We demonstrate an unseeded, multimode four-wave mixing process in hot $^{85}$Rb vapor, using two pump beams of the same frequency that cross at a small angle. This results in the simultaneous fulfillment of multiple phase-matching conditions that rei
nforce one another to produce four intensity-stabilized bright output modes at two different frequencies. Each generated photon is directly correlated to exactly two others, resulting in the preferred four-mode output, in contrast to other multimode four-wave mixing experiments. This provides significant insight into the optimal configuration of the output multimode squeezed and entangled states generated in such four-wave mixing systems. We examine the power, temperature and frequency dependence of this new output and compare to the conical four-wave mixing emission from a single pump beam. The generated beams are spatially separated, allowing a natural distribution for potential use in quantum communication and secret-sharing protocols.
We demonstrate a new four-wave mixing (4WM) geometry based on structured light. By utilizing near-field diffraction through a narrow slit, the pump beam is asymmetrically structured to modify the phase matching condition, generating multi-mode output
in both the spatial and frequency domains. We show that the frequency parameter enables selection of various spatial-mode outputs, including a twin-beam geometry which preserves relative intensity squeezing shared between the two beams. The results suggest that the engineering of atomic states via structured light may provide a pathway to a diverse set of quantum resources based on multi-mode squeezed light.
In this manuscript, we demonstrate the ability of nonlinear light-atom interactions to produce tunably non-Gaussian, partially self-healing optical modes. Gaussian spatial-mode light tuned near to the atomic resonances in hot rubidium vapor is shown
to result in non-Gaussian output mode structures that may be controlled by varying either the input beam power or the temperature of the atomic vapor. We show that the output modes exhibit a degree of self-reconstruction after encountering an obstruction in the beam path. The resultant modes are similar to truncated Bessel-Gauss modes that exhibit the ability to self-reconstruct earlier upon propagation than Gaussian modes. The ability to generate tunable, self-reconstructing beams has potential applications to a variety of imaging and communication scenarios.
Whispering gallery mode biosensors allow selective unlabelled detection of single proteins and, combined with quantum limited sensitivity, the possibility for noninvasive realtime observation of motor molecule motion. However, to date technical noise
sources, most particularly low frequency laser noise, have constrained such applications. Here we introduce a new technique for whispering gallery mode sensing based on direct detection of back-scattered light. This experimentally straightforward technique is immune to frequency noise in principle, and further, acts to suppress thermorefractive noise. We demonstrate 27 dB of frequency noise suppression, eliminating frequency noise as a source of sensitivity degradation and allowing an absolute frequency shift sensitivity of 76 kHz. Our results open a new pathway towards single molecule biophysics experiments and ultrasensitive biosensors.
