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The Effects of Radiation Damage on CLYC Performance

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 نشر من قبل Katherine Mesick
 تاريخ النشر 2017
  مجال البحث فيزياء
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Cs$_2$LiYCl$_6$:Ce$^{3+}$ (CLYC) is a new scintillator that is an attractive option for applications requiring the ability to detect both gamma rays and neutrons within a single volume. It is therefore of interest in applications that require low size, weight, or power, such as space applications. The radiation environment in space can over time damage the crystal structure of CLYC, leading to reduced performance. We have exposed 2 CLYC samples to 800 MeV protons at the Los Alamos Neutron Science Center, one to approximately 10 kRad and one to approximately 100 kRad. We measured the pulse shapes and amplitudes, energy resolution, and figure of merit for pulse-shape discrimination before and after irradiation. We have also measured the activation products and monitored for room-temperature annealing of the irradiated samples. The results of these measurements and the impact of radiation damage on CLYC performance is presented.

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Cerium-doped Cs$_2$LiYCl$_6$ (CLYC) and Cs$_2$LiLaBr$_x$Cl$_{6-x}$ (CLLBC) are scintillators in the elpasolite family that are attractive options for resource-constrained applications due to their ability to detect both gamma rays and neutrons within a single volume. Space-based detectors are one such application, however, the radiation environment in space can over time damage the crystal structure of the elpasolites, leading to degraded performance. We have exposed 4 samples each of CLYC and CLLBC to 800 MeV protons at the Los Alamos Neutron Science Center. The samples were irradiated with a total number of protons of 1.3$times$10$^{9}$, 1.3$times$10$^{10}$, 5.2$times$10$^{10}$, and 1.3$times$10$^{11}$, corresponding to estimated doses of 0.14, 1.46, 5.82, and 14.6 kRad, respectively on the CLYC samples and 0.14, 1.38, 5.52, and 13.8 kRad, respectively on the CLLBC samples. We report the impact these radiation doses have on the light output, activation, gamma-ray energy resolution, pulse shapes, and pulse-shape discrimination figure of merit for CLYC and CLLBC.
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