It has recently been realized that the first-order moment of the Berry curvature, namely the Berry curvature dipole (BCD) can give rise to non-linear current in a wide variety of time-reversal invariant and non-centrosymmetric materials. While the BC
D in two-dimensional Dirac systems is known to be finite only in the presence of either substantial spin-orbit coupling where low-energy Dirac quasiparticles form tilted cones or higher order warping of the Fermi surface, we argue that the low-energy Dirac quasiparticles arising from the merging of a pair of Dirac points without any tilt or warping of the Fermi surface can lead to a non-zero BCD. Remarkably, in such systems, the BCD is found to be independent of Dirac velocity as opposed to the Dirac dispersion with a tilt or warping effects. We further show that the proposed systems can naturally host helicity-dependent photocurrent due to their linear momentum-dependent Berry curvatures. Finally, we discuss an important byproduct of this work, i.e., nonlinear anomalous Nernst effect as a second-order thermal response.
The manifestation of chiral anomaly in Weyl semimetals typically relies on the observation of longitudinal magnetoconductance (LMC) along with the planar Hall effect, with a specific magnetic field and angle dependence. Here we solve the Boltzmann eq
uation in the semiclassical regime for a prototype of a Weyl semimetal, allowing for both intravalley and intervalley scattering, along with including effects from the orbital magnetic moment (OMM), in a geometry where the electric and magnetic fields are not necessarily parallel to each other. We construct the phase diagram in the relevant parameter space that describes the shift from positive to negative LMC in the presence of OMM and sufficiently strong intervalley scattering, as has been recently pointed out for only parallel electric and magnetic fields. On the other hand, we find that the chiral anomaly contribution to the planar Hall effect always remains positive (unlike the LMC) irrespective of the inclusion or exclusion of OMM, or the strength of the intervalley scattering. Our predictions can be directly tested in experiments, and may be employed as new diagnostic procedures to verify chiral anomaly in Weyl systems.
We theoretically investigate the optical activity of three dimensional Dirac semimetals (DSMs) using circular dichroism (CD). We show that DSMs in the presence of a magnetic field in any one of the mirror-symmetric planes of the materials exhibit a n
otable dichroic behavior. In particular, for different orientations of the light field with respect to the mirror-symmetric plane, the CD in type-II DSMs can detect the presence of mirror anomaly by showing sharply distinct patterns at the mirror-symmetric angle. Interestingly, CD can also distinguish type-II DSMs having only one Dirac point at a time-reversal invariant momentum from type-I DSMs with a pair of Dirac points on the rotation axis of the crystals.
We propose a way to observe the chiral magnetic effect in non-centrosymmetric Weyl semimetals under the action of strong electric field, via the non-linear part of their I-V characteristic that is odd in the external magnetic field, or odd-in-magneti
c field voltages in electrically open circuits. This effect relies on valley-selective heating in such materials, which in general leads to nonequilibrium valley population imbalances. In the presence of an external magnetic field, such a valley-imbalanced Weyl semimetal will in general develop an electric current along the direction of the magnetic field -- the chiral magnetic effect. We also discuss a specific experimental setup to observe the chiral magnetic effect of hot electrons.
We study the dynamic chiral magnetic conductivity (DCMC) and natural optical activity in an inversion-broken tilted Weyl semimetal (WSM). Starting from the Kubo formula, we derive the analytical expressions for the DCMC for two different directions o
f the incident electromagnetic wave. We show that the angle of rotation of the plane of polarization of the transmitted wave exhibits remarkable anisotropic behavior and is larger along the tilt direction. This striking anisotropy of DCMC which results in anisotropic optical activity and rotary power, can be experimentally observed as a topological magneto-electric effect of inversion-broken tilted WSMs. Finally, using the low energy Hamiltonian, we show that the DCMC follows the universal $frac{1}{omega^2}$ decay in the high frequency regime. In the low frequency regime, however, the DCMC shows sharp peaks at the tilt dependent effective chemical potentials of the left-handed and right-handed Weyl points. This can serve as a signature to distinguish between the type-I and type-II Weyl semimetals.
In addition to the well known chiral anomaly, Dirac semimetals have been argued to exhibit mirror anomaly, close analogue to the parity anomaly of ($2+1$)-dimensional massive Dirac fermions. The observable response of such anomaly is manifested in a
singular step-like anomalous Hall response across the mirror-symmetric plane in the presence of a magnetic field. Although this result seems to be valid in type-II Dirac semimetals (strictly speaking, in the linearized theory), we find that type-I Dirac semimetals do not possess such an anomaly in anomalous Hall response even at the level of the linearized theory. In particular, we show that the anomalous Hall response continuously approaches zero as one approaches the mirror symmetric angle in a type-I Dirac semimetal as opposed to the singular Hall response in a type-II Dirac semimetal. Moreover, we show that, under certain condition, the anomalous Hall response may vanish in a linearized type-I Dirac semimetal, even in the presence of time reversal symmetry breaking.
