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تسجيل مستخدم جديدTo reach neutron-rich heavy and superheavy nuclei by multinucleon transfer reactions with radioactive isotopes
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The dynamical mechanism of multinucleon transfer (MNT) reactions has been investigated within the dinuclear system (DNS) model, in which the sequential nucleon transfer is described by solving a set of microscopically derived master equations. Production cross sections, total kinetic energy spectra, angular distribution of formed fragments in the reactions of $^{124,132}$Sn+ $^{238}$U/$^{248}$Cm near Coulomb barrier energies are thoroughly analyzed. It is found that the total kinetic energies of primary fragments are dissipated from the relative motion energy and rotational energy of the two colliding nuclei. The fragments are formed in the forward angle domain. The energy dependence of the angular spectra is different between projectile-like and target-like fragments. Isospin equilibrium is governed under the potential energy surface. The production cross sections of neutron-rich isotopes are enhanced around the shell closure.
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Within the framework of the dinuclear system model, the production mechanism of neutron-rich heavy nuclei around N = 162 has been investigated systematically. The isotopic yields in the multinucleon transfer reaction of $^{238}$U + $^{248}$Cm was ana
lyzed and compared the available experimental data. Systematics on the production of superheavy nuclei via $^{238}$U on $^{252,254}$Cf, $^{254}$Es and $^{257}$Fm is investigated. It is found that the shell effect is of importance in the formation of neutron-rich nuclei around N=162 owing to the enhancement of fission barrier. The fragments in the multinucleon transfer reactions manifest the broad isotopic distribution and are dependent on the beam energy. The polar angles of the fragments tend to the forward emission with increasing the beam energy. The production cross sections of new isotopes are estimated and heavier targets are available for the neutron-rich superheavy nucleus formation. The optimal system and beam energy are proposed for the future experimental measurements.
The multinucleon transfer reactions in collisions of $^{136}$Xe+$^{198}$Pt at incident energies $E_{textrm{lab}}=$5.25, 6.20, 7.98, 10.0, and 15.0 MeV/nucleon are investigated by using the improved quantum molecular dynamics model. It is found that 6
.20 MeV/nucleon is the optimal incident energy for producing the neutron-rich heavy nuclei. About 80 unknown neutron-rich nuclei might be produced in this reaction with cross sections from 10$^{-6}$ to 10$^{-2}$ mb. The angular distributions of the neutron-rich isotopes are predicted.
Within the dinuclear system model, unknown neutron-deficient isotopes Np, Pu, Am, Cm, Bk, Cf, Es, Fm are investigated in $^{40}$Ca, $^{36,40}$Ar, $^{32}$S, $^{28}$Si,$^{24}$Mg induced fusion-evaporation reactions and multinucleon transfer reactions w
ith radioactive beams $^{59}$Cu,$^{69}$As,$^{90}$Nb,$^{91}$Tc, $^{94}$Rh, $^{105,110}$Sn, $^{118}$Xe induced with $^{238}$U near Coulomb barrier energies. The production cross sections of compound nuclei in the fusion-evaporation reactions and fragments yields in the multinucleon transfer reactions are calculated within the model. A statistical approach is used to evaluate the survival probability of excited nuclei via the both reaction mechanisms. A dynamical deformation is implemented into the model in the dissipation process. It is found that charge particle channels (alpha and proton) dominate in the decay process of proton-rich nuclides and the fusion-evaporation reactions are favorable to produce the new neutron-deficient actinide isotopes. The total kinetic energies and angular spectra of primary fragments are strongly dependent on colliding orientations.
The multinucleon transfer reaction in the collisions of $^{40}$Ca+$^{124}$Sn at $E_{textrm{c.m.}}=128.5$ MeV is investigated by using the improved quantum molecular dynamics model. The measured angular distributions and isotopic distributions of the
products are reproduced reasonably well by the calculations. The multinucleon transfer reactions of $^{40}$Ca+$^{112}$Sn, $^{58}$Ni+$^{112}$Sn, $^{106}$Cd+$^{112}$Sn, and $^{48}$Ca+$^{112}$Sn are also studied. It shows that the combinations of neutron-deficient projectile and target are advantageous to produce the exotic neutron-deficient nuclei near $N, Z$ = 50. The charged particles emission plays an important role at small impact parameters in the deexcitation processes of the system. The production cross sections of the exotic neutron-deficient nuclei in multinucleon transfer reactions are much larger than those measured in the fragmentation and fusion-evaporation reactions. Several new neutron-deficient nuclei can be produced in $^{106}$Cd+$^{112}$Sn reaction. The corresponding production cross sections for the new neutron-deficient nuclei, $^{101,102}$Sb, $^{103}$Te, and $^{106,107}$I, are 2.0 nb, 4.1 nb, 6.5 nb, 0.4 $mu$b and 1.0 $mu$b, respectively.
The heavy-ion fusion reactions induced by neutron-rich nuclei are investigated with the improved quantum molecular dynamics (ImQMD) model. With a subtle consideration of the neutron skin thickness of nuclei and the symmetry potential, the stability o
f nuclei and the fusion excitation functions of heavy-ion fusion reactions $^{16}$O+$^{76}$Ge, $^{16}$O+$^{154}$Sm, $^{40}$Ca+$^{96}$Zr and $^{132}$Sn+$^{40}$Ca are systematically studied. The fusion cross sections of these reactions at energies around the Coulomb barrier can be well reproduced by using the ImQMD model. The corresponding slope parameter of the symmetry energy adopted in the calculations is $L approx 78$ MeV and the surface energy coefficient is $g_{rm sur}=18pm 1.5$ MeVfm$^2$. In addition, it is found that the surface-symmetry term significantly influences the fusion cross sections of neutron-rich fusion systems. For sub-barrier fusion, the dynamical fluctuations in the densities of the reaction partners and the enhanced surface diffuseness at neck side result in the lowering of the fusion barrier.
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