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Dielectric optical nanoantennas play an important role in color displays, metasurface holograms, and wavefront shaping applications. They usually exploit Mie resonances as supported on nanostructures with high refractive index, such as Si and TiO2. However, these resonances normally cannot be tuned. Although phase change materials, such as the germanium-antimony-tellurium alloys and post transition metal oxides, such as ITO, have been used to tune optical antennas in the near infrared spectrum, tunable dielectric antennae in the visible spectrum remain to be demonstrated. In this paper, we designed and experimentally demonstrated tunable dielectric nanoantenna arrays with Mie resonances in the visible spectrum, exploiting phase transitions in wide-bandgap Sb2S3 nano-resonators. In the amorphous state, Mie resonances in these Sb2S3 nanostructures give rise to a strong structural color in reflection mode. Thermal annealing induced crystallization and laser induced amorphization of the Sb2S3 resonators allow the color to be tuned reversibly. We believe these tunable Sb2S3 nanoantennae arrays will enable a wide variety of tunable nanophotonic applications, such as high-resolution color displays, holographic displays, and miniature LiDAR systems.
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Metasurfaces are ultrathin nanostructured surfaces that can allow arbitrary manipulation of light. Implementing dynamic tunability into their design could allow the optical functions of metasurfaces to be rapidly modified at will. The most pronounced and robust tunability of optical properties is provided by phase-change materials such as vanadium dioxide (VO2) and germanium antimony telluride (GST), but their implementations have been limited only to near-infrared wavelengths. Here, we demonstrate that VO2 nanoantennas with widely tunable Mie resonances can be utilized for designing tunable metasurfaces in the visible range. In contrast to the dielectric-metallic phase transition-induced tunability in previous demonstrations, we show that dielectric Mie resonances in VO2 nanoantennas offer remarkable scattering and extinction modulation depths (5-8 dB and 1-3 dB, respectively) for tunability in the visible. Moreover, these strong resonances are optically switchable using a continuous-wave laser. Our results establish VO2 nanostructures as low-loss building blocks of optically tunable metasurfaces.
Electro-optic modulators from non-linear $chi^{(2)}$ materials are essential for sensing, metrology and telecommunications because they link the optical domain with the microwave domain. At present, most geometries are suited for fiber applications. In contrast, architectures that modulate directly free-space light at gigahertz (GHz) speeds have remained very challenging, despite their dire need for active free-space optics, in diffractive computing or for optoelectronic feedback to free-space emitters. They are typically bulky or suffer from much reduced interaction lengths. Here, we employ an ultrathin array of sub-wavelength Mie resonators that support quasi bound states in the continuum (BIC) as a key mechanism to demonstrate electro-optic modulation of free-space light with high efficiency at GHz speeds. Our geometry relies on hybrid silicon-organic nanostructures that feature low loss ($Q = $ 550 at $lambda_{res} = 1594$ nm) while being integrated with GHz-compatible coplanar waveguides. We maximize the electro-optic effect by using high-performance electro-optic molecules (whose electro-optic tensor we engineer in-device to exploit $r_{33} = 100$ pm/V) and by nanoscale optimization of the optical modes. We demonstrate both DC tuning and high speed modulation up to 5~GHz ($f_{EO,-3 dB} =3$ GHz) and shift the resonant frequency of the quasi-BIC by $Deltalambda_{res}=$11 nm, surpassing its linewidth. We contrast the properties of quasi-BIC modulators by studying also guided mode resonances that we tune by $Deltalambda_{res}=$20 nm. Our approach showcases the potential for ultrathin GHz-speed free-space electro-optic modulators.
Aligned, densely-packed carbon nanotube metamaterials prepared using vacuum filtration are an emerging infrared nanophotonic material. We report multiple hyperbolic plasmon resonances, together spanning the mid-infrared, in individual resonators made from aligned and densely-packed carbon nanotubes. In the first near-field scanning optical microscopy (NSOM) imaging study of nanotube metamaterial resonators, we observe distinct deeply-subwavelength field profiles at the fundamental and higher-order resonant frequencies. The wafer-scale area of the nanotube metamaterials allows us to combine this near-field imaging with a systematic far-field spectroscopic study of the scaling properties of many resonator arrays. Thorough theoretical modeling agrees with these measurements and identifies the resonances as higher-order Fabry-Perot (FP) resonances of hyperbolic waveguide modes. Nanotube resonator arrays show broadband extinction from 1.5-10 {mu}m and reversibly switchable extinction in the 3-5 {mu}m atmospheric transparency window through the coexistence of multiple modes in individual ribbons. Broadband carbon nanotube metamaterials supporting multiple resonant modes are a promising candidate for ultracompact absorbers, tunable thermal emitters, and broadband sensors in the mid-infrared.
Janus monolayers have long been captivated as a popular notion for breaking in-plane and out-of-plane structural symmetry. Originated from chemistry and materials science, the concept of Janus functions have been recently extended to ultrathin metasurfaces by arranging meta-atoms asymmetrically with respect to the propagation or polarization direction of the incident light. However, such metasurfaces are intrinsically static and the information they carry can be straightforwardly decrypted by scanning the incident light directions and polarization states once the devices are fabricated. In this Letter, we present a dynamic Janus metasurface scheme in the visible spectral region. In each super unit cell, three plasmonic pixels are categorized into two sets. One set contains a magnesium nanorod and a gold nanorod that are orthogonally oriented with respect to each other, working as counter pixels. The other set only contains a magnesium nanorod. The effective pixels on the Janus metasurface can be reversibly regulated by hydrogenation/dehydrogenation of the magnesium nanorods. Such dynamic controllability at visible frequencies allows for flat optical elements with novel functionalities including beam steering, bifocal lensing, holographic encryption, and dual optical function switching.
Based on the substantial difference in the response time for the resonant and background partitions at stepwise variations of the exiting signal, a simple exactly integrable model describing the dynamic Fano resonance (DFRs) is proposed. The model does not have any fitting parameters, may include any number of resonant partitions and exhibits high accuracy. It is shown that at the point of the destructive interference any sharp variation of the amplitude of the excitation (no matter an increase or a decrease) gives rise to pronounced flashes in the intensity of the output signal. In particular, the flash should appear behind the trailing edge of the exciting pulse, when the excitation is already over. The model is applied to explain the DFRs at the light scattering by a dielectric cylinder with two resonant modes excited simultaneously and exhibits the excellent agreement with the results of the direct numerical integration of the Maxwell equations.
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