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Magnetic compensated state attracted much interests due to the observed large exchange bias and large coercivity, and its potential applications in the antiferromagnetic spintronics with merit of no stray field. In this work, by ab initio calculations with KKR-CPA for the treatment of random substitution, we obtain the complete compensated states in the Ni (Pd, Pt) doped Mn3Ge-based D022-type tetragonal Heusler alloys. We find the total moment change is asymmetric across the compensation point (at ~ x = 0.3) in Mn3-xYxGe (Y = Ni, Pd, Pt), which is highly conforming to that experimentally observed in Mn3Ga. In addition, an uncommon discontinuous jump is observed across the critical zero-moment point, indicating that some non-trivial properties can emerge at this point. Further electronic analysis for the three compensation compositions reveals large spin polarizations, together with the high Curie temperature of the host Mn3Ge, making them promising candidates for spin transfer torque applications.
In recent years, antiferromagnetic spintronics has received much attention since ideal antiferromagnets do not produce stray fields and are much more stable to external magnetic fields compared to materials with net magnetization. Akin to antiferroma
Despite the potential advantages of information storage in antiferromagnetically coupled materials, it remains unclear whether one can control the magnetic moment orientation efficiently because of the cancelled magnetic moment. Here, we report spin-
We explore an opportunity to induce and control tetragonal distortion in materials. The idea involves formation of a binary alloy from parent compounds having body-centered and face-centered symmetries. The concept is illustrated in the case of FeNi$
Manipulation of magnetic ground states by effective control of competing magnetic interactions has led to the finding of many exotic magnetic states. In this direction, the tetragonal Heusler compounds consisting of multiple magnetic sublattices and
Based on high-throughput density functional theory calculations, we investigated the effects of light interstitial H, B, C, and N atoms on the magnetic properties of cubic Heusler alloys, with the aim to design new rare-earth free permanent magnets.