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Nanophotonic waveguides with sub-wavelength mode confinement and engineered dispersion profiles are an excellent platform for application-tailored nonlinear optical interactions at low pulse energies. Here, we present fully air clad suspended-silicon waveguides for infrared frequency comb generation with optical bandwidth limited only by the silicon transparency. The achieved spectra are lithographically tailored to span 2.1 octaves in the mid-infrared (2.0-8.5 um or 1170--5000 cm-1) when pumped at 3.10 um with 100 pJ pulses. Novel fork-shaped couplers provide efficient input coupling with only 1.5 dB loss. The coherence, brightness, and the stability of the generated light are highlighted in a dual frequency comb setup in which individual comb-lines are resolved with 30 dB extinction ratio and 100 MHz spacing in the wavelength range of 4.8-8.5 um (2100-1170 cm-1). These sources are used for broadband gas- and liquid-phase dual-comb spectroscopy with 100 MHz comb-line resolution. We achieve a peak spectral signal-to-noise ratio of 10 Hz^0.5 across a simultaneous bandwidth containing 112,200 comb-lines. These results provide a pathway to further integration with the developing high repetition rate frequency comb lasers for compact sensors with applications in chip-based chemical analysis and spectroscopy.
Low propagation loss in high confinement waveguides is critical for chip-based nonlinear photonics applications. Sophisticated fabrication processes which yield sub-nm roughness are generally needed to reduce scattering points at the waveguide interf
High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped periodically poled li
Carrier recombination dynamics in strip silicon nano-waveguides is analyzed through time-resolved pump-and-probe experiments, revealing a complex recombination dynamics at densities ranging from ${10^{14}}$ to ${10^{17}},$cm$^{{-3}}$. Our results sho
Ultraviolet frequency combs enable applications ranging from precision spectroscopy to atomic clocks by addressing the electronic transitions of atoms and molecules. Access to ultraviolet light via integrated nonlinear optics is usually hampered by t
We investigate theoretically frequency comb generation in a bottle microresonator accounting for the azimuthal and axial degrees of freedom. We first identify a discrete set of the axial nonlinear modes of a bottle microresonator that appear as tilte