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By means of ab initio calculations we study the effect of O-doping of Au chains containing a nanocontact represented by a Ni atom as a magnetic impurity. In contrast to pure Au chains, we find that with a minimun O-doping the $5d_{xz,yz}$ states of A u are pushed up, crossing the Fermi level. We also find that for certain O configurations, the Ni atom has two holes in the degenerate $3d_{xz,yz}$ orbitals, forming a spin $S=1$ due to a large Hund interaction. The coupling between the $5d_{xz,yz}$ Au bands and the $3d_{xz,yz}$ of Ni states leads to a possible realization of a two-channel $S=1$ Kondo effect. While this kind of Kondo effect is commonly found in bulk systems, it is rarely observed in low dimensions. The estimated Kondo scale of the system lies within the present achievable experimental resolution in transport measurements. Another possible scenario for certain atomic configurations is that one of the holes resides in a $3d_{z^2}$ orbital, leading to a two-stage Kondo effect, the second one with SU(4) symmetry.
We calculate the spectral density and occupations of a system of two capacitively coupled quantum dots, each one connected to its own pair of conducting leads, in a regime of parameters in which the total coupling to the leads for each dot $Gamma_i$ are different. The system has been used recently to perform pseudospin spectroscopy by controlling independently the voltages of the four leads. For an odd number of electrons in the system, $Gamma_1=Gamma_2$, equal dot levels $E_1=E_2$ and sufficiently large interdot repulsion $U_{12}$ the system lies in the SU(4) symmetric point of spin and pseudospin degeneracy in the Kondo regime. In the more realistic case $Gamma_1 eq Gamma_2$, pseudospin degeneracy is broken and the symmetry is reduced to SU(2). Nevertheless we find that the essential features of the SU(4) symmetric case are recovered by appropriately tuning the level difference $delta=E_2-E_1$. The system behaves as an SU(4) Kondo one at low energies. Our results are relevant for experiments which look for signatures of SU(4) symmetry in the Kondo regime of similar systems.
Films of the topological insulator Bi2Se3 are grown by molecular beam epitaxy with in-situ reflection high-energy electron diffraction. The films are shown to be high-quality by X-ray reflectivity and diffraction and atomic-force microscopy. Quantum interference control of photocurrents is observed by excitation with harmonically related pulses and detected by terahertz radiation. The injection current obeys the expected excitation irradiance dependence, showing linear dependence on the fundamental pulse irradiance and square-root irradiance dependence of the frequency-doubled optical pulses. The injection current also follows a sinusoidal relative-phase dependence between the two excitation pulses. These results confirm the third-order nonlinear optical origins of the coherently controlled injection current. Experiments are compared to a tight-binding band structure to illustrate the possible optical transitions that occur in creating the injection current.
A dominant cost for query evaluation in modern massively distributed systems is the number of communication rounds. For this reason, there is a growing interest in single-round multiway join algorithms where data is first reshuffled over many servers and then evaluated in a parallel but communication-free way. The reshuffling itself is specified as a distribution policy. We introduce a correctness condition, called parallel-correctness, for the evaluation of queries w.r.t. a distribution policy. We study the complexity of parallel-correctness for conjunctive queries as well as transferability of parallel-correctness between queries. We also investigate the complexity of transferability for certain families of distribution policies, including, for instance, the Hypercube distribution.
Realizing robust quantum information transfer between long-lived qubit registers is a key challenge for quantum information science and technology. Here we demonstrate unconditional teleportation of arbitrary quantum states between diamond spin qubit s separated by 3 meters. We prepare the teleporter through photon-mediated heralded entanglement between two distant electron spins and subsequently encode the source qubit in a single nuclear spin. By realizing a fully deterministic Bell-state measurement combined with real-time feed-forward we achieve teleportation in each attempt while obtaining an average state fidelity exceeding the classical limit. These results establish diamond spin qubits as a prime candidate for the realization of quantum networks for quantum communication and network-based quantum computing.
