ترغب بنشر مسار تعليمي؟ اضغط هنا

Frustrated minority spins in GeNi2O4

44   0   0.0 ( 0 )
 نشر من قبل Seunghun Lee
 تاريخ النشر 2007
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

Recently, two consecutive phase transitions were observed, upon cooling, in an antiferromagnetic spinel GeNi$_2$O$_4$ at $T_{N1}=12.1$ K and $T_{N2}=11.4$ K, respectively cite{matsuno, crawford}. Using unpolarized and polarized elastic neutron scattering we show that the two transitions are due to the existence of frustrated minority spins in this compound. Upon cooling, at $T_{N1}$ the spins on the $<111>$ kagome planes order ferromagnetically in the plane and antiferromagnetically between the planes (phase I), leaving the spins on the $<111>$ triangular planes that separate the kagome planes frustrated and disordered. At the lower $T_{N2}$, the triangular spins also order in the $<111>$ plane (phase II). We also present a scenario involving exchange interactions that qualitatively explains the origin of the two purely magnetic phase transitions.

قيم البحث

اقرأ أيضاً

66 - Julien Robert 2008
Using magnetization, specific heat and neutron scattering measurements, as well as exact calculations on realistic models, the magnetic properties of the lacuvo compound are characterized on a wide temperature range. At high temperature, this oxide i s well described by strongly correlated atomic $S$=1/2 spins while decreasing the temperature it switches to a set of weakly interacting and randomly distributed entangled pseudo spins $tilde S=1/2$ and $tilde S=0$. These pseudo-spins are built over frustrated clusters, similar to the kagome building block, at the vertices of a triangular superlattice, the geometrical frustration intervening then at different scales.
109 - T. Basu , T. Zou , Z. Dun 2020
Cubic spinel GeNi2O4 exhibits intriguing magnetic properties with two successive antiferromagnetic phase transitions (TN1 12.1 and TN2 11.4 K) with the absence of any structural transition. We have performed detailed heat capacity and magnetic measur ements in different crystallographic orientations. A new magnetic phase in presence of magnetic field (H > 4 T) along the [111] direction is revealed, which is not observed when the magnetic field is applied along the [100] and [110] directions. High field neutron powder diffraction measurements confirm such a change in magnetic phase, which could be ascribed to a spin reorientation in the presence of magnetic field. A strong magnetic anisotropy and competing magnetic interactions play a crucial role on the complex magnetic behavior in this cubic system.
The crystal structures of the A2B2O7-x Niobium-based pyrochlores Y2(Nb0.86Y0.14)2O6.91, CaYNb2O7, and Y2NbTiO7 are reported, determined by powder neutron diffraction. These compounds represent the first observation of B-site displacements in the pyro chlore structure: the B-site ions are found to be displaced from the ideal pyrochlore positions, creating electric dipoles. The orientations of these dipoles are fully analogous to orientations of the magnetic moments in Ising spin based magnetically frustrated pyrochlores. Diffuse scattering in electron diffraction patterns shows that the displacements are only short range ordered, indicative of geometric frustration of the collective dielectric state of the materials. Comparison to the crystal structure of the Nb5+ (d0) pyrochlore La2ScNbO7 supports the prediction that charge singlets, driven by the tendency of Nb to form metal-metal bonds, are present in these pyrochlores. The observed lack of long-range order to these singlets suggests that Nb4+-based pyrochlores represent the dielectric analogy to the geometric frustration of magnetic moments observed in rare earth pyrochlores.
The inability of systems of interacting objects to satisfy all constraints simultaneously leads to frustration. A particularly important consequence of frustration is the ability to access certain protected parts of a system without disturbing the ot hers. For magnets such protectorates have been inferred from theory and from neutron scattering, but their practical consequences have been unclear. We show that a magnetic analogue of optical hole-burning can address these protected spin clusters in a well-known, geometrically frustrated Heisenberg system, gadolinium gallium garnet. Our measurements additionally provide a resolution of a famous discrepancy between the bulk magnetometry and neutron diffraction results for this magnetic compound.
83 - S. Ji , S.-H. Lee , C. Broholm 2009
Using synchrotron X-rays and neutron diffraction we disentangle spin-lattice order in highly frustrated ZnCr$_2$O$_4$ where magnetic chromium ions occupy the vertices of regular tetrahedra. Upon cooling below 12.5 K the quandary of anti-aligning spin s surrounding the triangular faces of tetrahedra is resolved by establishing weak interactions on each triangle through an intricate lattice distortion. The resulting spin order is however, not simply a N{e}el state on strong bonds. A complex co-planar spin structure indicates that antisymmetric and/or further neighbor exchange interactions also play a role as ZnCr$_2$O$_4$ resolves conflicting magnetic interactions.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا