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113 - L. Chen , T. T. Han , C. Cai 2021
Pairing symmetry which characterizes the superconducting pairing mechanism is normally determined by measuring the superconducting gap structure ($|Delta_k|$). Here, we report the measurement of a strain-induced gap modulation ($partial|Delta_k|$) in uniaxially strained Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ utilizing angle-resolved photoemission spectroscopy and $in$-$situ$ strain-tuning. We found that the uniaxial strain drives Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ into a nematic superconducting state which breaks the four-fold rotational symmetry of the superconducting pairing. The superconducting gap increases on the $d_{yz}$ electron and hole pockets while it decreases on the $d_{xz}$ counterparts. Such orbital selectivity indicates that orbital-selective pairing exists intrinsically in non-nematic iron-based superconductors. The $d_{xz}$ and $d_{yz}$ pairing channels are balanced originally in the pristine superconducting state, but become imbalanced under uniaxial strain. Our results highlight the important role of intra-orbital scattering in mediating the superconducting pairing in iron-based superconductors. It also highlights the measurement of $partial|Delta_k|$ as an effective way to characterize the superconducting pairing from a perturbation perspective.
The recently discovered Indus stellar stream exhibits a diverse chemical signature compared to what is found for most other streams due to the abundances of two outlier stars, Indus$_$0 and Indus$_$13. Indus$_$13, exhibits an extreme enhancement in r apid neutron-capture ($r$-)process elements with $mathrm{[Eu/Fe]} = +1.81$. It thus provides direct evidence of the accreted nature of $r$-process enhanced stars. In this paper we present a detailed chemical analysis of the neutron-capture elements in Indus$_$13, revealing the star to be slightly actinide poor. The other outlier, Indus$_0$, displays a globular cluster-like signature with high N, Na, and Al abundances, while the rest of the Indus stars show abundances compatible with a dwarf galaxy origin. Hence, Indus$_0$ provides the first chemical evidence of a fully disrupted dwarf containing a globular cluster. We use the chemical signature of the Indus stars to discuss the nature of the stream progenitor which was likely a chemically evolved system, with a mass somewhere in the range from Ursa Minor to Fornax.
248 - T. T. Han , L. Chen , C. Cai 2021
Artificially created two-dimensional (2D) interfaces or structures are ideal for seeking exotic phase transitions due to their highly tunable carrier density and interfacially enhanced many-body interactions. Here, we report the discovery of a metal- insulator transition (MIT) and an emergent gapped phase in the metal-semiconductor interface that is created in 2H-MoTe$_2$ via alkali-metal deposition. Using angle-resolved photoemission spectroscopy, we found that the electron-phonon coupling is strong at the interface as characterized by a clear observation of replica shake-off bands. Such strong electron-phonon coupling interplays with disorder scattering, leading to an Anderson localization of polarons which could explain the MIT. The domelike emergent gapped phase could then be attributed to a polaron extended state or phonon-mediated superconductivity. Our results demonstrate the capability of alkali-metal deposition as an effective method to enhance the many-body interactions in 2D semiconductors. The surface-doped 2H-MoTe$_2$ is a promising candidate for realizing polaronic insulator and high-$T_c$ superconductivity.
289 - L. Chen , T. T. Han , C. Cai 2020
Excitonic insulator (EI) is an intriguing insulating phase of matter, where electrons and holes are bonded into pairs, so called excitons, and form a phase-coherent state via Bose-Einstein Condensation (BEC). Its theoretical concept has been proposed several decades ago, but the followed research is very limited, due to the rare occurrence of EI in natural materials and the lack of manipulating method of excitonic condensation. In this paper, we report the realization of a doping-controlled EI-to-semi-metal transition in Ta$_2$NiSe$_5$ using $in$-$situ$ potassium deposition. Combining with angle-resolved photoemission spectroscopy (ARPES), we delineate the evolution of electronic structure through the EI transition with unprecedented precision. The results not only show that Ta$ _2 $NiSe$ _5 $ (TNS) is an EI originated from a semi-metal non-interacting band structure, but also resolve two sequential transitions, which could be attributed to the phase-decoherence and pair-breaking respectively. Our results unveil the Bardeen-Cooper-Schrieffer (BCS)-BEC crossover behavior of TNS and demonstrate that its band structure and excitonic binding energy can be tuned precisely via alkali-metal deposition. This paves a way for investigations of BCS-BEC crossover phenomena, which could provide insights into the many-body physics in condensed matters and other many-body systems.
