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Angular momentum plays a central role in a multitude of phenomena in quantum mechanics, recurring in every length scale from the microscopic interactions of light and matter to the macroscopic behavior of superfluids. Vortex beams, carrying intrinsic orbital angular momentum (OAM), are now regularly generated with elementary particles such as photons and electrons, and harnessed for numerous applications including microscopy and communication. Untapped possibilities remain hidden in vortices of non-elementary particles, as their composite structure can lead to coupling of OAM with internal degrees of freedom. However, thus far, the creation of a vortex beam of a non-elementary particle has never been demonstrated experimentally. We present the first vortex beams of atoms and molecules, formed by diffracting supersonic beams of helium atoms and dimers, respectively, off binary masks made from transmission gratings. By achieving large particle coherence lengths and nanometric grating features, we observe a series of vortex rings corresponding to different OAM states in the accumulated images of particles impacting a detector. This method is general and can be applied to most atomic and molecular gases. Our results may open new frontiers in atomic physics, utilizing the additional degree of freedom of OAM to probe collisions and alter fundamental interactions.
In this work we show how constructing Wigner functions of heterogeneous quantum systems leads to new capability in the visualization of quantum states of atoms and molecules. This method allows us to display quantum correlations (entanglement) betwee
We experimentally investigate the optical storage of perfect optical vortex (POV) and spatially multimode perfect optical vortex (MPOV) beams via electromagnetically induced transparency (EIT) in a hot vapor cell. In particular, we study the role tha
We investigate theoretically the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom taking into account its fine-structure. The interaction involves the combination of first-or
Exchange of orbital angular momentum between Laguerre-Gaussian beam of light and center-of-mass motion of an atom or molecule is well known. We show that orbital angular momentum of light can also be transferred to the internal electronic or rotation
Improving axial resolution is of paramount importance for three-dimensional optical imaging systems. Here, we investigate the ultimate precision in axial localization using vortex beams. For Laguerre-Gauss beams, this limit can be achieved with just