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Experimental demonstration of an electrostatic orbital angular momentum sorter for electrons

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 Added by Vincenzo Grillo
 Publication date 2019
  fields Physics
and research's language is English




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We report the first experimental demonstration of an electrostatic electron orbital angular momentum (OAM) sorter, which can be used to analyze the OAM states of electrons in a transmission electron microscope. We verify the sorter functionality for several electron beams possessing different superpositions of OAM states, and use it to record the electron beams OAM spectra. Our current electrostatic OAM sorter has an OAM resolution of 2 in the units of h/bar - the reduced Planck constant. It is expected to increase the OAM resolution of the sorter to the optimal resolution of 1 in the future via fine control of the sorting phase elements.



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The orbital angular momentum (OAM) sorter is a new electron optical device for measuring an electron s OAM. It is based on two phase elements, which are referred to as the unwrapper and corrector and are placed in Fourier conjugate planes in an electron microscope. The most convenient implementation of this concept is based on the use of electrostatic phase elements, such as a charged needle as the unwrapper and a set of electrodes with alternating charges as the corrector. Here, we use simulations to assess the role of imperfections in such a device, in comparison to an ideal sorter. We show that the finite length of the needle and the boundary conditions introduce astigmatism, which leads to detrimental cross-talk in the OAM spectrum. We demonstrate that an improved setup comprising three charged needles can be used to compensate for this aberration, allowing measurements with a level of cross-talk in the OAM spectrum that is comparable to the ideal case.
We consider the problem of discriminating macromolecular structures in an electron microscope, through a specific beam shaping technique. Our approach is based on maximizing the which-molecule information extracted from the state of each electron. To this aim, the optimal observables are derived within the framework of quantum state discrimination, which allows one to fully account from the quantum character of the probe. We simulate the implementation of such optimal observable on a generalized orbital angular momentum (OAM) sorter and benchmark its performance against the best known real space approach.
We reveal for the first time a direct relationship between the diffraction of optical beams and their carrying orbital angular momentum (OAM). We experimentally demonstrate a novel phenomenon that the anisotropic diffraction can be induced by the OAM, predicted by us [Opt. Express, textbf{26}, 8084 (2018)], via the propagations of the elliptic beams with the OAM in linearly and both-linearly-and-nonlinearly isotropic media, respectively. In the former case, when its carrying OAM equals the so-called critical OAM, the spiraling elliptic Gaussian beam (fundamental eigenmode) is observed in the free space, where only the eigenmode with cylindrical-symmetry is supposed to exist for the beam without the OAM. In the latter case, the spiraling elliptic soliton, predicted by Desyatnikov et al. [Phys. Rev. Lett, textbf{104}, 053902 (2010)], is observed to stably propagate in a cylindrical lead glass. The power-controllable rotation of such an elliptic beam is also experimentally demonstrated.
Recently, a new device to measure the Orbital Angular Momentum (OAM) electronic spectrum after elastic/inelastic scattering in a transmission electron microscope has been introduced. We modified the theoretical framework needed to describe conventional low loss electron energy loss spectroscopy (EELS) experiments in transmission electron microscopes (TEM) to study surface plasmons in metallic nanostructures, to allow for an OAM post selection and devise new experiments for the analysis of these excitations in nanostructures. We found that unprecedented information on the symmetries and on the chirality of the plasmonic modes can be retrieved even with limited OAM and energy resolutions.
Free electrons with a helical phase front, referred to as twisted electrons, possess an orbital angular momentum (OAM) and, hence, a quantized magnetic dipole moment along their propagation direction. This intrinsic magnetic moment can be used to probe material properties. Twisted electrons thus have numerous potential applications in materials science. Measuring this quantity often relies on a series of projective measurements that subsequently change the OAM carried by the electrons. In this Letter, we propose a nondestructive way of measuring an electron beams OAM through the interaction of this associated magnetic dipole with a conductive loop. Such an interaction results in the generation of induced currents within the loop, which are found to be directly proportional to the electrons OAM value. Moreover, the electron experiences no OAM variations and only minimal energy losses upon the measurement, and, hence, the nondestructive nature of the proposed technique.
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