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تسجيل مستخدم جديدNature of Partial Magnetic Order in the Frustrated Antiferromagnet Gd2Ti2O7
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The frustrated pyrochlore antiferromagnet Gd$_{2}$Ti$_{2}$O$_{7}$ has an unusual partially-ordered magnetic structure at the lowest measurable temperatures. This structure is currently believed to involve four magnetic propagation vectors $mathbf{k}in langle frac{1}{2} frac{1}{2} frac{1}{2} rangle^*$ in a cubic 4-$mathbf{k}$ structure, based on analysis of magnetic diffuse-scattering data [J. Phys.: Condens. Matter 16, L321 (2004)]. Here, we present three pieces of evidence against the 4-$mathbf{k}$ structure. First, we report single-crystal neutron-diffraction measurements as a function of applied magnetic field, which are consistent with the selective field-induced population of non-cubic magnetic domains. Second, we present evidence from high-resolution powder neutron-diffraction measurements that rhombohedral strains exist within magnetic domains, which may be generated by magneto-elastic coupling only for the alternative 1-$mathbf{k}$ structure. Finally, we show that the argument previously used to rule out the 1-$mathbf{k}$ structure is flawed, and demonstrate that magnetic diffuse-scattering data can actually be fitted quantitatively by a 1-$mathbf{k}$ structure in which spin fluctuations on ordered and disordered magnetic sites are strongly coupled. Our results provide an experimental foundation on which to base theoretical descriptions of partially-ordered states.
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