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تسجيل مستخدم جديدProduction mechanism of neutron-deficient actinide isotopes in complete fusion reactions and multinucleon transfer reactions
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Within the dinuclear system model, unknown neutron-deficient isotopes Np, Pu, Am, Cm, Bk, Cf, Es, Fm are investigated in $^{40}$Ca, $^{36,40}$Ar, $^{32}$S, $^{28}$Si,$^{24}$Mg induced fusion-evaporation reactions and multinucleon transfer reactions with radioactive beams $^{59}$Cu,$^{69}$As,$^{90}$Nb,$^{91}$Tc, $^{94}$Rh, $^{105,110}$Sn, $^{118}$Xe induced with $^{238}$U near Coulomb barrier energies. The production cross sections of compound nuclei in the fusion-evaporation reactions and fragments yields in the multinucleon transfer reactions are calculated within the model. A statistical approach is used to evaluate the survival probability of excited nuclei via the both reaction mechanisms. A dynamical deformation is implemented into the model in the dissipation process. It is found that charge particle channels (alpha and proton) dominate in the decay process of proton-rich nuclides and the fusion-evaporation reactions are favorable to produce the new neutron-deficient actinide isotopes. The total kinetic energies and angular spectra of primary fragments are strongly dependent on colliding orientations.
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The multinucleon transfer reaction in the collisions of $^{40}$Ca+$^{124}$Sn at $E_{textrm{c.m.}}=128.5$ MeV is investigated by using the improved quantum molecular dynamics model. The measured angular distributions and isotopic distributions of the
products are reproduced reasonably well by the calculations. The multinucleon transfer reactions of $^{40}$Ca+$^{112}$Sn, $^{58}$Ni+$^{112}$Sn, $^{106}$Cd+$^{112}$Sn, and $^{48}$Ca+$^{112}$Sn are also studied. It shows that the combinations of neutron-deficient projectile and target are advantageous to produce the exotic neutron-deficient nuclei near $N, Z$ = 50. The charged particles emission plays an important role at small impact parameters in the deexcitation processes of the system. The production cross sections of the exotic neutron-deficient nuclei in multinucleon transfer reactions are much larger than those measured in the fragmentation and fusion-evaporation reactions. Several new neutron-deficient nuclei can be produced in $^{106}$Cd+$^{112}$Sn reaction. The corresponding production cross sections for the new neutron-deficient nuclei, $^{101,102}$Sb, $^{103}$Te, and $^{106,107}$I, are 2.0 nb, 4.1 nb, 6.5 nb, 0.4 $mu$b and 1.0 $mu$b, respectively.
Within the framework of the dinuclear system model, the production mechanism of neutron-rich heavy nuclei around N = 162 has been investigated systematically. The isotopic yields in the multinucleon transfer reaction of $^{238}$U + $^{248}$Cm was ana
lyzed and compared the available experimental data. Systematics on the production of superheavy nuclei via $^{238}$U on $^{252,254}$Cf, $^{254}$Es and $^{257}$Fm is investigated. It is found that the shell effect is of importance in the formation of neutron-rich nuclei around N=162 owing to the enhancement of fission barrier. The fragments in the multinucleon transfer reactions manifest the broad isotopic distribution and are dependent on the beam energy. The polar angles of the fragments tend to the forward emission with increasing the beam energy. The production cross sections of new isotopes are estimated and heavier targets are available for the neutron-rich superheavy nucleus formation. The optimal system and beam energy are proposed for the future experimental measurements.
The dynamical mechanism of multinucleon transfer (MNT) reactions has been investigated within the dinuclear system (DNS) model, in which the sequential nucleon transfer is described by solving a set of microscopically derived master equations. Produc
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