Recent analysis of the second data release of Gaia has revealed a number of new stellar streams surrounding the Milky Way. It has been suggested that one of these streams, Gjoll, is associated with the globular cluster NGC 3201, but thus far the asso ciation has only been based on kinematics of the stream stars. In this work we identify five likely stream members in the Gaia data that are bright enough for high-resolution spectroscopic follow-up with the Harlan J. Smith telescope at McDonald Observatory. One star is ruled out as a member based on its radial velocity. Abundance analysis of the remaining four kinematic members reveals a good chemical match to NGC 3201 for two of the stars, driven by their similar Al and $alpha$-element abundances. Of the remaining two, one shows no chemical similarity to NGC 3201 and is likely an unassociated Milky Way halo field star, while the other exhibits a similar Al abundance but has somewhat lower $alpha$-element abundances. The chemical tagging of stars in the Gjoll stream to NGC 3201 confirms this association and provides direct proof of the hierarchical formation of the Milky Way.
107 - T. T. Han , L. Chen , C. Cai 2020
When passing through a phase transition, electronic system saves energy by opening energy gaps at the Fermi level. Delineating the energy gap anisotropy provides insights into the origin of the interactions that drive the phase transition. Here, we r eport the angle-resolved photoemission spectroscopy (ARPES) study on the detailed gap anisotropies in both the tetragonal magnetic and superconducting phases in Sr$_{1-x}$Na$_x$Fe$_2$As$_2$. First, we found that the spin-density-wave (SDW) gap is strongly anisotropic in the tetragonal magnetic phase. The gap magnitude correlates with the orbital character of Fermi surface closely. Second, we found that the SDW gap anisotropy is isostructural to the superconducting gap anisotropy regarding to the angular dependence, gap minima locations, and relative gap magnitudes. Our results indicate that the superconducting pairing interaction and magnetic interaction share the same origin. The intra-orbital scattering plays an important role in constructing these interactions resulting in the orbital-selective magnetism and superconductivity in iron-based superconductors.
99 - C. Cai , T. T. Han , Z. G. Wang 2020
Nematic phase intertwines closely with high-Tc superconductivity in iron-based superconductors. Its mechanism, which is closely related to the pairing mechanism of superconductivity, still remains controversial. Comprehensive characterization of how the electronic state reconstructs in the nematic phase is thus crucial. However, most experiments focus only on the reconstruction of band dispersions. Another important characteristic of electronic state, the spectral weight, has not been studied in details so far. Here, we studied the spectral weight transfer in the nematic phase of FeSe$_{0.9}$S$_{0.1}$ using angle-resolved photoemission spectroscopy and in-situ detwinning technique. There are two elliptical electron pockets overlapping with each other orthogonally at the Brillouin zone corner. We found that, upon cooling, one electron pocket loses spectral weight and fades away, while the other electron pocket gains spectral weight and becomes pronounced. Our results show that the symmetry breaking of electronic state is manifested by not only the anisotropic band dispersion but also the band-selective modulation of spectral weight. Our observation completes our understanding of the nematic electronic state, and put strong constraints on the theoretical models. It further provide crucial clues to understand the gap anisotropy and orbital-selective pairing in iron-selenide superconductors.
