Measurement of the Angular Dependence of the Dipole-Dipole Interaction Between Two Individual Rydberg Atoms at a Forster Resonance

We measure the angular dependence of the resonant dipole-dipole interaction between two individual Rydberg atoms with controlled relative positions. By applying a combination of static electric and magnetic fields on the atoms, we demonstrate the possibility to isolate a single interaction channel at a Forster resonance, that shows a well-defined angular dependence. We first identify spectroscopically the Forster resonance of choice and we then perform a direct measurement of the interaction strength between the two atoms as a function of the angle between the internuclear axis and the quantization axis. Our results show good agreement with the expected angular dependence $propto(1-3cos^2theta)$, and represent an important step towards quantum state engineering in two-dimensional arrays of individual Rydberg atoms.

Coherent Excitation Transfer in a Spin Chain of Three Rydberg Atoms

We study coherent excitation hopping in a spin chain realized using highly excited individually addressable Rydberg atoms. The dynamics are fully described in terms of an XY spin Hamiltonian with a long range resonant dipole-dipole coupling that scales as the inverse third power of the lattice spacing, $C_3/R^3$. The experimental data demonstrate the importance of next neighbor interactions which are manifest as revivals in the excitation dynamics. The results suggest that arrays of Rydberg atoms are ideally suited to large scale, high-fidelity quantum simulation of spin dynamics.

Coherent dipole-dipole coupling between two single atoms at a Forster resonance

Resonant energy transfers, i.e. the non-radiative redistribution of an electronic excitation between two particles coupled by the dipole-dipole interaction, lie at the heart of a variety of chemical and biological phenomena, most notably photosynthesis. In 1948, Forster established the theoretical basis of fluorescence resonant energy transfer (FRET), paving the ground towards the widespread use of FRET as a spectroscopic ruler for the determination of nanometer-scale distances in biomolecules. The underlying mechanism is a coherent dipole-dipole coupling between particles, as already recognized in the early days of quantum mechanics, but this coherence was not directly observed so far. Here, we study, both spectroscopically and in the time domain, the coherent, dipolar-induced exchange of electronic excitations between two single Rydberg atoms separated by a controlled distance as large as 15 microns, and brought into resonance by applying a small electric field. The coherent oscillation of the system between two degenerate pair states occurs at a frequency that scales as the inverse third power of the distance, the hallmark of dipole-dipole interactions. Our results not only demonstrate, at the most fundamental level of two atoms, the basic mechanism underlying FRET, but also open exciting prospects for active tuning of strong, coherent interactions in quantum many-body systems.

A purely dipolar quantum gas

We report on experiments exploring the physics of dipolar quantum gases using a Chromium Bose-Einstein condensate (BEC). By means of a Feshbach resonance, it is possible to reduce the effects of short range interactions and reach a regime where the physics is governed by the long-range, anisotropic dipole-dipole interaction between the large ($6 mu_{rm B}$) magnetic moments of Chromium atoms. Several dramatic effects of the dipolar interaction are observed: the usual inversion of ellipticity of the condensate during time-of flight is inhibited, the stability of the dipolar gas depends strongly on the trap geometry, and the explosion following the collapse of an unstable dipolar condensate displays d-wave like features.

Strong dipolar effects in a quantum ferrofluid

We report on the realization of a Chromium Bose-Einstein condensate (BEC) with strong dipolar interaction. By using a Feshbach resonance, we reduce the usual isotropic contact interaction, such that the anisotropic magnetic dipole-dipole interaction between 52Cr atoms becomes comparable in strength. This induces a change of the aspect ratio of the cloud, and, for strong dipolar interaction, the inversion of ellipticity during expansion - the usual smoking gun evidence for BEC - can even be suppressed. These effects are accounted for by taking into account the dipolar interaction in the superfluid hydrodynamic equations governing the dynamics of the gas, in the same way as classical ferrofluids can be described by including dipolar terms in the classical hydrodynamic equations. Our results are a first step in the exploration of the unique properties of quantum ferrofluids.

Stabilizing a purely dipolar quantum gas against collapse

We report on the experimental observation of the dipolar collapse of a quantum gas which sets in when we reduce the contact interaction below some critical value using a Feshbach resonance. Due to the anisotropy of the dipole-dipole interaction, the stability of a dipolar Bose-Einstein condensate depends not only on the strength of the contact interaction, but also on the trapping geometry. We investigate the stability diagram and find good agreement with a universal stability threshold arising from a simple theoretical model. Using a pancake-shaped trap with the dipoles oriented along the short axis of the trap, we are able to tune the scattering length to zero, stabilizing a purely dipolar quantum gas.