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تسجيل مستخدم جديدTorque magnetometry studies of metamagnetic transitions in single-crystal HoNi_{2}B_{2}C and ErNi_{2}B_{2}C at Tapprox 1.9 K
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The metamagnetic transitions in single-crystal rare-earth nickel borocarbide HoNi_{2}B_{2}C and ErNi_{2}B_{2}C have been studied at 1.9 K with a Quantum Design torque magnetometer. The critical fields of the transitions depend crucially on the angle between applied field and the easy axis [110] for HoNi_2B_2C and [100] for ErNi_2B_2C. Torque measurements have been made while changing angular direction of the magnetic field (parallel to basal tetragonal ab-planes) in a wide angular range (more than two quadrants). The results are used not only to check and refine the angular diagram for metamagnetic transitions in these compounnds, but also to find new features of the metamagnetic states. Among new results for the Ho borocarbide are the influence of a multidomain antiferromagnetic state, and ``frustrated behavior of the magnetic system for field directions close to the hard axis [100]. Torque measurements of the Er borocarbide clearly show that the sequence of metamagnetic transitions with increasing field (and the corresponding number of metamagnetic states) depends on the angular direction of the magnetic field relative to the easy axis.
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The metamagnetic transitions in single-crystal ErNi$_2$B$_2$C have been studied at 1.9 K with a Quantum Design torque magnetometer. The critical fields of the transitions depend crucially on the angle between applied field and the easy axis [100]. To
rque measurements have been made while changing angular direction of the magnetic field (parallel to basal tetragonal $ab$-planes) in a wide angular range (more than two quadrants). Sequences of metamagnetic transitions with increasing field are found to be different for the magnetic field along (or close enough to) the easy [100] axis from that near the hard [110] axis. The study have revealed new metamagnetic states in ErNi$_{2}$B$_2$C which were not apparent in previous longitudinal-magnetization and neutron studies.
Metamagnetic transitions in single-crystal rare-earth nickel borocarbide HoNi$_2$B$_2$C have been studied at Tapprox 1.9 K with a Quantum Design torque magnetometer. This compound is highly anisotropic with a variety of metamagnetic states at low tem
perature which includes antiferromagnetic, ferrimagnetic, non-collinear and ferromagnetic-like (saturated paramagnet) states. The critical fields of the transitions depend crucially on the angle $theta$ between applied field and the easy axis [110]. Measurements of torque along the c-axis have been made while changing the angular direction of the magnetic field (parallel to basal tetragonal $ab$-planes) and with changing field at fixed angle over a wide angular range. Two new phase boundaries in the region of the non-collinear phase have been observed, and the direction of the magnetization in this phase has been precisely determined. At low field the antiferromagnetic phase is observed to be multidomain. In the angular range very close to the hard axis [100] ($-6^{circ} lesssimphi lesssim 6^{circ}$, where $phi$ is the angle between field and the hard axis) the magnetic behavior is found to be ``frustrated with a mixture of phases with different directions of the magnetization.
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features expected for the corresponding magnetic modes, namely k_{1}=(0.55,0,0) at x=0; k_{2}=([nicefrac] icefrac{1}{2}</LaTeX>,0,[nicefrac]<LaTeX> icefrac{1}{2}) at x= 0.2; k_{3}=(0,0,[nicefrac] icefrac{1}{3}) at x= 0.6, and k_{4}=(0,0,0) at x= 0.8 and 1. For x=0.4, even though the neutron diffraction indicates a k_{2} mode, but with a reduced magnetic moment, the magnetization, the ac susceptibility, and resistivity indicate two magnetic events; furthermore, deviation from Curie-Weiss behavior is observed below 150 K for this sample. These features, together with the evolution of both magnetic moment and critical temperature, are attributed to an interplay between competing magnetic couplings; for the particular x=0.4 case, additional factors such as crystalline electric field effects may be in operation.
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