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تسجيل مستخدم جديدObservation of a random singlet state in a diluted Kitaev honeycomb material
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We report a $^{35}$Cl nuclear magnetic resonance (NMR) study of the diluted Kitaev material $alpha$-Ru$_{1-x}$Ir$_x$Cl$_3$ ($x=0.1$ and $0.2$) where non-magnetic Ir$^{3+}$ dopants substitute Ru$^{3+}$ ions. Upon dilution, the $^{35}$Cl spectra exhibit unusual large magnetic inhomogeneity, which sets in at temperatures below the Kitaev exchange energy scale. At the same time, the $^{35}$Cl spin-lattice relaxation rate $T_1^{-1}$ as a function of dilution and magnetic field unravels a critical doping of $x_capprox 0.22$, towards which both the field-induced spin gap and the zero-field magnetic ordering are simultaneously suppressed, while novel gapless low-energy spin excitations dominate the relaxation process. These NMR findings point to the stabilization of a random singlet phase in $alpha$-Ru$_{1-x}$Ir$_x$Cl$_3$, arising from the interplay of dilution and exchange frustration in the quantum limit.
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Quantum spin liquid is a disordered magnetic state with fractional spin excitations. Its clearest example is found in an exactly solved Kitaev honeycomb model where a spin flip fractionalizes into two types of anyons, quasiparticles that are neither
fermions nor bosons: a pair of gauge fluxes and a Majorana fermion. Here we demonstrate this kind of fractionalization in the Kitaev paramagnetic state of the honeycomb magnet $alpha$-RuCl$_3$. The spin-excitation gap measured by nuclear magnetic resonance consists of the predicted Majorana fermion contribution following the cube of the applied magnetic field, and a finite zero-field contribution matching the predicted size of the gauge-flux gap. The observed fractionalization into gapped anyons survives in a broad range of temperatures and magnetic fields despite inevitable non-Kitaev interactions between the spins, which are predicted to drive the system towards a gapless ground state. The gapped character of both anyons is crucial for their potential application in topological quantum computing.
In this work we investigate whether the Kitaev honeycomb model can serve as a starting point to realize the intriguing physics of the Sachdev-Ye-Kitaev model. The starting point is to strain the system which leads to flat bands reminiscent of Landau
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Strong spin-orbital-coupling magnetic systems with the honeycomb structure can provide bond-directional interactions which may result in Kitaev quantum spin liquids and exotic anyonic excitations. However, one of the key ingredients in real materials
$-$disorders$-$has been much less studied in Kitaev systems. Here we synthesized a trigonal SrIr$_2$O$_{6-delta}$ with $delta approx 0.25$, which consists of two-dimensional honeycomb Ir planes with edge-sharing IrO$_6$ octahedra. First-principles computation and experimental measurements suggest that the electronic system is gapped, and there should be no magnetic moment as the Ir$^{5+}$ ion has no unpaired electrons. However, significant magnetism has been observed in the material, and it can be attributed to disorders that are most likely from oxygen vacancies. No magnetic order is found down to 0.05 K, and the low-temperature magnetic properties exhibit power-law behaviors in magnetic susceptibility and zero-field specific heat, and a single-parameter scaling of the specific heat under magnetic fields. These results provide strong evidence for the existence of the random singlet phase in SrIr$_2$O$_{6-delta}$, which offers a different member to the family of spin-orbital entangled iridates and Kitaev materials.
$alpha$-RuCl$_{3}$ is a major candidate for the realization of the Kitaev quantum spin liquid, but its zigzag antiferromagnetic order at low temperatures indicates deviations from the Kitaev model. We have quantified the spin Hamiltonian of $alpha$-R
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