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Register a new userDualism of the 4f electrons and high-temperature antiferromagnetism of the heavy-fermion compound YbCoC$_{2}$
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We report on the first study of the noncentrosymmetric ternary carbide YbCoC$_{2}$. Our magnetization, specific heat, resistivity and neutron diffraction measurements consistently show that the system behaves as a heavy-fermion compound, displaying an amplitude-modulated magnetic structure below the Neel temperature reaching $T_{N}$ = 33 K under pressure. Such a large value, being the highest among the Yb-based systems, is explained in the light of our ab initio calculations, which show that the 4f electronic states of Yb have a dual nature -- i.e., due to their strong hybridization with the 3d states of Co, 4f states expose both localized and itinerant properties.
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We report results from neutron scattering experiments on single crystals of YbBiPt that demonstrate antiferromagnetic order characterized by a propagation vector, $tau_{rm{AFM}}$ = ($frac{1}{2} frac{1}{2} frac{1}{2}$), and ordered moments that align along the [1 1 1] direction of the cubic unit cell. We describe the scattering in terms of a two-Gaussian peak fit, which consists of a narrower component that appears below $T_{rm{N}}~approx 0.4$ K and corresponds to a magnetic correlation length of $xi_{rm{n}} approx$ 80 $rm{AA}$, and a broad component that persists up to $T^*approx$ 0.7 K and corresponds to antiferromagnetic correlations extending over $xi_{rm{b}} approx$ 20 $rm{AA}$. Our results illustrate the fragile magnetic order present in YbBiPt and provide a path forward for microscopic investigations of the ground states and fluctuations associated with the purported quantum critical point in this heavy-fermion compound.
We report a study on the interplay between antiferromagnetism (AFM) and superconductivity (SC) in a heavy-fermion compound CeRhIn$_5$ under pressure $P=1.75$ GPa. The onset of the magnetic order is evidenced from a clear split of $^{115}$In-NQR spectrum due to the spontaneous internal field below the Neel temperature $T_N=2.5$ K. Simultaneously, bulk SC below $T_c=2.0$ K is demonstrated by the observation of the Meissner diamagnetism signal whose size is the same as in the exclusively superconducting phase. These results indicate that the AFM coexists homogeneously with the SC at a microscopic level.
We report on the anisotropic properties of Pauli-limited superconductivity (SC) and antiferromagnetism (AFM) in the solid solutions CeCo(In_{1-x}Zn_x)_5 (x<=0.07). In CeCo(In_{1-x}Zn_x)_5, the SC transition temperature T_c is continuously reduced from 2.3 K (x=0) to ~1.4 K (x=0.07) by doping Zn, and then the AFM order with the transition temperature of T_N~2.2 K develops for x larger than ~0.05. The present thermal, transport and magnetic measurements under magnetic field B reveal that the substitution of Zn for In yields little change of low-temperature upper critical field mu_0H_{c2} for both the tetragonal a and c axes, while it monotonically reduces the SC transition temperature T_c. In particular, the magnitudes of mu_0H_{c2} at the nominal Zn concentration of x = 0.05 (measured Zn amount of ~0.019) are 11.8 T for B||a and 4.8 T for B||c, which are as large as those of pure compound though T_c is reduced to 80% of that for x=0. We consider that this feature originates from a combination of both an enhanced AFM correlation and a reduced SC condensation energy in these alloys. It is also clarified that the AFM order differently responds to the magnetic field, depending on the field directions. For B||c, the clear anomaly due to the AFM transition is observed up to the AFM critical field of ~5 T in the thermodynamic quantities, whereas it is rapidly damped with increasing B for B||a. We discuss this anisotropic response on the basis of a rich variety of the AFM modulations involved in the Ce115 compounds.
The tilted balance among competing interactions can yield a rich variety of ground states of quantum matter. In most Ce-based heavy fermion systems, this can often be qualitatively described by the famous Doniach phase diagram, owing to the competition between the Kondo screening and the Ruderman-Kittel-Kasuya-Yoshida exchange interaction. Here, we report an unusual pressure-temperature phase diagram beyond the Doniach one in CeCuP2. At ambient pressure, CeCuP2 displays typical heavy-fermion behavior, albeit with a very low carrier density. With lowering temperature, it shows a crossover from a non Fermi liquid to a Fermi liquid at around 2.4 K. But surprisingly, the Kondo coherence temperature decreases with increasing pressure, opposite to that in most Ce-based heavy fermion compounds. Upon further compression, two superconducting phases are revealed. At 48.0 GPa, the transition temperature reaches 6.1 K, the highest among all Ce-based heavy fermion superconductors. We argue for possible roles of valence tuning and fluctuations associated with its special crystal structure in addition to the hybridization effect. These unusual phase diagrams suggest that CeCuP2 is a novel platform for studying the rich heavy fermions physics beyond the conventional Doniach paradigm.
Ce 3d-4f resonant angle-resolved photoemission measurements on CeCoGe$_{1.2}$Si$_{0.8}$ and CeCoSi$_{2}$ have been performed to understand the Fermi surface topology as a function of hybridization strength between Ce 4$f$- and conduction electrons in heavy-fermion systems. We directly observe that the hole-like Ce 4$f$-Fermi surfaces of CeCoSi$_{2}$ is smaller than that of CeCoGe$_{1.2}$Si$_{0.8}$, indicating the evolution of the Ce 4$f$-Fermi surface with the increase of the hybridization strength. In comparision with LDA calculation, the Fermi surface variation cannot be understood even though the overall electronic structure are roughly explained, indicating the importance of strong correlation effects. We also discuss the relation between the Ce 4$f$-Fermi surface variation and the Kondo peaks.
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