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Constraints on the Microphysics of Plutos Photochemical Haze from New Horizons Observations

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 Added by Peter Gao
 Publication date 2016
  fields Physics
and research's language is English




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The New Horizons flyby of Pluto confirmed the existence of hazes in its atmosphere. Observations of a large high- to low- phase brightness ratio, combined with the blue color of the haze, suggest that the haze particles are fractal aggregates, analogous to the photochemical hazes on Titan. Therefore, studying the Pluto hazes can shed light on the similarities and differences between the Pluto and Titan atmospheres. We model the haze distribution using the Community Aerosol and Radiation Model for Atmospheres assuming that the distribution is shaped by sedimentation and coagulation of particles originating from photochemistry. Hazes composed of both purely spherical and purely fractal aggregate particles are considered. Agreement between model results and occultation observations is obtained with aggregate particles when the downward flux of photochemical products is equal to the column-integrated methane destruction rate ~1.2 $times$ 10$^{-14}$ g cm$^{-2}$ s$^{-1}$, while for spherical particles the mass flux must be 2-3 times greater. This flux is nearly identical to the haze production flux of Titan previously obtained by comparing microphysical model results to Cassini observations. The aggregate particle radius is sensitive to particle charging, and a particle charge to radius ratio of 30 e-/{mu}m is necessary to produce ~0.1-0.2 {mu}m aggregates near Plutos surface, in accordance with forward scattering measurements. Such a particle charge to radius ratio is 2-4 times higher than those previously obtained for Titan. Hazes composed of spheres with the same particle charge to radius ratio have particles that are 4 times smaller. These results further suggest that the haze particles are fractal aggregates. We also consider the effect of condensation of HCN, and C$_{2}$-hydrocarbons on the haze particles, which may play an important role in shaping their distributions.



