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Bulk materials possessing a relative electric permittivity $varepsilon$ close to zero exhibit giant Kerr nonlinearities. However, harnessing this response in guided-wave geometries is not straightforward, due to the extreme and counter-intuitive properties of epsilon-near-zero materials. Here we investigate, through rigorous calculations of the Kerr nonlinear coefficient, how the remarkable nonlinear properties of such materials can be exploited in several different types of structures, including bulk films, plasmonic nanowires, and metal nanoapertures. We find the largest Kerr nonlinear response when both the modal area and the group velocity are simultaneously minimized, corresponding to omnidirectional field enhancement. The physical insights developed will be key for understanding and engineering nonlinear nanophotonic systems with extreme nonlinearities and point to new design paradigms.
We observe unique absorption resonances in silver/silica multilayer-based epsilon-near-zero (ENZ) metamaterials that are related to radiative bulk plasmon-polariton states of thin-films originally studied by Ferrell (1958) and Berreman (1963). In the
We investigate non-diffracting hollow-core nonlinear optical waves propagating in a layered nanoscaled metal-dielectric structure characterized by a very small average linear dielectric permittivity (Nonlinear Epsilon-Near-Zero metamaterial). We anal
Near-infrared epsilon-near-zero (ENZ) metamaterial slabs based on silver-germanium (Ag-Ge) multilayers are experimentally demonstrated. Transmission, reflection and absorption spectra are characterized and used to determine the complex refractive ind
Vibrational ultrastrong coupling (USC), where the light-matter coupling strength is comparable to the vibrational frequency of molecules, presents new opportunities to probe the interactions of molecules with zero-point fluctuations, harness cavity-e
An optical topological transition is defined as the change in the photonic isofrequency surface around epsilon-near-zero (ENZ) frequencies which can considerably change the spontaneous emission of a quantum emitter placed near a metamaterial slab. He