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Bulk materials possessing a relative electric permittivity $varepsilon$ close to zero exhibit giant Kerr nonlinearities. However, harnessing this response in guided-wave geometries is not straightforward, due to the extreme and counter-intuitive prop erties of epsilon-near-zero materials. Here we investigate, through rigorous calculations of the Kerr nonlinear coefficient, how the remarkable nonlinear properties of such materials can be exploited in several different types of structures, including bulk films, plasmonic nanowires, and metal nanoapertures. We find the largest Kerr nonlinear response when both the modal area and the group velocity are simultaneously minimized, corresponding to omnidirectional field enhancement. The physical insights developed will be key for understanding and engineering nonlinear nanophotonic systems with extreme nonlinearities and point to new design paradigms.
Silicon is an ideal material for on-chip applications, however its poor acoustic properties limit its performance for important optoacoustic applications, particularly for Stimulated Brillouin Scattering (SBS). We theoretically show that silicon inve rse opals exhibit a strongly improved acoustic performance that enhances the bulk SBS gain coefficient by more than two orders of magnitude. We also design a waveguide that incorporates silicon inverse opals and which has SBS gain values that are comparable with chalcogenide glass waveguides. This research opens new directions for opto-acoustic applications in on-chip material systems.
We compute the SBS gain for a metamaterial comprising a cubic lattice of dielectric spheres suspended in a background dielectric material. Theoretical methods are presented to calculate the optical, acoustic, and opto-acoustic parameters that describ e the SBS properties of the material at long wavelengths. Using the electromagnetic and strain energy densities we accurately characterise the optical and acoustic properties of the metamaterial. From a combination of energy density methods and perturbation theory, we recover the appropriate terms of the photoelastic tensor for the metamaterial. We demonstrate that electrostriction is not necessarily the dominant mechanism in the enhancement and suppression of the SBS gain coefficient in a metamaterial, and that other parameters, such as the Brillouin linewidth, can dominate instead. Examples are presented that exhibit an order of magnitude enhancement in the SBS gain as well as perfect suppression.
Using full opto-acoustic numerical simulations, we demonstrate enhancement and suppression of the SBS gain in a metamaterial comprising a subwavelength cubic array of dielectric spheres suspended in a dielectric background material. We develop a gene ral theoretical framework and present several numerical examples using technologically important materials. For As$_2$S$_3$ spheres in silicon, we achieve a gain enhancement of more than an order of magnitude compared to pure silicon, and for GaAs spheres in silicon, full suppression is obtained. The gain for As$_2$S$_3$ glass can also be strongly suppressed by embedding silica spheres. The constituent terms of the gain coefficient are shown to depend in a complex way on the filling fraction. We find that electrostriction is the dominant effect behind the control of SBS in bulk media.
Temporal optical solitons have been the subject of intense research due to their intriguing physics and applications in ultrafast optics and supercontinuum generation. Conventional bright optical solitons result from the interaction of anomalous grou p-velocity dispersion and self-phase modulation. Here we report the discovery of an entirely new class of bright solitons arising purely from the interaction of negative fourth-order dispersion and self-phase modulation, which can occur even for normal group-velocity dispersion. We provide experimental and numerical evidence of shape-preserving propagation and flat temporal phase for the fundamental pure-quartic soliton and periodically modulated propagation for the higher-order pure-quartic solitons. Using analytic theory, we derive the approximate shape of the fundamental pure-quartic soliton exhibiting excellent agreement with our experimental observations. Our discovery, enabled by the unique dispersion of photonic crystal waveguides, could find applications in communications and ultrafast lasers.
We design extremely flexible ultrahigh-Q diamond-based double-heterostructure photonic crystal slab cavities by modifying the refractive index of the diamond. The refractive index changes needed for ultrahigh-Q cavities with $Q ~ 10^7$, are well with in what can be achieved ($Delta n sim 0.02$). The cavity modes have relatively small volumes $V<2 (lambda /n)^3$, making them ideal for cavity quantum electro-dynamic applications. Importantly for realistic fabrication, our design is flexible because the range of parameters, cavity length and the index changes, that enables an ultrahigh-Q is quite broad. Furthermore as the index modification is post-processed, an efficient technique to generate cavities around defect centres is achievable, improving prospects for defect-tolerant quantum architectures.
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