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تسجيل مستخدم جديدRobust approximation of tensor networks: application to grid-free tensor factorization of the Coulomb interaction
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Approximation of a tensor network by approximating (e.g., factorizing) one or more of its constituent tensors can be improved by canceling the leading-order error due to the constituents approximation. The utility of such robust approximation is demonstrated for robust canonical polyadic (CP) approximation of a (density-fitting) factorized 2-particle Coulomb interaction tensor. The resulting algebraic (grid-free) approximation for the Coulomb tensor, closely related to the factorization appearing in pseudospectral and tensor hypercontraction approaches, is efficient and accurate, with significantly reduced rank compared to the naive (non-robust) approximation. Application of the robust approximation to the particle-particle ladder term in the coupled-cluster singles and doubles reduces the size complexity from $mathcal{O}(N^6)$ to $mathcal{O}(N^5)$ with robustness ensuring negligible errors in chemically-relevant energy differences using CP ranks approximately equal to the size of the density-fitting basis.
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