Recent experimental observations of magnetization plateau in metallic tetraboride $textrm{TmB}_{4}$ have created a lot of interest in these class of materials. Hysteretic longitudinal resistance and anomalous Hall Effect are other remarkable features
in the rare-earth tetraborides which represent experimental realizations of Archimedean Shastry-Sutherland (SSL) lattice. Electronic band structures, calculated under GGA and GGA+SO approximations, show that $textrm{TmB}_{4}$ is a narrow band system with considerable correlation in its f-level. Strong correlation effects in this system are studied under single-site dynamical mean field theory (DMFT) [LDA+DMFT scheme] using multi-orbital generalization of iterated perturbation theory (MO-IPT). Pseudo-gap behaviour in spectral function and non-Fermi liquid behaviour of self-energy shows non-trivial strong correlation effects present in this geometrically frustrated metallic magnets. We also consider the extant, heather-to-neglected, strong atomic spin-orbit coupling (SOC) effects. While there is a significant change in the topology of the Fermi surface in the presence of SOC, the non-Fermi liquid behavior survives. The system can be modelled by an effective two orbital spinless Falicov-Kimball model together with two free band like states.
Strong light-matter interactions in layered transition metal dichalcogenides (TMDs) open up vivid possibilities for novel exciton-based devices. The optical properties of TMDs are dominated mostly by the tightly bound excitons and more complex quasip
articles, the biexcitons. Instead of physically exfoliated monolayers, the solvent-mediated chemical exfoliation of these 2D crystals is a cost-effective, large-scale production method suitable for real device applications. We explore the ultrafast excitonic processes in WS$_{2}$ dispersion using broadband femtosecond pump-probe spectroscopy at room temperature. We detect the biexcitons experimentally and calculate their binding energies, in excellent agreement with earlier theoretical predictions. Using many-body physics, we show that the excitons act like Weiner-Mott excitons and explain the origin of excitons via first-principles calculations. Our detailed time-resolved investigation provides ultrafast radiative and non-radiative lifetimes of excitons and biexcitons in WS$_{2}$. Indeed, our results demonstrate the potential for excitonic quasiparticle-controlled TMDs-based devices operating at room temperature.
Weyl semimetals are intriguing topological states of matter that support various anomalous magneto-transport phenomena. One such phenomenon is a negative longitudinal ($mathbf{ abla} T parallel mathbf{B}$) magneto-thermal resistivity, which arises du
e to chiral magnetic effect (CME). In this paper we show that another fascinating effect induced by CME is the planar thermal Hall effect (PTHE), i.e., appearance of an in-plane transverse temperature gradient when the current due to $mathbf{ abla} T$ and the magnetic field $mathbf{B}$ are not aligned with each other. Using semiclassical Boltzmann transport formalism in the relaxation time approximation we compute both longitudinal magneto-thermal conductivity (LMTC) and planar thermal Hall conductivity (PTHC) for a time reversal symmetry breaking WSM. We find that both LMTC and PTHC are quadratic in B in type-I WSM whereas each follows a linear-B dependence in type-II WSM in a configuration where $mathbf{ abla} T$ and B are applied along the tilt direction. In addition, we investigate the Wiedemann-Franz law for an inversion symmetry broken WSM (e.g., WTe$_{2}$) and find that this law is violated in these systems due to both chiral anomaly and CME.
Negative longitudinal magnetoresistance, in the presence of an external magnetic field parallel to the direction of an applied current, has recently been experimentally verified in Weyl semimetals and topological insulators in the bulk conduction lim
it. The appearance of negative longitudinal magnetoresistance in topological semimetals is understood as an effect of chiral anomaly, whereas it is not well-defined in topological insulators. Another intriguing phenomenon, planar Hall effect - appearance of a transverse voltage in the plane of applied co-planar electric and magnetic fields not perfectly aligned to each other, a configuration in which the conventional Hall effect vanishes, has recently been suggested to exist in Weyl semimetals. In this paper we present a quasi-classical theory of planar Hall effect of a three-dimensional topological insulator in the bulk conduction limit. Starting from Boltzmann transport equations we derive the expressions for planar Hall conductivity and longitudinal magnetoconductivity in topological insulators and show the important roles played by the orbital magnetic moment for the appearance of planar Hall effect. Our theoretical results predict specific experimental signatures for topological insulators that can be directly checked in experiments.
