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113 - Yongkang Luo , Han Han , Hao Tan 2011
A cerium containing pnictide, CeNiAsO, crystallized in the ZrCuSiAs type structure, has been investigated by measuring transport and magnetic properties, as well as specific heat. We found that CeNiAsO is an antiferromagnetic dense Kondo lattice meta llic compound with Kondo scale $T_K sim$ 15 K and shows an enhanced Sommerfeld coefficient of $gamma_0 sim$ 203 mJ/mol$cdot$K$^{2}$. While no superconductivity can been observed down to 30 mK, Ce ions exhibit two successive antiferromagnetic (AFM) transitions. We propose that the magnetic moment of Ce ion could align in the G type AFM order below the first transition at $T_{N1}$=9.3 K, and it might be modified into the C type AFM order below a lower transition at $T_{N2}$=7.3 K. Our results indicate that the 3$d-4f$ interlayer Kondo interactions play an important role in Ni-based Ce-containing pnictide.
79 - Yongkang Luo , Qian Tao , Yuke Li 2009
We report measurements of structural phase transition of four parent compounds $R$FeAsO ($R$ = La, Sm, Gd, and Tb) by means of low-temperature X-ray diffraction (XRD). Magnetic transition temperatures associated with Fe ions ($T_{N1}$) are also deter mined from the temperature dependence of resistivity. As $R$ is changed from La, through Sm and Gd, to Tb, both the c-axis and a-axis lattice constants decrease significantly. Meanwhile both the structural phase transition temperature ($T_S$) and $T_{N1}$ decrease monotonously. It is also found that the temperature gap between $T_S$ and $T_{N1}$ becomes smaller when the distance between FeAs layer becomes shorter. This result is consistent with magnetically driven structural phase transition and suggests that the dimensionality have an important effect on the AFM ordering.
80 - Yuke Li , Xiao Lin , Qian Tao 2009
We report Zn-doping effect in the parent and F-doped LaFeAsO oxy-arsenides. Slight Zn doping in LaFe$_{1-x}$Zn$_{x}$AsO drastically suppresses the resistivity anomaly around 150 K associated with the antiferromagnetic (AFM) spin density wave (SDW) in the parent compound. The measurements of magnetic susceptibility and thermopower confirm further the effect of Zn doping on AFM order. Meanwhile Zn doping does not affect or even enhances the $T_c$ of LaFe$_{1-x}$Zn$_{x}$AsO$_{0.9}$F$_{0.1}$, in contrast to the effect of Zn doping in high-$T_c$ cuprates. We found that the solubility of Zn content ($x$) is limited to less than 0.1 in both systems and further Zn doping (i.e., $x$ $geq$ 0.1) causes phase separation. Our study clearly indicates that the non-magnetic impurity of Zn$^{2+}$ ions doped in the Fe$_2$As$_2$ layers affects selectively the AFM order, and superconductivity remains robust against the Zn doping in the F-doped superconductors.
233 - Y. K. Li , X. Lin , Z. W. Zhu 2009
We investigate superconductivity and transport properties of Co doped SmFe$_{1-x}$Co$_{x}$AsO system. The antiferromagnetic (AFM) spin-density wave (SDW) order is rapidly suppressed by Co doping, and superconductivity emerges as $x$ $geq$ 0.05. $T_c$ $^{mid}$ increases with increasing Co content, shows a maximum of 17.2 K at the optimally doping of $xsim$ 0.10. A phase diagram is derived based on the transport measurements and a dome-like $T_c$ versus $x$ curve is established. Meanwhile we found that the normal state thermopower might consist of two different contributions. One contribution increases gradually with increasing $x$, and the other contribution is abnormally enhanced in the superconducting window 0.05 $leq$ $x$ $leq$ 0.20, and shows a dome-like doping dependence. A close correlation between $T_{c}$ and the abnormally enhanced term of thermopower is proposed.
125 - L. J. Li , Q. B. Wang , Y. K. Luo 2008
A series of 122 phase BaFe$_{2-x}$Ni$_x$As$_2$ ($x$ = 0, 0.055, 0.096, 0.18, 0.23) single crystals were grown by self flux method and a dome-like Ni doping dependence of superconducting transition temperature is discovered. The transition temperature $T_c^{on}$ reaches a maximum of 20.5 K at $x$ = 0.096, and it drops to below 4 K as $x$ $geq$ 0.23. The negative thermopower in the normal state indicates that electron-like charge carrier indeed dominates in this system. This Ni-doped system provides another example of superconductivity induced by electron doping in the 122 phase.
74 - X. F. Xu , Z. A. Xu , T. J. Liu 2008
We present the first measurement on Nernst effect in the normal state of odd-parity, spin-triplet superconductor Sr$_{2}$RuO$_{4}$. Below 100 K, the Nernst signal was found to be negative, large, and, as a function of magnetic field, nonlinear. Its m agnitude increases with the decreasing temperature until reaching a maximum around $T^*$ $approx$ 20 - 25 K, below which it starts to decrease linearly as a function of temperature. The large value of the Nernst signal appears to be related to the multiband nature of the normal state and the nonlinearity to band-dependent magnetic fluctuation in Sr$_{2}$RuO$_{4}$. We argue that the sharp decrease in Nernst signal below $T^*$ is due to the suppression of quasiparticle scattering and the emergence of band-dependent coherence in the normal state. The observation of a sharp kink in the temperature dependent thermopower around $T^*$ and a sharp drop of Hall angle at low temperatures provide additional support to this picture.
143 - Z. W. Zhu , Z. A. Xu , X. Lin 2008
We report the first Nernst effect measurement on the new iron-based superconductor LaO$_{1-x}$F$_{x}$FeAs $(x=0.1)$. In the normal state, the Nernst signal is negative and very small. Below $T_{c}$ a large positive peak caused by vortex motion is obs erved. The flux flowing regime is quite large compared to conventional type-II superconductors. However, a clear deviation of the Nernst signal from normal state background and an anomalous depression of off-diagonal thermoelectric current in the normal state between $T_{c}$ and 50 K are observed. We propose that this anomaly in the normal state Nernst effect could correlate with the SDW fluctuations.
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