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Haze in Plutos atmosphere was detected in images by both the Long Range Reconnaissance Imager (LORRI) and the Multispectral Visible Imaging Camera (MVIC) on New Horizons. LORRI observed haze up to altitudes of at least 200 km above Plutos surface at solar phase angles from ~20{deg} to ~169{deg}. The haze is structured with about ~20 layers, and the extinction due to haze is greater in the northern hemisphere than at equatorial or southern latitudes. However, more haze layers are discerned at equatorial latitudes. A search for temporal variations found no evidence for motions of haze layers (temporal changes in layer altitudes) on time scales of 2 to 5 hours, but did find evidence of changes in haze scale height above 100 km altitude. An ultraviolet extinction attributable to the atmospheric haze was also detected by the ALICE ultraviolet spectrograph on New Horizons. The haze particles are strongly forward-scattering in the visible, and a microphysical model of haze is presented which reproduces the visible phase function just above the surface with 0.5 {mu}m spherical particles, but also invokes fractal aggregate particles to fit the visible phase function at 45 km altitude and account for UV extinction. A model of haze layer generation by orographic excitation of gravity waves is presented. This model accounts for the observed layer thickness and distribution with altitude. Haze particles settle out of the atmosphere and onto Plutos surface, at a rate sufficient to alter surface optical properties on seasonal time scales. Plutos regional scale albedo contrasts may be preserved in the face of the haze deposition by atmospheric collapse.
Plutos atmospheric haze settles out rapidly compared with geological timescales. It needs to be accounted for as a surface material, distinct from Plutos icy bedrock and from the volatile ices that migrate via sublimation and condensation on seasonal timescales. This paper explores how a steady supply of atmospheric haze might affect three distinct provinces on Pluto. We pose the question of why they each look so different from one another if the same haze material is settling out onto all of them. Cthulhu is a more ancient region with comparatively little present-day geological activity, where the haze appears to simply accumulate over time. Sputnik Planitia is a very active region where glacial convection, as well as sublimation and condensation rapidly refresh the surface, hiding recently deposited haze from view. Lowell Regio is a region of intermediate age featuring very distinct coloration from the rest of Pluto. Using a simple model haze particle as a colorant, we are not able to match the colors in both Lowell Regio and Cthulhu. To account for their distinct colors, we propose that after arrival at Plutos surface, haze particles may be less inert than might be supposed from the low surface temperatures. They must either interact with local materials and environments to produce distinct products in different regions, or else the supply of haze must be non-uniform in time and/or location, such that different products are delivered to different places.
Pluto has a heterogeneous surface, despite a global haze deposition rate of ~1 micrometer per orbit (Cheng et al., 2017; Grundy et al., 2018). While there could be spatial variation in the deposition rate, this has not yet been rigorously quantified, and naively the haze should coat the surface more uniformly than was observed. One way (among many) to explain this contradiction is for atmospheric pressure at the surface to drop low enough to interrupt haze production and stop the deposition of particles onto part of the surface, driving heterogeneity. If the surface pressure drops to less than 10^-3 - 10^-4 microbar and the CH4 mixing ratio remains nearly constant at the observed 2015 value, the atmosphere becomes transparent to ultraviolet radiation (Young et al., 2018), which would shut off haze production at its source. If the surface pressure falls below 0.06 microbar, the atmosphere ceases to be global, and instead is localized over only the warmest part of the surface, restricting the location of deposition (Spencer et al., 1997). In Plutos current atmosphere, haze monomers collect together into aggregate particles at beginning at 0.5 microbar; if the surface pressure falls below this limit, the appearance of particles deposited at different times of year and in different locations could be different. We use VT3D, an energy balance model (Young, 2017), to model the surface pressure on Pluto in current and past orbital configurations for four possible static N2 ice distributions: the observed northern hemisphere distribution with (1) a bare southern hemisphere, (2) a south polar cap, (3) a southern zonal band, and finally (4) a distribution that is bare everywhere except inside the boundary of Sputnik Planitia. We also present a sensitivity study showing the effect of mobile N2 ice...(cont.)
82 - B. Sicardy , J. Talbot , E. Meza 2016
We present results from a multi-chord Pluto stellar occultation observed on 29 June 2015 from New Zealand and Australia. This occurred only two weeks before the NASA New Horizons flyby of the Pluto system and serves as a useful comparison between ground-based and space results. We find that Plutos atmosphere is still expanding, with a significant pressure increase of 5$pm$2% since 2013 and a factor of almost three since 1988. This trend rules out, as of today, an atmospheric collapse associated with Plutos recession from the Sun. A central flash, a rare occurrence, was observed from several sites in New Zealand. The flash shape and amplitude are compatible with a spherical and transparent atmospheric layer of roughly 3~km in thickness whose base lies at about 4~km above Plutos surface, and where an average thermal gradient of about 5 K~km$^{-1}$ prevails. We discuss the possibility that small departures between the observed and modeled flash are caused by local topographic features (mountains) along Plutos limb that block the stellar light. Finally, using two possible temperature profiles, and extrapolating our pressure profile from our deepest accessible level down to the surface, we obtain a possible range of 11.9-13.7~$mu$bar for the surface pressure.
UV radiation can induce photochemical processes in exoplanet atmospheres and produce haze particles. Recent observations suggest that haze and/or cloud layers could be present in the upper atmospheres of exoplanets. Haze particles play an important role in planetary atmospheres and may provide a source of organic material to the surface which may impact the origin or evolution of life. However, very little information is known about photochemical processes in cool, high-metallicity exoplanetary atmospheres. Previously, we investigated haze formation and particle size distribution in laboratory atmosphere simulation experiments using AC plasma as the energy source. Here, we use UV photons to initiate the chemistry rather than the AC plasma, since photochemistry driven by UV radiation is important for understanding exoplanet atmospheres. We present photochemical haze formation in current UV experiments, we investigated a range of atmospheric metallicities (100x, 1000x, and 10000x solar metallicity) at three temperatures (300 K, 400 K, and 600 K). We find that photochemical hazes are generated in all simulated atmospheres with temperature-dependent production rates: the particles produced in each metallicity group decrease as the temperature increases. The images taken with atomic force microscopy show the particle size (15-190 nm) varies with temperature and metallicity. Our laboratory experimental results provide new insight into the formation and properties of photochemical haze, which could guide exoplanet atmosphere modeling and help to analyze and interpret current and future observations of exoplanets.
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