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We investigate the evolution of binary fractions in star clusters using N-body models of up to 100000 stars. Primordial binary frequencies in these models range from 5% to 50%. Simulations are performed with the NBODY4 code and include a full mass spectrum of stars, stellar evolution, binary evolution and the tidal field of the Galaxy. We find that the overall binary fraction of a cluster almost always remains close to the primordial value, except at late times when a cluster is near dissolution. A critical exception occurs in the central regions where we observe a marked increase in binary fraction with time -- a simulation starting with 100000 stars and 5% binaries reached a core binary frequency as high as 40% at the end of the core-collapse phase (occurring at 16 Gyr with ~20000 stars remaining). Binaries are destroyed in the core by a variety of processes as a cluster evolves, but the combination of mass-segregation and creation of new binaries in exchange interactions produces the observed increase in relative number. We also find that binaries are cycled into and out of cluster cores in a manner that is analogous to convection in stars. For models of 100000 stars we show that the evolution of the core-radius up to the end of the initial phase of core-collapse is not affected by the exact value of the primordial binary frequency (for frequencies of 10% or less). We discuss the ramifications of our results for the likely primordial binary content of globular clusters.
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