Experiments have been performed to measure magnetoelectric properties of room temperature spirally ordered Sr3Co2Fe24O41 hexaferrite slabs. The measured properties include the magnetic permeability, the magnetization and the strain all as a function
of the electric field E and the magnetic intensity H. The material hexaferrite Sr3Co2Fe24O41 exhibits broken symmetries for both time reversal and parity. The product of the two symmetries remains unbroken. This is the central feature of these magnetoelectric materials. A simple physical model is proposed to explain the magnetoelectric effect in these materials.
Alternating layers of granular Iron (Fe) and Titanium dioxide (TiO$_{2-delta}$) were deposited on (100) Lanthanum aluminate (LaAlO$_3$) substrates in low oxygen chamber pressure using a controlled pulsed laser ablation deposition technique. The total
thickness of the film was about 200 nm. The films show ferromagnetic behavior for temperatures ranging from 4 to $400 ^oK$. The layered film structure was characterized as p-type magnetic semiconductor at $300 ^oK$ with a carrier density of the order of $10^{20} /cm^3$. The undoped pure TiO$_{2-delta}$ film was characterized as an n-type magnetic semiconductor. The hole carriers were excited at the interface between the granular Fe and TiO$_{2-delta}$ layers similar to holes excited in the metal/n-type semiconductor interface commonly observed in Metal-Oxide-Semiconductor (MOS) devices. The holes at the interface were polarized in an applied magnetic field raising the possibility that these granular MOS structures can be utilized for practical spintronic device applications.
