimensional graphene on a highly regular lattice.
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