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Spin defects in silicon carbide (SiC) have attracted increasing interests due to their excellent optical and spin properties, which are useful in quantum information processing. In this work, we systematically investigate the temperature dependence of spin properties of divacancy defects in implanted 4H-SiC. The zero-field splitting parameter D, the inhomogeneous dephasing time $T_2^{*}$, the coherence time $T_2$, and the depolarization time $T_1$ are extensively explored in a temperature range from 5 K to 300 K. Two samples implanted with different nitrogen molecule ion fluences ($N_2^{+}$, $10^{14}/rm cm^{2}$ and $10^{13}/rm cm^{2}$) are investigated, whose spin properties are shown to have similar temperature-dependent behaviors. Still, the sample implanted with a lower ion fluence has longer $T_2$ and $T_1$. We provide possible theoretical explanations for the observed temperature-dependent dynamics. Our work promotes the understanding of the temperature dependence of spin properties in solid-state systems, which can be helpful for constructing wide temperature-range thermometers based on the mature semiconductor material.
Recently, vacancy-related spin defects in silicon carbide (SiC) have been demonstrated to be potentially suitable for versatile quantum interface building and scalable quantum network construction. Significant efforts have been undertaken to identify
Long coherence times are key to the performance of quantum bits (qubits). Here, we experimentally and theoretically show that the Hahn-echo coherence time (T2) of electron spins associated with divacancy defects in 4H-SiC reaches 1.3 ms, one of the l
Optically addressable spin defects in silicon carbide (SiC) are an emerging platform for quantum information processing. Lending themselves to modern semiconductor nanofabrication, they promise scalable high-efficiency spin-photon interfaces. We demo
Silicon-vacancy qubits in silicon carbide (SiC) are emerging tools in quantum technology applications due to their excellent optical and spin properties. In this paper, we explore the effect of temperature and strain on these properties by focusing o
Irradiation-induced lattice defects in silicon carbide (SiC) have already exceeded their previous reputation as purely performance-inhibiting. With their remarkable quantum properties, such as long room-temperature spin coherence and the possibility