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Register a new userSuper-Rayleigh Slopes in Transmission Spectra of Exoplanets Generated by Photochemical Haze
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Spectral slopes in optical transmission spectra of exoplanetary atmospheres encapsulate information on the properties of exotic clouds. The slope is usually attributed to the Rayleigh scattering caused by tiny aerosol particles, whereas recent retrieval studies have suggested that the slopes are often steeper than the canonical Rayleigh slopes. Here, we propose that photochemical haze formed in vigorously mixing atmospheres can explain such super-Rayleigh slopes. We first analytically show that the spectral slope can be steepened by the vertical opacity gradient in which atmospheric opacity increases with altitude. Using a microphysical model, we demonstrate that such opacity gradient can be naturally generated by photochemical haze, especially when the eddy mixing is substantially efficient. The transmission spectra of hazy atmospheres can be demarcated into four typical regimes in terms of the haze mass flux and eddy diffusion coefficient. We find that the transmission spectrum can have the spectral slope 2--4 times steeper than the Rayleigh slope if the eddy diffusion coefficient is sufficiently high and the haze mass flux falls into a moderate value. Based on the eddy diffusion coefficient suggested by a recent study of atmospheric circulations, we suggest that photochemical haze preferentially generates super-Rayleigh slopes at planets with equilibrium temperature of 1000--1500 K, which might be consistent with results of recent retrieval studies. Our results would help to interpret the observations of spectral slopes from the perspective of haze formation.
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UV radiation can induce photochemical processes in exoplanet atmospheres and produce haze particles. Recent observations suggest that haze and/or cloud layers could be present in the upper atmospheres of exoplanets. Haze particles play an important role in planetary atmospheres and may provide a source of organic material to the surface which may impact the origin or evolution of life. However, very little information is known about photochemical processes in cool, high-metallicity exoplanetary atmospheres. Previously, we investigated haze formation and particle size distribution in laboratory atmosphere simulation experiments using AC plasma as the energy source. Here, we use UV photons to initiate the chemistry rather than the AC plasma, since photochemistry driven by UV radiation is important for understanding exoplanet atmospheres. We present photochemical haze formation in current UV experiments, we investigated a range of atmospheric metallicities (100x, 1000x, and 10000x solar metallicity) at three temperatures (300 K, 400 K, and 600 K). We find that photochemical hazes are generated in all simulated atmospheres with temperature-dependent production rates: the particles produced in each metallicity group decrease as the temperature increases. The images taken with atomic force microscopy show the particle size (15-190 nm) varies with temperature and metallicity. Our laboratory experimental results provide new insight into the formation and properties of photochemical haze, which could guide exoplanet atmosphere modeling and help to analyze and interpret current and future observations of exoplanets.
The New Horizons flyby of Pluto confirmed the existence of hazes in its atmosphere. Observations of a large high- to low- phase brightness ratio, combined with the blue color of the haze, suggest that the haze particles are fractal aggregates, analogous to the photochemical hazes on Titan. Therefore, studying the Pluto hazes can shed light on the similarities and differences between the Pluto and Titan atmospheres. We model the haze distribution using the Community Aerosol and Radiation Model for Atmospheres assuming that the distribution is shaped by sedimentation and coagulation of particles originating from photochemistry. Hazes composed of both purely spherical and purely fractal aggregate particles are considered. Agreement between model results and occultation observations is obtained with aggregate particles when the downward flux of photochemical products is equal to the column-integrated methane destruction rate ~1.2 $times$ 10$^{-14}$ g cm$^{-2}$ s$^{-1}$, while for spherical particles the mass flux must be 2-3 times greater. This flux is nearly identical to the haze production flux of Titan previously obtained by comparing microphysical model results to Cassini observations. The aggregate particle radius is sensitive to particle charging, and a particle charge to radius ratio of 30 e-/{mu}m is necessary to produce ~0.1-0.2 {mu}m aggregates near Plutos surface, in accordance with forward scattering measurements. Such a particle charge to radius ratio is 2-4 times higher than those previously obtained for Titan. Hazes composed of spheres with the same particle charge to radius ratio have particles that are 4 times smaller. These results further suggest that the haze particles are fractal aggregates. We also consider the effect of condensation of HCN, and C$_{2}$-hydrocarbons on the haze particles, which may play an important role in shaping their distributions.
