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We observe a disappearance of the 1/3 magnetization plateau and a striking change of the magnetic configuration under a moderate doping of the model triangular antiferromagnet RbFe(MoO4)2. The reason is an effective lifting of degeneracy of mean-field ground states by a random potential of impurities, which compensates, in the low temperature limit, the fluctuation contribution to free energy. These results provide a direct experimental confirmation of the fluctuation origin of the ground state in a real frustrated system. The change of the ground state to a least collinear configuration reveals an effective positive biquadratic exchange provided by the structural disorder. On heating, doped samples regain the structure of a pure compound thus allowing for an investigation of the remarkable competition between thermal and structural disorder.
RbFe(MoO4)2 is a quasi-two-dimensional (quasi-2D) triangular lattice antiferromagnet (TLA) that displays a zero-field magnetically-driven multiferroic phase with a chiral spin structure. By inelastic neutron scattering, we determine quantitatively th
The coupling of magnetic chiralities to the ferroelectric polarisation in multiferroic RbFe(MoO$_4$)$_2$ is investigated by neutron spherical polarimetry. Because of the axiality of the crystal structure below $T_textrm{c}$ = 190 K, helicity and tria
We identify and discuss the ground state of a quantum magnet on a triangular lattice with bond-dependent Ising-type spin couplings, that is, a triangular analog of the Kitaev honeycomb model. The classical ground-state manifold of the model is spanne
We report a high-resolution neutron diffraction study on the orbitally-degenerate spin-1/2 hexagonal antiferromagnet AgNiO2. A structural transition to a tripled unit cell with expanded and contracted NiO6 octahedra indicates root(3) x root(3) charge
Spin liquids occuring in 2D frustrated spin systems were initially assumed to appear at strongest frustration, but evidence grows that they more likely intervene at transitions between two different types of order. To identify if this is more general