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Register a new userLight-Driven Raman Coherence as a Non-Thermal Route to Ultrafast Topology Switching
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A grand challenge underlies the entire field of topology-enabled quantum logic and information science: how to establish topological control principles driven by quantum coherence and understand the time-dependence of such periodic driving? Here we demonstrate a THz pulse-induced phase transition in Dirac materials that is periodically driven by vibrational coherence due to excitation of the lowest Raman-active mode. Above a critical field threshold, there emerges a long-lived metastable phase with unique Raman coherent phonon-assisted switching dynamics, absent for optical pumping. The switching also manifest itself by non-thermal spectral shape, relaxation slowing down near the Lifshitz transition where the critical Dirac point (DP) occurs, and diminishing signals at the same temperature that the Berry curvature induced Anomalous Hall Effect varnishes. These results, together with first-principles modeling, identify a mode-selective Raman coupling that drives the system from strong to weak topological insulators, STI to WTI, with a Dirac semimetal phase established at a critical atomic displacement controlled by the phonon pumping. Harnessing of vibrational coherence can be extended to steer symmetry-breaking transitions, i.e., Dirac to Weyl ones, with implications on THz topological quantum gate and error correction applications.
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Exciting atomic oscillations with light is a powerful technique to control the electronic properties of materials, leading to remarkable phenomena such as light-induced superconductivity and ultrafast insulator to metal transitions. Here we show that light-driven lattice vibrations can be utilised to encode efficiently spin information in a magnetic medium. Intense mid-infrared electric field pulses, tuned to resonance with a vibrational normal mode of antiferromagnetic DyFeO3, drive the emergence of long-living weak ferromagnetic order. Light-driven phonon displacements promptly lower the energy barrier separating competing magnetic states, allowing the alignment of spins to occur within a few picoseconds, via non-equilibrium dynamics of the magnetic energy landscape.
We discuss the procedure for gauging on-site $mathbb{Z}_2$ global symmetries of three-dimensional lattice Hamiltonians that permute quasi-particles and provide general arguments demonstrating the non-Abelian character of the resultant gauged theories. We then apply this general procedure to lattice models of several well known fracton phases: two copies of the X-Cube model, two copies of Haahs cubic code, and the checkerboard model. Where the former two models possess an on-site $mathbb{Z}_2$ layer exchange symmetry, that of the latter is generated by the Hadamard gate. For each of these models, upon gauging, we find non-Abelian subdimensional excitations, including non-Abelian fractons, as well as non-Abelian looplike excitations and Abelian fully mobile pointlike excitations. By showing that the looplike excitations braid non-trivially with the subdimensional excitations, we thus discover a novel gapped quantum order in 3D, which we term a panoptic fracton order. This points to the existence of parent states in 3D from which both topological quantum field theories and fracton states may descend via quasi-particle condensation. The gauged cubic code model represents the first example of a gapped 3D phase supporting (inextricably) non-Abelian fractons that are created at the corners of fractal operators.
I propose a method for ultrafast switching of ferroelectric polarization using mid-infrared pulses. This involves selectively exciting the highest frequency $A_1$ phonon mode of a ferroelectric material with an intense mid-infrared pulse. Large amplitude oscillations of this mode provides a unidirectional force to the lattice such that it displaces along the lowest frequency $A_1$ phonon mode coordinate because of a nonlinear coupling of the type $g Q_{textrm{P}} Q_{textrm{IR}}^2$ between the two modes. First principles calculations show that this coupling is large in transition-metal oxide ferroelectrics, and the sign of the coupling is such that the lattice displaces in the switching direction. Furthermore, I find that the lowest frequency $A_1$ mode has a large $Q_{textrm{P}}^3$ order anharmonicity, which causes a discontinuous switch of electric polarization as the pump amplitude is continuously increased.
We use femtosecond electron diffraction to study ultrafast lattice dynamics in the highly correlated antiferromagnetic (AF) semiconductor NiO. Using the scattering vector (Q) dependence of Bragg diffraction, we introduce a Q-resolved effective lattice temperature, and identify a nonthermal lattice state with preferential displacement of O compared to Ni ions, which occurs within ~0.3 ps and persists for 25 ps. We associate this with transient changes to the AF exchange striction-induced lattice distortion, supported by the observation of a transient Q-asymmetry of Friedel pairs. Our observation highlights the role of spin-lattice coupling in routes towards ultrafast control of spin order.
Charge kinks are considered as fundamental excitations in quarter-filled charge-ordered ladders. The strength of the coupling of the kinks to the three-dimensional lattice depends on their energy. The integrated intensity of Raman scattering by kink-antikink pairs is proportional to $phi ^{5}$ or $phi ^{4},$ where $phi $ is the order parameter. The exponent is determined by the system parameters and by the strength of the electron-phonon coupling.
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