The Kepler mission revealed a class of planets known as super-puffs, with masses only a few times larger than Earths but radii larger than Neptune, giving them very low mean densities. All three of the known planets orbiting the young solar-type star Kepler 51 are super-puffs. The Kepler 51 system thereby provides an opportunity for a comparative study of the structures and atmospheres of this mysterious class of planets, which may provide clues about their formation and evolution. We observed two transits each of Kepler 51b and 51d with the Wide Field Camera 3 (WFC3) on the Hubble Space Telescope. Combining new WFC3 transit times with re-analyzed Kepler data and updated stellar parameters, we confirmed that all three planets have densities lower than 0.1 g/cm$^{3}$. We measured the WFC3 transmission spectra to be featureless between 1.15 and 1.63 $mu$m, ruling out any variations greater than 0.6 scale heights (assuming a H/He dominated atmosphere), thus showing no significant water absorption features. We interpreted the flat spectra as the result of a high-altitude aerosol layer (pressure $<$3 mbar) on each planet. Adding this new result to the collection of flat spectra that have been observed for other sub-Neptune planets, we find support for one of the two hypotheses introduced by Crossfield and Kreidberg (2017), that planets with cooler equilibrium temperatures have more high-altitude aerosols. We strongly disfavor their other hypothesis that the H/He mass fraction drives the appearance of large amplitude transmission features.
We present a grid of forward model transmission spectra, adopting an isothermal temperature-pressure profile, alongside corresponding equilibrium chemical abundances for 117 observationally significant hot exoplanets (Equilibrium Temperatures of 547-2710 K). This model grid has been developed using a 1D radiative-convective-chemical equilibrium model termed ATMO, with up-to-date high temperature opacities. We present an interpretation of observations of ten exoplanets, including best fit parameters and $chi^{2}$ maps. In agreement with previous works, we find a continuum from clear to hazy/cloudy atmospheres for this sample of hot Jupiters. The data for all the 10 planets are consistent with sub-solar to solar C/O ratio, 0.005 to 10 times solar metallicity and water rather than a methane dominated infrared spectra. We then explore the range of simulated atmospheric spectra for different exoplanets, based on characteristics such as temperature, metallicity, C/O-ratio, haziness and cloudiness. We find a transition value for the metallicity between 10 and 50 times solar, which leads to substantial changes in the transmission spectra. We also find a transition value of C/O ratio, from water to carbon species dominated infrared spectra, as found by previous works, revealing a temperature dependence of this transition point ranging from $sim$0.56 to $sim$1-1.3 for equilibrium temperatures from $sim$900 to $sim$2600 K. We highlight the potential of the spectral features of HCN and C$_2$H$_2$ to constrain the metallicities and C/O ratios of planets, using JWST observations. Finally, our entire grid ($sim$460,000 simulations) is publicly available and can be used directly with the JWST simulator PandExo for planning observations.
Recently, properties of exoplanet atmospheres have been constrained via multi-wavelength transit observation, which measures an apparent decrease in stellar brightness during planetary transit in front of its host star (called transit depth). Sets of transit depths so far measured at different wavelengths (called transmission spectra) are somewhat diverse: Some show steep spectral slope features in the visible, some contain featureless spectra in the near-infrared, some show distinct features from radiative absorption by gaseous species. These facts infer the existence of haze in the atmospheres especially of warm, relatively low-density super-Earths and mini-Neptunes. Previous studies that addressed theoretical modeling of transmission spectra of hydrogen-dominated atmospheres with haze used some assumed distribution and size of haze particles. In this study, we model the atmospheric chemistry, derive the spatial and size distributions of haze particles by simulating the creation, growth and settling of hydrocarbon haze particles directly, and develop transmission spectrum models of UV-irradiated, solar-abundance atmospheres of close-in warm ($sim$ 500 K) exoplanets. We find that the haze is distributed in the atmosphere much more broadly than previously assumed and consists of particles of various sizes. We also demonstrate that the observed diversity of transmission spectra can be explained by the difference in the production rate of haze monomers, which is related to the UV irradiation intensity from host stars.
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