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Register a new userHigh temperature antiferromagnetism in Yb based heavy fermion systems proximate to a Kondo insulator
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Given the parallelism between the physical properties of Ce and Yb based magnets and heavy fermions due to the electron-hole symmetry, it has been rather odd that the transition temperature of the Yb based compounds is normally very small, as low as $sim$ 1 K or even lower, whereas Ce counterparts may often have the transition temperature well exceeding 10 K. Here, we report our experimental discovery of the transition temperature reaching 20 K for the first time in a Yb based compound at ambient pressure. The Mn substitution at the Al site in an intermediate valence state of $alpha$-YbAlB$_{4}$ not only induces antiferromagnetic transition at a record high temperature of 20 K but also transforms the heavy fermion liquid state in $alpha$-YbAlB$_{4}$ into a highly resistive metallic state proximate to a Kondo insulator.
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Insulating states can be topologically nontrivial, a well-established notion that is exemplified by the quantum Hall effect and topological insulators. By contrast, topological metals have not been experimentally evidenced until recently. In systems with strong correlations, they have yet to be identified. Heavy fermion semimetals are a prototype of strongly correlated systems and, given their strong spin-orbit coupling, present a natural setting to make progress. Here we advance a Weyl-Kondo semimetal phase in a periodic Anderson model on a noncentrosymmetric lattice. The quasiparticles near the Weyl nodes develop out of the Kondo effect, as do the surface states that feature Fermi arcs. We determine the key signatures of this phase, which are realized in the heavy fermion semimetal Ce$_3$Bi$_4$Pd$_3$. Our findings provide the much-needed theoretical foundation for the experimental search of topological metals with strong correlations, and open up a new avenue for systematic studies of such quantum phases that naturally entangle multiple degrees of freedom.
We report on the first study of the noncentrosymmetric ternary carbide YbCoC$_{2}$. Our magnetization, specific heat, resistivity and neutron diffraction measurements consistently show that the system behaves as a heavy-fermion compound, displaying an amplitude-modulated magnetic structure below the Neel temperature reaching $T_{N}$ = 33 K under pressure. Such a large value, being the highest among the Yb-based systems, is explained in the light of our ab initio calculations, which show that the 4f electronic states of Yb have a dual nature -- i.e., due to their strong hybridization with the 3d states of Co, 4f states expose both localized and itinerant properties.
We report results from neutron scattering experiments on single crystals of YbBiPt that demonstrate antiferromagnetic order characterized by a propagation vector, $tau_{rm{AFM}}$ = ($frac{1}{2} frac{1}{2} frac{1}{2}$), and ordered moments that align along the [1 1 1] direction of the cubic unit cell. We describe the scattering in terms of a two-Gaussian peak fit, which consists of a narrower component that appears below $T_{rm{N}}~approx 0.4$ K and corresponds to a magnetic correlation length of $xi_{rm{n}} approx$ 80 $rm{AA}$, and a broad component that persists up to $T^*approx$ 0.7 K and corresponds to antiferromagnetic correlations extending over $xi_{rm{b}} approx$ 20 $rm{AA}$. Our results illustrate the fragile magnetic order present in YbBiPt and provide a path forward for microscopic investigations of the ground states and fluctuations associated with the purported quantum critical point in this heavy-fermion compound.
The Kondo-Spin Glass competition is studied in a theoretical model of a Kondo lattice with an intra-site Kondo type exchange interaction treated within the mean field approximation, an inter-site quantum Ising exchange interaction with random couplings among localized spins and an additional transverse field in the x direction, which represents a simple quantum mechanism of spin flipping. We obtain two second order transition lines from the spin-glass state to the paramagnetic one and then to the Kondo state. For a reasonable set of the different parameters, the two second order transition lines do not intersect and end in two distinct QCP.
We have succeeded in growing single crystals of the heavy-fermion superconductor CeCo(In1-xZnx)5 with x<=0.07. Measurements of specific heat, electrical resistivity, dc magnetization and ac susceptibility revealed that the superconducting (SC) transition temperature Tc decreases from 2.25 K (x=0) to 1.8 K (x=0.05) by doping Zn into CeCoIn5. Furthermore, these measurements indicate a development of a new ordered phase below T_o ~ 2.2 K for x=>0.05, characterized by the reduced magnetization and electrical resistivity in the ordered phase, and the enhancement of specific heat at T_o. This phase transition can be also recognized by the shoulder-like anomaly seen at H_o ~ 55 kOe in the field variations of the magnetization at low temperatures, which is clearly distinguished from the superconducting critical fields Hc2=49 kOe for x=0.05 and 42 kOe for x=0.07. We suggest from these results that the antiferromagnetic (AFM) order is generated by doping Zn, and the interplay between the SC and AFM orders is realized in CeCo(In1-xZnx)5.
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