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Thermodynamic Properties and Elementary Excitations in Quantum Sine-Gordon Spin System KCuGaF6

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 Added by Toshio Ono
 Publication date 2007
  fields Physics
and research's language is English




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Thermodynamic properties and elementary excitations in $S=1/2$ one-dimensional Heisenberg antiferromagnet KCuGaF$_6$ were investigated by magnetic susceptibility, specific heat and ESR measurements. Due to the Dzyaloshinsky-Moriya interaction with alternating $D$-vectors and/or the staggered $g$-tensor, the staggered magnetic field is induced when subjected to external magnetic field. Specific heat in magnetic field clearly shows the formation of excitation gap, which is attributed to the staggered magnetic field. The specific heat data was analyzed on the basis of the quantum sine-Gordon (SG) model. We observed many ESR modes including one soliton and three breather excitations characteristic of the quantum SG model.

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The material copper pyrimidine dinitrate (Cu-PM) is a quasi-one-dimensional spin system described by the spin-1/2 XXZ Heisenberg antiferromagnet with Dzyaloshinskii-Moriya interactions. Based on numerical results obtained by the density-matrix renormalization group, exact diagonalization, and accompanying electron spin resonance (ESR) experiments we revisit the spin dynamics of this compound in an applied magnetic field. Our calculations for momentum and frequency-resolved dynamical quantities give direct access to the intensity of the elementary excitations at both zero and finite temperature. This allows us to study the system beyond the low-energy description by the quantum sine-Gordon model. We find a deviation from the Lorentz invariant dispersion for the single-soliton resonance. Furthermore, our calculations only confirm the presence of the strongest boundary bound state previously derived from a boundary sine-Gordon field theory, while composite boundary-bulk excitations have too low intensities to be observable. Upon increasing the temperature, we find a temperature-induced crossover of the soliton and the emergence of new features, such as interbreather transitions. The latter observation is confirmed by our ESR experiments on Cu-PM over a wide range of the applied field.
We report the results of muon-spin spectroscopy ($mu^+$SR) measurements on the staggered molecular spin chain [pym-Cu(NO$_3$)$_2$(H$_2$O)$_2$] (pym = pyrimidine), a material previously described using sine-Gordon field theory. Zero-field $mu^+$SR reveals a long range magnetically-ordered ground state below a transition temperature $T_mathrm{N}=0.22(1)$ K. Using longitudinal-field (LF) $mu^+$SR we investigate the dynamic response in applied magnetic fields $0< B < 500$ mT and find evidence for ballistic spin transport. Our LF $mu^+$SR measurements on the chiral spin chain [Cu(pym)(H$_2$O)$_4$]SiF$_6 cdot $H$_2$O instead demonstrate one-dimensional spin diffusion and the distinct spin transport in these two systems likely reflects differences in their magnetic excitations.
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Considering experimental results obtained on three prototype compounds, TMMC, CsCoCl3 (or CsCoBr3) and Cu Benzoate, we discuss the importance of non-linear excitations in the physics of quantum (and classical) antiferromagnetic spin chains.
We follow the evolution of the elementary excitations of the quantum antiferromagnet TlCuCl3 through the pressure-induced quantum critical point, which separates a dimer-based quantum disordered phase from a phase of long-ranged magnetic order. We demonstrate by neutron spectroscopy the continuous emergence in the weakly ordered state of a low-lying but massive excitation corresponding to longitudinal fluctuations of the magnetic moment. This mode is not present in a classical description of ordered magnets, but is a direct consequence of the quantum critical point.
We review the intriguing many-body physics resulting out of the interplay of a single, local impurity and the two-particle interaction in a one-dimensional Fermi system. Even if the underlying homogeneous correlated system is taken to be metallic, this interplay leads to an emergent quantum phase transition between metallic and insulating states. We show that the zero temperature critical point and the universal low-energy physics associated to it, is realized in two different models, the field theoretical local sine-Gordon model and spinless fermions on a lattice with nearest-neighbor hopping and two-particle interaction, as well as in an experimental setup consisting of a highly tunable quantum circuit. Despite the different high-energy physics of the three systems the universal low-energy scaling curves of the conductance as a function of temperature agree up to a very high precision without any free parameter. Overall this provides a convincing example of how emergent universality in complex systems originating from a common underlying quantum critical point establishes a bridge between different fields of physics. In our case between field theory, quantum many-body theory of correlated Fermi systems, and experimental circuit quantum electrodynamics.
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