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Register a new userEfficient molecule discrimination in electron microcopy through an optimized orbital angular momentum sorter
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We consider the problem of discriminating macromolecular structures in an electron microscope, through a specific beam shaping technique. Our approach is based on maximizing the which-molecule information extracted from the state of each electron. To this aim, the optimal observables are derived within the framework of quantum state discrimination, which allows one to fully account from the quantum character of the probe. We simulate the implementation of such optimal observable on a generalized orbital angular momentum (OAM) sorter and benchmark its performance against the best known real space approach.
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Quantum complementarity states that particles, e.g. electrons, can exhibit wave-like properties such as diffraction and interference upon propagation. textit{Electron waves} defined by a helical wavefront are referred to as twisted electrons~cite{uchida:10,verbeeck:10,mcmorran:11}. These electrons are also characterised by a quantized and unbounded magnetic dipole moment parallel to their propagation direction, as they possess a net charge of $-|e|$~cite{bliokh:07}. When interacting with magnetic materials, the wavefunctions of twisted electrons are inherently modified~cite{lloyd:12b,schattschneider:14a,asenjo:14}. Such variations therefore motivate the need to analyze electron wavefunctions, especially their wavefronts, in order to obtain information regarding the materials structure~cite{harris:15}. Here, we propose, design, and demonstrate the performance of a device for measuring an electrons azimuthal wavefunction, i.e. its orbital angular momentum (OAM) content. Our device consists of nanoscale holograms designed to introduce astigmatism onto the electron wavefunctions and spatially separate its phase components. We sort pure and superposition OAM states of electrons ranging within OAM values of $-10$ and $10$. We employ the device to analyze the OAM spectrum of electrons having been affected by a micron-scale magnetic dipole, thus establishing that, with a midfield optical configuration, our sorter can be an instrument for nano-scale magnetic spectroscopy.
We report the first experimental demonstration of an electrostatic electron orbital angular momentum (OAM) sorter, which can be used to analyze the OAM states of electrons in a transmission electron microscope. We verify the sorter functionality for several electron beams possessing different superpositions of OAM states, and use it to record the electron beams OAM spectra. Our current electrostatic OAM sorter has an OAM resolution of 2 in the units of h/bar - the reduced Planck constant. It is expected to increase the OAM resolution of the sorter to the optimal resolution of 1 in the future via fine control of the sorting phase elements.
Free electrons with a helical phase front, referred to as twisted electrons, possess an orbital angular momentum (OAM) and, hence, a quantized magnetic dipole moment along their propagation direction. This intrinsic magnetic moment can be used to probe material properties. Twisted electrons thus have numerous potential applications in materials science. Measuring this quantity often relies on a series of projective measurements that subsequently change the OAM carried by the electrons. In this Letter, we propose a nondestructive way of measuring an electron beams OAM through the interaction of this associated magnetic dipole with a conductive loop. Such an interaction results in the generation of induced currents within the loop, which are found to be directly proportional to the electrons OAM value. Moreover, the electron experiences no OAM variations and only minimal energy losses upon the measurement, and, hence, the nondestructive nature of the proposed technique.
Orbital angular momentum (OAM) of light is an attractive degree of freedom for funda- mentals studies in quantum mechanics. In addition, the discrete unbounded state-space of OAM has been used to enhance classical and quantum communications. Unambiguous mea- surement of OAM is a key part of all such experiments. However, state-of-the-art methods for separating single photons carrying a large number of different OAM values are limited to a theoretical separation efficiency of about 77 percent. Here we demonstrate a method which uses a series of unitary optical transformations to enable the measurement of lights OAM with an experimental separation efficiency of more than 92 percent. Further, we demonstrate the separation of modes in the angular position basis, which is mutually unbiased with respect to the OAM basis. The high degree of certainty achieved by our method makes it particu- larly attractive for enhancing the information capacity of multi-level quantum cryptography systems.
The spatial modes of light, carrying a quantized amount of orbital angular momentum (OAM), is one of the excellent candidates that provides access to high-dimensional quantum states, which essentially makes it promising towards building high-dimensional quantum networks. In this paper, we report the storage and retrieval of photonic qubits encoded with OAM state in the cold atomic ensemble, achieving an average conditional fidelity above 98% and retrieval efficiency around 65%. The photonic OAM qubits are encoded with weak coherent states at the single-photon level and the memory is based on electromagnetically induced transparency in an elongated cold rubidium atomic ensemble. Our work constitutes an efficient node that is needed towards high dimensional and large scale quantum networks.
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