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In this work, we study crystalline electric field effects in the heavy fermion superconductor CeIrIn5. We observe two regions of broad magnetic response in the inelastic neutron scattering spectra at 10 K. The first corresponds to the transition between the gamma7 groundstate doublet and the first excited state doublet at 4 meV interwoven with a broad quasielastic contribution. The second region corresponds to the transition between the ground state and the second excited state doublet at 28 meV. The large Lorentzian half-widths of the peaks (~10 meV) calls into question calculations for the specific heat and magnetic susceptibility that assume sharp crystal field levels. Consequently, we have calculated the inelastic neutron scattering spectra and magnetic susceptibility using the Anderson impurity model within the non-crossing approximation (NCA) including the effects of crystal field level splitting.
We present results for the electronic structure of plutonium by using a recently developed quasiparticle self-consistent $GW$ method (qsgw). We consider a paramagnetic solution without spin-orbit interaction as a function of volume for the face-cente
SrTm$_2$O$_4$ has been investigated using heat capacity, magnetic susceptibility, magnetization in pulsed fields, and inelastic neutron scattering measurements. These results show that the system is highly anisotropic, has gapped low-energy dispersin
We derive an exact operatorial reformulation of the rotational invariant slave boson method and we apply it to describe the orbital differentiation in strongly correlated electron systems starting from first principles. The approach enables us to tre
In terms of a semi-phenomenological exchange charge model, we have obtained estimates of parameters of the crystal field and parameters of the electron-deformation interaction in terbium titanate Tb2Ti2O7 with a pyrochlore structure. The obtained set
We report a study on the temperature dependence of the charge-neutral crystal field (dd) excitations in cupric oxide, using nonresonant inelastic x-ray scattering (IXS) spectroscopy. Thanks to a very high energy resolution (60 meV), we observe therma