اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدQuantum-Spillover-Enhanced Surface-Plasmonic Absorption at the Interface of Silver and High-Index Dielectrics
192
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
We demonstrate an unexpectedly strong surface-plasmonic absorption at the interface of silver and high-index dielectrics based on electron and photon spectroscopy. The measured bandwidth and intensity of absorption deviate significantly from the classical theory. Our density-functional calculation well predicts the occurrence of this phenomenon. It reveals that due to the low metal-to-dielectric work function at such interfaces, conduction electrons can display a drastic quantum spillover, causing the interfacial electron-hole pair production to dominate the decay of surface plasmons. This finding can be of fundamental importance in understanding and designing quantum nano-plasmonic devices that utilize noble metals and high-index dielectrics.
قيم البحث
اقرأ أيضاً
Spectroscopic analysis of large biomolecules is critical in a number of applications, including medical diagnostics and label-free biosensing. Recently, it has been shown that Raman spectroscopy of proteins can be used to diagnose some diseases, incl
uding a few types of cancer. These experiments have however been performed using traditional Raman spectroscopy and the development of the Surface enhanced Raman spectroscopy (SERS) assays suitable for large biomolecules could lead to a substantial decrease in the amount of specimen necessary for these experiments. We present a new method to achieve high local field enhancement in surface enhanced Raman spectroscopy through the simultaneous adjustment of the lattice plasmons and localized surface plasmon polaritons, in a periodic bilayer nanoantenna array resulting in a high enhancement factor over the sensing area, with relatively high uniformity. The proposed plasmonic nanostructure is comprised of two interacting nanoantenna layers, providing a sharp band-edge lattice plasmon mode and a wide-band localized surface plasmon for the separate enhancement of the pump and emitted Raman signals. We demonstrate the application of the proposed nanostructure for the spectral analysis of large biomolecules by binding a protein (streptavidin) selectively on the hot-spots between the two stacked layers, using a low concentration solution (100 nM) and we successfully acquire its SERS spectrum.
Periodic arrays of air nanoholes in thin metal films that support surface plasmon resonances can provide an alternative approach for boosting the light-matter interactions at the nanoscale. Indeed, nanohole arrays have garnered great interest in rece
nt years for their use in biosensing, light emission enhancement and spectroscopy. However, the large-scale use of nanohole arrays in emerging technology requires new low-cost fabrication techniques. Here, we demonstrate a simple technique to fabricate nanohole arrays and examine their photonic applications. In contrast to the complicated and most commonly used electron beam lithography technique, hexagonal arrays of nanoholes are fabricated by using a simple combination of shadowing nanosphere lithography technique and electron beam deposition. These arrays are shown to offer enhancements in the lasing emission of an organic dye liquid gain medium with a quality factor above 150. Additionally, a 7-fold increase in Purcell factor is observed for CdSe quantum dot-integrated nanohole arrays.
The gain-assisted plasmonic analogue of electromagnetically induced transparency (EIT) in a metallic metamaterial is investigated for the purpose to enhance the sensing performance of the EIT-like plasmonic structure. The structure is composed of thr
ee bars in one unit, two of which are parallel to each other (dark quadrupolar element) but perpendicular to the third bar (bright dipolar element), The results show that, in addition to the high sensitivity to the refractive-index fluctuation of the surrounding medium, the figure of merit for such active EIT-like metamaterials can be greatly enhanced, which is attributed to the amplified narrow transparency peak.
The control of quantum states of light at the nanoscale has become possible in recent years with the use of plasmonics. Here, many types of nanophotonic devices and applications have been suggested that take advantage of quantum optical effects, desp
ite the inherent presence of loss. A key example is quantum plasmonic sensing, which provides sensitivity beyond the classical limit using entangled N00N states and their generalizations in a compact system operating below the diffraction limit. In this work, we experimentally demonstrate the excitation and propagation of a two-plasmon entangled N00N state (N=2) in a silver nanowire, and assess the performance of our system for carrying out quantum sensing. Polarization entangled photon pairs are converted into plasmons in the silver nanowire, which propagate over a distance of 5 um and re-convert back into photons. A full analysis of the plasmonic system finds that the high-quality entanglement is preserved throughout. We measure the characteristic super-resolution phase oscillations of the entangled state via coincidence measurements. We also identify various sources of loss in our setup and show how they can be mitigated, in principle, in order to reach super-sensitivity that goes beyond the classical sensing limit. Our results show that polarization entanglement can be preserved in a plasmonic nanowire and that sensing with a quantum advantage is possible with moderate loss present.
By extracting the permittivity of monolayer MoS2 from experiments, the optical absorption of monolayer MoS2 prepared on top of one-dimensional photonic crystal (1DPC) or metal films is investigated theoretically. The 1DPC and metal films act as reson
ant back reflectors that can enhance absorption of monolayer MoS2 substantially over a broad spectral range due to the Fabry-Perot cavity effect. The absorption of monolayer MoS2 can also be tuned by varying either the distance between the monolayer MoS2 and the back reflector or the thickness of the cover layers.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