68 - Bas Spitters 2013
In the (covariant) topos approach to quantum theory by Heunen, Landsman and Spitters, one associates to each unital C*-algebra, A, a topos T(A) of sheaves on a locale and a commutative C*-algebra, a, within that topos. The Gelfand spectrum of a is a locale S in this topos, which is equivalent to a bundle over the base locale. We further develop this external presentation of the locale S, by noting that the construction of the Gelfand spectrum in a general topos can be described using geometric logic. As a consequence, the spectrum, seen as a bundle, is computed fibrewise. As a by-product of the geometricity of Gelfand spectra, we find an explicit external description of the spectrum whenever the topos is a functor category. As an intermediate result we show that locally perfect maps compose, so that the externalization of a locally compact locale in a topos of sheaves over a locally compact locale is locally compact, too.
We calculate the nonequilibrium conductance of a system of two capacitively coupled quantum dots, each one connected to its own pair of conducting leads. The system has been used recently to perform pseudospin spectroscopy by controlling independentl y the voltages of the four leads. The pseudospin is defined by the orbital occupation of one or the other dot. Starting from the SU(4) symmetric point of spin and pseudospin degeneracy in the Kondo regime, for an odd number of electrons in the system, we show how the conductance through each dot varies as the symmetry is reduced to SU(2) by a pseudo-Zeeman splitting, and as bias voltages are applied to any of the dots. We analize the expected behavior of the system in general, and predict characteristic fingerprint features of the SU(4) to SU(2) crossover that have not been observed so far.
Collinear phase-matched optical rectification is studied in ZnGeP$_{2}$ pumped with near-infrared light. The pump-intensity dependence is presented for three crystal lengths (0.3, 1.0 and 3.0 mm) to determine the effects of linear optical absorption, nonlinear optical absorption and terahertz free-carrier absorption on the generation. Critical parameters such as the coherence length (for velocity matching), dispersion length (for linear pulse broadening) and nonlinear length (for self-phase modulation) are determined for this material. These parameters provide insight into the upper limit of pulse intensity and crystal length required to generate intense terahertz pulse without detriment to the pulse shape. It is found that for 1-mm thick ZnGeP$_{2}$(012), pumped at 1.28 micron with intensity of ~15 GW/cm2 will produce intense undistorted pulses, whereas longer crystals or larger intensities modify the pulse shape to varying degrees. Moreover, phase-matching dispersion maps are presented for the terahertz generation over a large tuning range (1.1-2.4 micron) in longer (3 mm) crystal, demonstrating the phase-matching bandwidth and phase mismatch that leads to fringing associated with multi-pulse interference. All observed results are simulated numerically showing good qualitative agreement.
We calculate the nonequilibrium conductance through a molecule or a quantum dot in which the occupation of the relevant electronic level is coupled with intensity $lambda$ to a phonon mode, and also to two conducting leads. The system is described by the Anderson-Holstein Hamiltonian. We solve the problem using the Keldysh formalism and the non-crossing approximation (NCA) for both, the electron-electron and the electron-phonon interactions. We obtain a moderate decrease of the Kondo temperature $T_K$ with $lambda$ for fixed renormalized energy of the localized level $tilde{E_d}$. The meaning and value of $tilde{E_d}$ are discussed. The spectral density of localized electrons shows in addition to the Kondo peak of width $2 T_K$, satellites of this peak shifted by multiples of the phonon frequency $ omega_0$. The nonequilibrium conductance as a function of bias voltage $V_b$ at small temperatures, also displays peaks at multiples of $omega_0$ in addition to the central dominant Kondo peak near $V_b=0$.
We propose the use of a silicon-core optical fiber for terahertz (THz) waveguide applications. Finite-difference time-domain simulations have been performed based on a cylindrical waveguide with a silicon core and silica cladding. High-resistivity si licon has a flat dispersion over a 0.1 - 3 THz range, making it viable for propagation of tunable narrowband CW THz and possibly broadband picosecond pules of THz radiation. Simulations show the propagation dynamics and the integrated intensity, from which transverse mode profiles and absorption lengths are extraced. It is found that for 140 - 250 micron core diameters the mode is primarily confined to the core, such that the overall absorbance is only slightly less than in bulk polycrystalline silicon.
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