71 - C. Cai , T. T. Han , Z. G. Wang 2020
Unveiling the driving force for a phase transition is normally difficult when multiple degrees of freedom are strongly coupled. One example is the nematic phase transition in iron-based superconductors. Its mechanism remains controversial due to a co mplex intertwining among different degrees of freedom. In this paper, we report a method for measuring the nematic susceptibly of FeSe$_{0.9}$S$_{0.1}$ using angle-resolved photoemission spectroscopy (ARPES) and an $in$-$situ$ strain-tuning device. The nematic susceptibility is characterized as an energy shift of band induced by a tunable uniaxial strain. We found that the temperature-dependence of the nematic susceptibility is strongly momentum dependent. As the temperature approaches the nematic transition temperature from the high temperature side, the nematic susceptibility remains weak at the Brillouin zone center while showing divergent behavior at the Brillouin zone corner. Our results highlight the complexity of the nematic order parameter in the momentum space, which provides crucial clues to the driving mechanism of the nematic phase transition. Our experimental method which can directly probe the electronic susceptibly in the momentum space provides a new way to study the complex phase transitions in various materials.
We present a detailed abundance analysis of the three brightest member stars at the top of the giant branch of the ultra-faint dwarf galaxy Grus~II. All stars exhibit a higher than expected $mathrm{[Mg/Ca]}$ ratio compared to metal-poor stars in othe r ultra-faint dwarf galaxies and in the Milky Way halo. Nucleosynthesis in high mass ($geqslant 20$M$_odot$) core-collapse supernovae has been shown to create this signature. The abundances of this small sample (3) stars suggest the chemical enrichment of Grus~II could have occurred through substantial high-mass stellar evolution and is consistent with the framework of a top-heavy initial mass function. However, with only three stars it can not be ruled out that the abundance pattern is the result of a stochastic chemical enrichment at early times in the galaxy. The most metal-rich of the three stars also possesses a small enhancement in rapid neutron-capture ($r$-process) elements. The abundance pattern of the $r$-process elements in this star matches the scaled $r$-process pattern of the solar system and $r$-process enhanced stars in other dwarf galaxies and in the Milky Way halo, hinting at a common origin for these elements across a range of environments. All current proposed astrophysical sites of $r$-process element production are associated with high-mass stars, thus the possible top-heavy initial mass function of Grus~II would increase the likelihood of any of these events occurring. The time delay between the $alpha$ and $r$-process element enrichment of the galaxy favors a neutron star merger as the origin of the $r$-process elements in Grus~II.
The detailed chemical composition of most metal-poor halo stars has been found to be highly uniform, but a minority of stars exhibit dramatic enhancements in their abundances of heavy neutron-capture elements and/or of carbon. The key question for Ga lactic chemical evolution models is whether these peculiarities reflect the composition of the natal clouds, or if they are due to later mass transfer of processed material from a binary companion. If the former case applies, the observed excess of certain elements was implanted within selected clouds in the early ISM from a production site at interstellar distances. Our aim is to determine the frequency and orbital properties of binaries among these chemically peculiar stars. This information provides the basis for deciding whether mass transfer from a binary companion is necessary and sufficient to explain their unusual compositions. This paper discusses our study of a sample of 17 moderately (r-I) and highly (r-II) r-process-element enhanced VMP and EMP stars. High-resolution, low signal-to-noise spectra of the stars were obtained at roughly monthly intervals over 8 years with the FIES spectrograph at the Nordic Optical Telescope. From these spectra, radial velocities with an accuracy of ~100 m/s were determined by cross-correlation against an optimized template. 14 of the programme stars exhibit no significant RV variation over this period, while 3 are binaries with orbits of typical eccentricity for their periods, resulting in a normal binary frequency of ~18+-6% for the sample. Our results confirm our preliminary conclusion from 2011, based on partial data, that the chemical peculiarity of the r-I and r-II stars is not caused by any putative binary companions. Instead, it was imprinted on the natal molecular clouds of these stars by an external, distant source. Models of the ISM in early galaxies should account for such mechanisms.
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