ترغب بنشر مسار تعليمي؟ اضغط هنا

Argon annealing of the oxygen-isotope exchanged manganite La_{0.8}Ca_{0.2}MnO_{3+y}

75   0   0.0 ( 0 )
 نشر من قبل Guo-Meng Zhao
 تاريخ النشر 2000
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

We have resolved a controversial issue concerning the oxygen-isotope shift of the ferromagnetic transition temperature T_{C} in the manganite La_{0.8}Ca_{0.2}MnO_{3+y}. We show that the giant oxygen-isotope shift of T_C observed in the normal oxygen-isotope exchanged samples is indeed intrinsic, while a much smaller shift observed in the argon annealed samples is an artifact. The argon annealing causes the 18O sample to partially exchange back to the 16O isotope due to a small 16O contamination in the Ar gas. Such a contamination is commonly caused by the oxygen outgas that is trapped in the tubes, connectors and valves. The present results thus umambiguously demonstrate that the observed large oxygen isotope effect is an intrinsic property of manganites, and places an important constraint on the basic physics of these materials.

قيم البحث

اقرأ أيضاً

We have studied acoustoelectric (AE) effect produced by surface acoustic waves (SAW) in a monolithic layered structure, composed of piezodielectric LiNbO_{3} substrate and La_{0.67}Ca_{0.33}MnO_{3} film. The experiments unexpectedly revealed in the l ongitudinal AE effect an anomalous contribution, invariant upon reversal of SAW propagation, which coexists with the ordinary (odd in wave vector) effect. The anomalous effect dominates near the metal-insulator transition, while the ordinary effect prevails at high and low temperatures. We show that the anomalous effect is caused by strong modulation of the film conductivity produced by the SAW elastic deformations.
78 - K. H. Kim , M. Uehara , C. Hess 2000
We measured thermal conductivity, k, thermoelectric power, S, and dc electric conductivity, sigma, of La_{5/8-x}Pr_{x}Ca_{3/8}MnO_{3}, showing an intricate interplay between metallic ferromagnetism (FM) and charge ordering (CO) instability. The chang e of k, S and sigma with temperature (T) and x agrees well with the effective medium theories for binary metal-insulator mixtures. This agreement clearly demonstrates that with the variation of T as well as x, the relative volumes of FM and CO phases drastically change and percolative metal-insulator transition occurs in the mixture of FM and CO domains.
The specific heat C of Ce_{0.8}La_{0.2}Al_{3} has been measured as a function of temperature T in magnetic fields up to 14 T. A large peak in C at 2.3 K has recently been ascribed to an anisotropic Kondo effect in this compound. A 14-T field depresse s the temperature of the peak by only 0.2 K, but strongly reduces its height. The corresponding peak in C/T shifts from 2.1 K at zero field to 1.7 K at 14 T. The extrapolated specific heat coefficient C/T(T->0) increases with field over the range studied. We show that these trends are inconsistent with the anisotropic Kondo model.
We report a detailed study of the electric transport and magnetic properties of the LaNdCaMnO manganite system. Substitution of LaIII by smaller NdIII ions, reduces the mean ionic radius of the A site ion. We have studied samples in the entire range between rich La and rich Nd compounds. Results of DC magnetization and resistivity show that doping destabilize the FM character of the pure La compound and triggers the formation of a phase separated state at intermediate doping. We have also found evidence of a dynamical behaviour within the phase separated state. A phase diagram is constructed, summarizing the effect of chemical substitution on the system.
Materials that exhibit colossal magnetoresistance (CMR) are currently the focus of an intense research effort, driven by the technological applications that their sensitivity lends them to. Using the angular correlation of photons from electron-posit ron annihilation, we present a first glimpse of the Fermi surface of a material that exhibits CMR, supported by ``virtual crystal electronic structure calculations. The Fermi surface is shown to be sufficiently cubic in nature that it is likely to support nesting.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا