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Initializing quantum registers with high fidelity is a fundamental precondition for many applications like quantum information processing and sensing. The electronic and nuclear spins of a Nitrogen-Vacancy (NV) center in diamond form an interesting hybrid quantum register that can be initialized by a combination of laser, microwave, and radio-frequency pulses. However, the laser illumination, which is necessary for achieving electron spin polarization, also has the unwanted side-effect of depolarizing the nuclear spin. Here, we study how the depolarization dynamics of the $^{14}$N nuclear spin depends on the laser wavelength. We show experimentally that excitation with an orange laser (594 nm) causes significantly less nuclear spin depolarization compared to the green laser (532 nm) typically used for excitation and hence leads to higher nuclear spin polarization. This could be because orange light excitation inhibits ionization of NV$^{0}$ into NV$^{-}$ and therefore suppresses one source of noise acting on the nuclear spin.
We present a scheme to generate entangled photons using the NV centers in diamond. We show how the long-lived nuclear spin in diamond can mediate entanglement between multiple photons thereby increasing the length of entangled photon string. With the
Integrating atomic quantum memories based on color centers in diamond with on-chip photonic devices would enable entanglement distribution over long distances. However, efforts towards integration have been challenging because color centers can be hi
A common impediment to qubit performance is imperfect state initialization. In the case of the diamond nitrogen-vacancy (NV) center, the initialization fidelity is limited by fluctuations in the defects charge state during optical pumping. Here, we u
We investigated the depth dependence of coherence times of nitrogen-vacancy (NV) centers through precisely depth controlling by a moderately oxidative at 580{deg}C in air. By successive nanoscale etching, NV centers could be brought close to the diam
Nuclear spins nearby nitrogen-vacancy (NV) centers in diamond are excellent quantum memory for quantum computing and quantum sensing, but are difficult to be initialized due to their weak interactions with the environment. Here we propose and demonst