اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدAbsorption enhancing proximity effects in aperiodic nanowire arrays
159
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
Aperiodic Nanowire (NW) arrays have higher absorption than equivalent periodic arrays, making them of interest for photovoltaic applications. An inevitable property of aperiodic arrays is the clustering of some NWs into closer proximity than in the equivalent periodic array. We focus on the modes of such clusters and show that the reduced symmetry associated with cluster formation allows external coupling into modes which are dark in periodic arrays, thus increasing absorption. To exploit such modes fully, arrays must include tightly clustered NWs that are unlikely to arise from fabrication variations but must be created intentionally.
قيم البحث
اقرأ أيضاً
Absorption spectroscopy is widely used to detect samples with spectral specificity. Here, we propose and demonstrate a method for enhancing the sensitivity of absorption spectroscopy. Exploiting multiple light scattering generated by a boron nitride
(h-BN) scattering cavity, the optical path lengths of light inside a diffusive reflective cavity are significantly increased, resulting in more than ten times enhancement of sensitivity in absorption spectroscopy. We demonstrate highly sensitive spectral measurements of low concentrations of malachite green and crystal violet aqueous solutions. Because this method only requires the addition of a scattering cavity to existing absorption spectroscopy, it is expected to enable immediate and widespread applications in various fields, from analytical chemistry to environmental sciences.
In this paper we show that arrays of core-shell nanoparticles function as effective thin absorbers of light. In contrast to known metamaterial absorbers, the introduced absorbers are formed by single planar arrays of spherical inclusions and enable f
ull absorption of light incident on either or both sides of the array. We demonstrate possibilities for realizing different kinds of symmetric absorbers, including resonant, ultra-broadband, angularly selective, and all-angle absorbers. The physical principle behind these designs is explained considering balanced electric and magnetic responses of unit cells. Photovoltaic devices and thermal emitters are the two most important potential applications of the proposed designs.
The optical response of a coupled nanowire dimer is studied using a fully quantum mechanical approach. The translational invariance of the system allows to apply the time--dependent density functional theory for the plasmonic dimer with the largest s
ize considered so far in quantum calculations. Detailed comparisons with results from classical electromagnetic calculations based on local and non local hydrodynamic response, as well as with results of the recently developed quantum corrected model is performed. We show that electron tunneling and dynamical screening are the major nonlocal quantum effects determining the plasmonic modes and field enhancement in the system. Account for the electron tunneling at small junction sizes allows semi-quantitative description of quantum results within classical framework. We also discuss the shortcomings of classical treatments using non-local dielectric permittivities based on hydrodynamic models. Finally, the implications of the actual position of the screening charge density for the plasmon ruler applications are demonstrated.
Hexagonally aligned, free-standing silicon nanowire (SiNW) arrays serve as photonic resonators which, as compared to a silicon (Si) thin film, do not only absorb more visible (VIS) and near-infrared (NIR) light, but also show an inherent photonic lig
ht concentration that enhances their performance as solar absorbers. Using numerical simulations we show, how light concentration is induced by high optical cross sections of the individual SiNWs but cannot be optimized independently of the SiNW array absorption. While an ideal spatial density exists, for which the SiNW array absorption for VIS and NIR wavelengths reaches a maximum, the spatial correlation of SiNWs in an array suppresses the formation of optical Mie modes responsible for light concentration. We show that different from SiNWs with straight sidewalls, arrays of inverted silicon nanocones (SiNCs) permit to avoid the mode suppression. In fact they give rise to an altered set of photonic modes which is induced by the spatial correlation of SiNCs in the array, and therefore show a higher degree of freedom to independently optimize light absorption and light concentration. Apart from explaining the good light absorbing and concentrating properties of SiNC arrays, the work justifies a revaluation of SiNW arrays as optical absorbers.
Nanowire arrays exhibit efficient light coupling and strong light trapping, making them well suited to solar cell applications. The processes that contribute to their absorption are interrelated and highly dispersive, so the only current method of op
timizing the absorption is by intensive numerical calculations. We present an efficient alternative which depends solely on the wavelength-dependent refractive indices of the constituent materials. We choose each array parameter such that the number of modes propagating away from the absorber is minimized while the number of resonant modes within the absorber is maximized. From this we develop a semi-analytic method that quantitatively identifies the small range of parameters where arrays achieve maximum short circuit currents. This provides a fast route to optimizing NW array cell efficiencies by greatly reducing the geometries to study with full device models. Our approach is general and applies to a variety of materials and to a large range of array thicknesses.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
