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The generation of the shortest isolated attosecond pulses requires both broad spectral bandwidth and control of the spectral phase. Rapid progress has been made in both aspects, leading to the generation of the world-record-shortest 67 as light pulses in 2012, and broadband attosecond continua covering a wide range of extreme ultraviolet and soft x-ray wavelengths. Such pulses have been successfully applied in photoelectron/photoion spectroscopy and the recently developed attosecond transient absorption spectroscopy to study electron dynamics in matter. In this Review, we discuss the significant recent advancement in the generation, characterization, and application of ultrabroadband isolated attosecond pulses with spectral bandwidth comparable to the central frequency, which can in principle be compressed to a single optical cycle.
The generation of coherent light pulses in the extreme ultraviolet (XUV) spectral region with attosecond pulse durations constitutes the foundation of the field of attosecond science. Twenty years after the first demonstration of isolated attosecond
High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest attosecond (as) pulses have been produced only in the extreme ultraviolet (EUV) region o
On the basis of real-time ab initio calculations, we study the non-perturbative interaction of two-color laser pulses with MgO crystal in the strong field regime to generate isolated attosecond pulse from high-harmonic emissions from MgO crystal. In
The shortest light pulses produced to date are of the order of a few tens of attoseconds, with central frequencies in the extreme ultraviolet range and bandwidths exceeding tens of eV. They are often produced as a train of pulses separated by half th
Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting to measure