We provide a theoretical framework describing slow-light polaritons interacting via atomic Rydberg states. We use a diagrammatic method to analytically derive the scattering properties of two polaritons. We identify parameter regimes where polariton-
polariton interactions are repulsive. Furthermore, in the regime of attractive interactions, we identify multiple two-polariton bound states, calculate their dispersion, and study the resulting scattering resonances. Finally, the two-particle scattering properties allow us to derive the effective low-energy many-body Hamiltonian. This theoretical platform is applicable to ongoing experiments.
We describe the effect of thermal motion and buffer-gas collisions on a four-level closed N system interacting with strong pump(s) and a weak probe. This is the simplest system that experiences electromagnetically induced absorption (EIA) due to tran
sfer of coherence via spontaneous emission from the excited to ground state. We investigate the influence of Doppler broadening, velocity-changing collisions (VCC), and phase-changing collisions (PCC) with a buffer gas on the EIA spectrum of optically active atoms. In addition to exact expressions, we present an approximate solution for the probe absorption spectrum, which provides physical insight into the behavior of the EIA peak due to VCC, PCC, and wave-vector difference between the pump and probe beams. VCC are shown to produce a wide pedestal at the base of the EIA peak, which is scarcely affected by the pump-probe angular deviation, whereas the sharp central EIA peak becomes weaker and broader due to the residual Doppler-Dicke effect. Using diffusion-like equations for the atomic coherences and populations, we construct a spatial-frequency filter for a spatially structured probe beam and show that Ramsey narrowing of the EIA peak is obtained for beams of finite width.
Self-similar solutions of the coherent diffusion equation are derived and measured. The set of real similarity solutions is generalized by the introduction of a nonuniform phase surface, based on the elegant Gaussian modes of optical diffraction. In
an experiment of light storage in a gas of diffusing atoms, a complex initial condition is imprinted, and its diffusion dynamics is monitored. The self-similarity of both the amplitude and the phase pattern is demonstrated, and an algebraic decay associated with the mode order is measured. Notably, as opposed to a regular diffusion spreading, a self-similar contraction of a special subset of the solutions is predicted and observed.
The population distribution within the ground-state of an atomic ensemble is of large significance in a variety of quantum optics processes. We present a method to reconstruct the detailed population distribution from a set of absorption measurements
with various frequencies and polarizations, by utilizing the differences between the dipole matrix elements of the probed transitions. The technique is experimentally implemented on a thermal rubidium vapor, demonstrating a population-based analysis in two optical pumping examples. The results are used to verify and calibrate an elaborated numerical model, and the limitations of the reconstruction scheme which result from the symmetry properties of the dipole matrix elements are discussed.
We experimentally demonstrate the manipulation of optical diffraction, utilizing the atomic thermal motion in a hot vapor medium of electromagnetically-induced transparency (EIT). By properly tuning the EIT parameters, the refraction induced by the a
tomic motion may completely counterbalance the paraxial free-space diffraction and by that eliminates the effect of diffraction for arbitrary images. By further manipulation, the diffraction can be doubled, biased asymmetrically to induced deflection, or even reversed. The latter allows an experimental implementation of an analogy to a negative-index lens.
The probability of a random walker to return to its starting point in dimensions one and two is unity, a theorem first proven by G. Polya. The recurrence probability -- the probability to be found at the origin at a time t, is a power law with a crit
ical exponent d/2 in dimensions d=1,2. We report an experiment that directly measures the Laplace transform of the recurrence probability in one dimension using Electromagnetically Induced Transparency (EIT) of coherent atoms diffusing in a vapor-cell filled with buffer gas. We find a regime where the limiting form of the complex EIT spectrum is universal and only depends on the effective dimensionality in which the random recurrence takes place. In an effective one-dimensional diffusion setting, the measured spectrum exhibits power law dependence over two decades in the frequency domain with a critical exponent of 0.56 close to the expected value 0.5. Possible extensions to more elaborate diffusion schemes are briefly discussed.
We present a scheme for eliminating the optical diffraction of slow-light in a thermal atomic medium of electromagnetically induced transparency. Nondiffraction is achieved for an arbitrary paraxial image by manipulating the susceptibility in momentu
m space, in contrast to the common approach, which employs guidance of specific modes by manipulating the susceptibility in real space. For negative two-photon detuning, the moving atoms drag the transverse momentum components unequally, resulting in a Doppler trapping of light by atoms in two dimensions.
Two-photon processes that involve different sub-levels of the ground state of an atom, are highly sensitive to depopulation and decoherence within the ground state. For example, the spectral width of electromagnetically induced transparency resonance
s in $Lambda-$type system, are strongly affected by the ground state depopulation and decoherence rates. We present a direct measurement of decay rates between hyperfine and Zeeman sub-levels in the ground state of $^{87}$Rb vapor. Similar to the relaxation-in-the-dark technique, pumping lasers are used to pre-align the atomic vapor in a well defined quantum state. The free propagation of the atomic state is monitored using a Ramsey-like method. Coherence times in the range 1-10 ms were measured for room temperature atomic vapor. In the range of the experimental parameters used in this study, the dominant process inducing Zeeman decoherence is the spin-exchange collisions between rubidium atoms.
Reversible and coherent storage of light in atomic medium is a key-stone of future quantum information applications. In this work, arbitrary two-dimensional images are slowed and stored in warm atomic vapor for up to 30 $mu$s, utilizing electromagnet
ically induced transparency. Both the intensity and the phase patterns of the optical field are maintained. The main limitation on the storage resolution and duration is found to be the diffusion of atoms. A techniqueanalogous to phase-shift lithography is employed to diminish the effect of diffusion on the visibility of the reconstructed image.
We present a theoretical model for electromagnetically induced transparency (EIT) in vapor, that incorporates atomic motion and velocity-changing collisions into the dynamics of the density-matrix distribution. Within a unified formalism we demonstra
te various motional effects, known for EIT in vapor: Doppler-broadening of the absorption spectrum; Dicke-narrowing and time-of-flight broadening of the transmission window for a finite-sized probe; Diffusion of atomic coherence during storage of light and diffusion of the light-matter excitation during slow-light propagation; and Ramsey-narrowing of the spectrum for a probe and pump beams of finite-size.
