Recent experiments suggest that the superconducting order parameter of Sr$_2$RuO$_4$ has two components. A two-component order parameter has multiple degrees of freedom in the superconducting state that can result in low-energy collective modes or th
e formation of domain walls -- a possibility that would explain a number of experimental observations including the smallness of the time reversal symmetry breaking signal at T$_mathrm{c}$ and telegraph noise in critical current experiments. We perform ultrasound attenuation measurements across the superconducting transition of Sr$_2$RuO$_4$ using resonant ultrasound spectroscopy (RUS). We find that the attenuation for compressional sound increases by a factor of seven immediately below T$_mathrm{c}$, in sharp contrast with what is found in both conventional ($s$-wave) and high-T$_mathrm{c}$ ($d$-wave) superconductors. We find our observations to be most consistent with the presence of domain walls between different configurations of the superconducting state. The fact that we observe an increase in sound attenuation for compressional strains, and not for shear strains, suggests an inhomogeneous superconducting state formed of two distinct, accidentally-degenerate superconducting order parameters that are not related to each other by symmetry. Whatever the mechanism, a factor of seven increase in sound attenuation is a singular characteristic with which any potential theory of the superconductivity in Sr$_2$RuO$_4$ must be reconciled.
Sr$_2$RuO$_4$ has stood as the leading candidate for a spin-triplet superconductor for 26 years. Recent NMR experiments have cast doubt on this candidacy, however, and it is difficult to find a theory of superconductivity that is consistent with all
experiments. What is needed are symmetry-based experiments that can rule out broad classes of possible superconducting order parameters. Here we use resonant ultrasound spectroscopy to measure the entire symmetry-resolved elastic tensor of Sr$_2$RuO$_4$ through the superconducting transition. We observe a thermodynamic discontinuity in the shear elastic modulus $c_{66}$, requiring that the superconducting order parameter is two-component. A two-component $p$-wave order parameter, such as $p_x+i p_y$, naturally satisfies this requirement. As this order parameter appears to be precluded by recent NMR experiments, we suggest that two other two-component order parameters, namely $left{d_{xz},d_{yz}right}$ or $left{d_{x^2-y^2},g_{xy(x^2-y^2)}right}$, are now the prime candidates for the order parameter of Sr$_2$RuO$_4$.
Quantum materials are epitomized by the influence of collective modes upon their macroscopic properties. Relatively few examples exist, however, whereby coherence of the ground-state wavefunction directly contributes to the conductivity. Notable exam
ples include the quantizing effects of high magnetic fields upon the 2D electron gas, the collective sliding of charge density waves subject to high electric fields, and perhaps most notably the macroscopic phase coherence that enables superconductors to carry dissipationless currents. Here we reveal that the low temperature hidden order state of URu$_2$Si$_2$ exhibits just such a connection between the quantum and macroscopic worlds -- under large voltage bias we observe non-linear contributions to the conductivity that are directly analogous to the manifestation of phase slips in one-dimensional superconductors [1], suggesting a complex order parameter for hidden order
Weyl fermions are a new ingredient for correlated states of electronic matter. A key difficulty has been that real materials also contain non-Weyl quasiparticles, and disentangling the experimental signatures has proven challenging. We use magnetic f
ields up to 95 tesla to drive the Weyl semimetal TaAs far into its quantum limit (QL), where only the purely chiral 0th Landau levels (LLs) of the Weyl fermions are occupied. We find the electrical resistivity to be nearly independent of magnetic field up to 50 tesla: unusual for conventional metals but consistent with the chiral anomaly for Weyl fermions. Above 50 tesla we observe a two-order-of-magnitude increase in resistivity, indicating that a gap opens in the chiral LLs. Above 80 tesla we observe strong ultrasonic attenuation below 2 kelvin, suggesting a mesoscopically-textured state of matter. These results point the way to inducing new correlated states of matter in the QL of Weyl semimetals.
Magneto-quantum oscillation experiments in high temperature superconductors show a strong thermally-induced suppression of the oscillation amplitude approaching critical dopings---in support of a quantum critical origin of their phase diagrams. We su
ggest that, in addition to a thermodynamic mass enhancement, these experiments may directly indicate the increasing role of quantum fluctuations that suppress the oscillation amplitude through inelastic scattering. We show that the traditional theoretical approaches beyond Lifshitz-Kosevich to calculate the oscillation amplitude in correlated metals result in a contradiction with the third law of thermodynamics and suggest a way to rectify this problem.
Close to optimal doping, the copper oxide superconductors show strange metal behavior, suggestive of strong fluctuations associated with a quantum critical point. Such a critical point requires a line of classical phase transitions terminating at zer
o temperature near optimal doping inside the superconducting dome. The underdoped region of the temperature-doping phase diagram from which superconductivity emerges is referred to as the pseudogap because evidence exists for partial gapping of the conduction electrons, but so far there is no compelling thermodynamic evidence as to whether the pseudogap is a distinct phase or a continuous evolution of physical properties on cooling. Here we report that the pseudogap in YBCO cuprate superconductors is a distinct phase, bounded by a line of phase transitions. The doping dependence of this line is such that it terminates at zero temperature inside the superconducting dome. From this we conclude that quantum criticality drives the strange metallic behavior and therefore superconductivity in the cuprates.
We describe a variational calculation for the problem of screening of a point charge in a layered correlated metal for dopings close to the Mott transition where the screening is non-linear due to the proximity to the incompressible insulating state.
We find that external charge can induce locally incompressible regions and that the non-linear dependence of the screening on density can induce overscreening in the nearest nearby layers while preserving overall charge neutrality.
We calculate Raman response functions on the Fermi surface in metallic cuprates.
We discuss the necessary symmetry conditions and the different ways in which they can be physically realized for the occurrence of ferromagnetism accompanying the loop current orbital magnetic order observed by polarized neutron-diffraction experimen
ts or indeed any other conceivable principal order in the under-doped phase of cuprates. We contrast the Kerr effect experiments in single crystals observing ferromagnetism with the direct magnetization measurements in large powder samples, which do not observe it. We also suggest experiments to resolve the differences among the experiments, all of which we believe to be correct.
We calculate the screening charge density distribution due to a point charge, such as that of a positive muon ($mu^+$), placed between the planes of a highly anisotropic layered metal. In underdoped hole cuprates the screening charge converts the cha
rge density in the metallic-plane unit cells in the vicinity of the $mu^+$ to nearly its value in the insulating state. The current-loop ordered state observed by polarized neutron diffraction then vanishes in such cells, and also in nearby cells over a distance of order the intrinsic correlation length of the loop-ordered state. This in turn strongly suppresses the loop-current field at the $mu^+$ site. We estimate this suppressed field in underdoped YBa$_2$Cu$_3$O$_{6+x}$ and La$_{2-x}$Sr$_x$CuO$_4$, and find consistency with the observed 0.2--0.3 G field in the former case and the observed upper bound of $sim$0.2 G in the latter case. This resolves the controversy between the neutron diffraction and $mu$SR experiments. The screening calculation also has relevance for the effect of other charge impurities in the cuprates, such as the dopants themselves.
